Removal of Cd(II) and Cu(II) from Aqueous Solution by Na+-Modified Pisha Sandstone

Heavy metals have caused serious environmental issues, which are enriched during open-cast coal mining. It is urgent to develop sustainable remediation materials to protect and restore the contaminated soil and aquifers in mining areas. The feasibility of applying Pisha sandstone (PS) and Na+-modifi...

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Published inJournal of chemistry Vol. 2020; no. 2020; pp. 1 - 13
Main Authors Zhang, Zhiqin, Fan, Chenbin, Peng, Qi, Cui, Yongxing, Wang, Xia, Zhang, Xingchang
Format Journal Article
LanguageEnglish
Published Cairo, Egypt Hindawi Publishing Corporation 2020
Hindawi
John Wiley & Sons, Inc
Wiley
Subjects
Adsorbents
Adsorption
Aqueous solutions
Aquifers
Coal mines
Coal mining
Endothermic reactions
Environmental impact
Equilibrium
Heavy metals
Isotherms
Kinetics
Linearity
Metals
Minerals
Reaction kinetics
Remediation
Sandstone
Soil contamination
Soil remediation
Studies
Surface water
China
Japan
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Abstract Heavy metals have caused serious environmental issues, which are enriched during open-cast coal mining. It is urgent to develop sustainable remediation materials to protect and restore the contaminated soil and aquifers in mining areas. The feasibility of applying Pisha sandstone (PS) and Na+-modified Pisha sandstone (Na-PS) for adsorption of heavy metals was evaluated. Na-PS exhibited maximum Cd(II) and Cu(II) removal rates of 65.9% and 99.8%, respectively, exceeding the corresponding values for PS (8.2% and 1.3%, respectively) in 1 × 10−3 M solution. Efficient heavy metals adsorption occurred in the pH range 5.0–6.0. The adsorption of Cu(II) and Cd(II) on PS and Na-PS was characterized by kinetic models and adsorption isotherms and was well represented by pseudo-second-order kinetics (R2 > 0.99) and the Langmuir and Freundlich isotherm models. The values of the thermodynamic parameters indicated that the interactions were spontaneous endothermic reactions. Binary solutions adsorption isotherms indicated that the linearity of the adsorption amount and initial concentration of Cu(II) and Cd(II) was better in certain ranges and the adsorbents were selective towards Cu(II) rather than Cd(II). Therefore, PSs can be used as excellent adsorbents for Cu(II) and Cd(II) remediation from contaminated surface water.
AbstractList Heavy metals have caused serious environmental issues, which are enriched during open-cast coal mining. It is urgent to develop sustainable remediation materials to protect and restore the contaminated soil and aquifers in mining areas. The feasibility of applying Pisha sandstone (PS) and Na+-modified Pisha sandstone (Na-PS) for adsorption of heavy metals was evaluated. Na-PS exhibited maximum Cd(II) and Cu(II) removal rates of 65.9% and 99.8%, respectively, exceeding the corresponding values for PS (8.2% and 1.3%, respectively) in 1 × 10−3 M solution. Efficient heavy metals adsorption occurred in the pH range 5.0–6.0. The adsorption of Cu(II) and Cd(II) on PS and Na-PS was characterized by kinetic models and adsorption isotherms and was well represented by pseudo-second-order kinetics (R2 > 0.99) and the Langmuir and Freundlich isotherm models. The values of the thermodynamic parameters indicated that the interactions were spontaneous endothermic reactions. Binary solutions adsorption isotherms indicated that the linearity of the adsorption amount and initial concentration of Cu(II) and Cd(II) was better in certain ranges and the adsorbents were selective towards Cu(II) rather than Cd(II). Therefore, PSs can be used as excellent adsorbents for Cu(II) and Cd(II) remediation from contaminated surface water.
Heavy metals have caused serious environmental issues, which are enriched during open-cast coal mining. It is urgent to develop sustainable remediation materials to protect and restore the contaminated soil and aquifers in mining areas. The feasibility of applying Pisha sandstone (PS) and Na + -modified Pisha sandstone (Na-PS) for adsorption of heavy metals was evaluated. Na-PS exhibited maximum Cd(II) and Cu(II) removal rates of 65.9% and 99.8%, respectively, exceeding the corresponding values for PS (8.2% and 1.3%, respectively) in 1 × 10 −3  M solution. Efficient heavy metals adsorption occurred in the pH range 5.0–6.0. The adsorption of Cu(II) and Cd(II) on PS and Na-PS was characterized by kinetic models and adsorption isotherms and was well represented by pseudo-second-order kinetics ( R 2  > 0.99) and the Langmuir and Freundlich isotherm models. The values of the thermodynamic parameters indicated that the interactions were spontaneous endothermic reactions. Binary solutions adsorption isotherms indicated that the linearity of the adsorption amount and initial concentration of Cu(II) and Cd(II) was better in certain ranges and the adsorbents were selective towards Cu(II) rather than Cd(II). Therefore, PSs can be used as excellent adsorbents for Cu(II) and Cd(II) remediation from contaminated surface water.
Author Wang, Xia
Peng, Qi
Fan, Chenbin
Zhang, Xingchang
Cui, Yongxing
Zhang, Zhiqin
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Copyright Copyright © 2020 Xia Wang et al.
Copyright © 2020 Xia Wang et al. This is an open access article distributed under the Creative Commons Attribution License (the “License”), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. http://creativecommons.org/licenses/by/4.0
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Snippet Heavy metals have caused serious environmental issues, which are enriched during open-cast coal mining. It is urgent to develop sustainable remediation...
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SubjectTerms Adsorbents
Adsorption
Aqueous solutions
Aquifers
Coal mines
Coal mining
Endothermic reactions
Environmental impact
Equilibrium
Heavy metals
Isotherms
Kinetics
Linearity
Metals
Minerals
Reaction kinetics
Remediation
Sandstone
Soil contamination
Soil remediation
Studies
Surface water
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Title Removal of Cd(II) and Cu(II) from Aqueous Solution by Na+-Modified Pisha Sandstone
URI https://search.emarefa.net/detail/BIM-1181532
https://dx.doi.org/10.1155/2020/2805479
https://www.proquest.com/docview/2381579093
https://doaj.org/article/a48e8e9eb6c54e2d8bcd39d0b5f7f7cc
Volume 2020
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