Effects of Deuterium Isotopes on Pt(II) Complexes and Their Impact on Organic NIR Emitters

Insight into effect of deuterium isotopes on organic near‐IR (NIR) emitters was explored by the use of self‐assembled Pt(II) complexes H‐3‐f and HPh‐3‐f, and their deuterated analogues D‐3‐f and DPh‐3‐f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission...

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Published inAngewandte Chemie International Edition Vol. 63; no. 10; pp. e202317571 - n/a
Main Authors Wang, Sheng‐Fu, Zhou, Dong‐Ying, Kuo, Kai‐Hua, Wang, Chih‐Hsing, Hung, Chieh‐Ming, Yan, Jie, Liao, Liang‐Sheng, Hung, Wen‐Yi, Chi, Yun, Chou, Pi‐Tai
Format Journal Article
LanguageEnglish
Published WEINHEIM Wiley 04.03.2024
Wiley Subscription Services, Inc
EditionInternational ed. in English
Subjects
Chemistry
Chemistry, Multidisciplinary
Deuteration
Deuterium
Emission
Emissions
Emitters
Isotope effect
Isotopes
Near Infrared
Near infrared radiation
Organic Light Emitting Diodes
Photoluminescence
Photons
Physical Sciences
Pt(II) Complexes
Radiance
Science & Technology
Self-assembly
Thin films
Deuterium
LIGHT-EMITTING-DIODES
Organic Light Emitting Diodes
Isotope effect
Near Infrared
OLEDS
Pt(II) Complexes
EMISSION
Near Infrared, Pt(II) Complexes, Deuterium, Isotope effect, Organic Light Emitting Diodes
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Abstract Insight into effect of deuterium isotopes on organic near‐IR (NIR) emitters was explored by the use of self‐assembled Pt(II) complexes H‐3‐f and HPh‐3‐f, and their deuterated analogues D‐3‐f and DPh‐3‐f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H‐3‐f and D‐3‐f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh‐3‐f (800 nm, 50 %) and DPh‐3‐f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near‐infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D‐3‐f and DPh‐3‐f emitters attain EQEmax of 15.5 % (radiance 31,287 mW Sr−1 m−2) and 16.6 % (radiance of 32,279 mW Sr−1 m−2) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm. We have developed general guidelines for the effect of deuterium isotopes on the NIR emission efficiency of Pt(II) complexes and common organic NIR emitters. Also, in this study the NIR OLED based on deuterated Pt(II) complex DPh‐3‐f emitter attains 796 nm electroluminescence with EQEmax of 16.6 % and radiance of 32,279 mW Sr−1 m−2, which sets new records for NIR OLEDs of >750 nm.
AbstractList Insight into effect of deuterium isotopes on organic near-IR (NIR) emitters was explored by the use of self-assembled Pt(II) complexes H-3-f and HPh-3-f, and their deuterated analogues D-3-f and DPh-3-f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H-3-f and D-3-f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29% and 50%, respectively. Distinction in PLQY is also observed for HPh-3-f (800 nm, 50%) and DPh-3-f (798 nm, 67%). We then elucidated the theoretical differences in the impact on near-infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D-3-f and DPh-3-f emitters attain EQEmax of 15.5% (radiance 31,287 mW Sr-1 m-2) and 16.6% (radiance of 32,279 mW Sr-1 m-2) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of > 750 nm.
Insight into effect of deuterium isotopes on organic near-IR (NIR) emitters was explored by the use of self-assembled Pt(II) complexes H-3-f and HPh-3-f, and their deuterated analogues D-3-f and DPh-3-f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H-3-f and D-3-f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh-3-f (800 nm, 50 %) and DPh-3-f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near-infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D-3-f and DPh-3-f emitters attain EQEmax of 15.5 % (radiance 31,287 mW Sr-1  m-2 ) and 16.6 % (radiance of 32,279 mW Sr-1  m-2 ) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm.Insight into effect of deuterium isotopes on organic near-IR (NIR) emitters was explored by the use of self-assembled Pt(II) complexes H-3-f and HPh-3-f, and their deuterated analogues D-3-f and DPh-3-f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H-3-f and D-3-f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh-3-f (800 nm, 50 %) and DPh-3-f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near-infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D-3-f and DPh-3-f emitters attain EQEmax of 15.5 % (radiance 31,287 mW Sr-1  m-2 ) and 16.6 % (radiance of 32,279 mW Sr-1  m-2 ) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm.
Insight into effect of deuterium isotopes on organic near-IR (NIR) emitters was explored by the use of self-assembled Pt(II) complexes H-3-f and HPh-3-f, and their deuterated analogues D-3-f and DPh-3-f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at similar to 810 nm, H-3-f and D-3-f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh-3-f (800 nm, 50 %) and DPh-3-f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near-infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D-3-f and DPh-3-f emitters attain EQE(max) of 15.5 % (radiance 31,287 mW Sr-1 m(-2)) and 16.6 % (radiance of 32,279 mW Sr-1 m(-2)) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm.
Insight into effect of deuterium isotopes on organic near‐IR (NIR) emitters was explored by the use of self‐assembled Pt(II) complexes H‐3‐f and HPh‐3‐f, and their deuterated analogues D‐3‐f and DPh‐3‐f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H‐3‐f and D‐3‐f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh‐3‐f (800 nm, 50 %) and DPh‐3‐f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near‐infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D‐3‐f and DPh‐3‐f emitters attain EQE max of 15.5 % (radiance 31,287 mW Sr −1 m −2 ) and 16.6 % (radiance of 32,279 mW Sr −1 m −2 ) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm.
Insight into effect of deuterium isotopes on organic near‐IR (NIR) emitters was explored by the use of self‐assembled Pt(II) complexes H‐3‐f and HPh‐3‐f, and their deuterated analogues D‐3‐f and DPh‐3‐f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H‐3‐f and D‐3‐f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh‐3‐f (800 nm, 50 %) and DPh‐3‐f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near‐infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D‐3‐f and DPh‐3‐f emitters attain EQEmax of 15.5 % (radiance 31,287 mW Sr−1 m−2) and 16.6 % (radiance of 32,279 mW Sr−1 m−2) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm.
Insight into effect of deuterium isotopes on organic near‐IR (NIR) emitters was explored by the use of self‐assembled Pt(II) complexes H‐3‐f and HPh‐3‐f, and their deuterated analogues D‐3‐f and DPh‐3‐f, respectively (Scheme 2). In vacuum deposited thin film, albeit having nearly identical emission spectral feature maximized at ~810 nm, H‐3‐f and D‐3‐f exhibit remarkable difference in photoluminescence quantum yield (PLQY) of 29 % and 50 %, respectively. Distinction in PLQY is also observed for HPh‐3‐f (800 nm, 50 %) and DPh‐3‐f (798 nm, 67 %). We then elucidated the theoretical differences in the impact on near‐infrared (NIR) luminescence between Pt(II) complexes and organic small molecules upon deuteration. The results establish a general guideline for the deuteration on NIR emission efficiency. From a perspective of practical application, NIR OLEDs based on D‐3‐f and DPh‐3‐f emitters attain EQEmax of 15.5 % (radiance 31,287 mW Sr−1 m−2) and 16.6 % (radiance of 32,279 mW Sr−1 m−2) at 764 nm and 796 nm, respectively, both of which set new records for NIR OLEDs of >750 nm. We have developed general guidelines for the effect of deuterium isotopes on the NIR emission efficiency of Pt(II) complexes and common organic NIR emitters. Also, in this study the NIR OLED based on deuterated Pt(II) complex DPh‐3‐f emitter attains 796 nm electroluminescence with EQEmax of 16.6 % and radiance of 32,279 mW Sr−1 m−2, which sets new records for NIR OLEDs of >750 nm.
ArticleNumber 202317571
Author Chou, Pi‐Tai
Liao, Liang‐Sheng
Chi, Yun
Hung, Wen‐Yi
Kuo, Kai‐Hua
Yan, Jie
Zhou, Dong‐Ying
Wang, Chih‐Hsing
Hung, Chieh‐Ming
Wang, Sheng‐Fu
Author_xml – sequence: 1
  givenname: Sheng‐Fu
  surname: Wang
  fullname: Wang, Sheng‐Fu
  organization: National Taiwan University
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  givenname: Dong‐Ying
  surname: Zhou
  fullname: Zhou, Dong‐Ying
  organization: Soochow University
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  surname: Kuo
  fullname: Kuo, Kai‐Hua
  organization: National Taiwan University
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  givenname: Chih‐Hsing
  surname: Wang
  fullname: Wang, Chih‐Hsing
  organization: National Taiwan University
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  givenname: Chieh‐Ming
  surname: Hung
  fullname: Hung, Chieh‐Ming
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Issue 10
Keywords Deuterium
LIGHT-EMITTING-DIODES
Organic Light Emitting Diodes
Isotope effect
Near Infrared
OLEDS
Pt(II) Complexes
EMISSION
Near Infrared, Pt(II) Complexes, Deuterium, Isotope effect, Organic Light Emitting Diodes
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Snippet Insight into effect of deuterium isotopes on organic near‐IR (NIR) emitters was explored by the use of self‐assembled Pt(II) complexes H‐3‐f and HPh‐3‐f, and...
Insight into effect of deuterium isotopes on organic near-IR (NIR) emitters was explored by the use of self-assembled Pt(II) complexes H-3-f and HPh-3-f, and...
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StartPage e202317571
SubjectTerms Chemistry
Chemistry, Multidisciplinary
Deuteration
Deuterium
Emission
Emissions
Emitters
Isotope effect
Isotopes
Near Infrared
Near infrared radiation
Organic Light Emitting Diodes
Photoluminescence
Photons
Physical Sciences
Pt(II) Complexes
Radiance
Science & Technology
Self-assembly
Thin films
Title Effects of Deuterium Isotopes on Pt(II) Complexes and Their Impact on Organic NIR Emitters
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.202317571
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=Summon&SrcAuth=ProQuest&DestApp=WOS&DestLinkType=FullRecord&UT=001157629000001
https://www.ncbi.nlm.nih.gov/pubmed/38230818
https://www.proquest.com/docview/2931483218
https://www.proquest.com/docview/2915987969
Volume 63
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