Nitrogen doped carbon quantum dots mediated silver phosphate/bismuth vanadate Z-scheme photocatalyst for enhanced antibiotic degradation

[Display omitted] A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, sca...

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Published inJournal of colloid and interface science Vol. 529; pp. 11 - 22
Main Authors Zhang, Jin, Yan, Ming, Yuan, Xingzhong, Si, Mengying, Jiang, Longbo, Wu, Zhibin, Wang, Hou, Zeng, Guangming
Format Journal Article
LanguageEnglish
Published United States Elsevier Inc 01.11.2018
Subjects
Ag3PO4
bismuth
BiVO4
carbon quantum dots
electron paramagnetic resonance spectroscopy
lighting
mineralization
N-CQDs
nitrogen
oxygen
phosphates
photocatalysis
photocatalysts
photoluminescence
scanning electron microscopy
silver
Tetracycline
Visible light photocatalysis
X-ray diffraction
X-ray photoelectron spectroscopy
Visible light photocatalysis
Ag3PO4
BiVO4
N-CQDs
Tetracycline
AgPO
BiVO
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Abstract [Display omitted] A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, scanning electron microscopy, transmission electron micrograph, UV–vis diffuse reflection spectroscopy, vis photoluminescence and electron spin resonance analysis. The photocatalytic performances of as-prepared photocatalysts were used for degradation of tetracycline (TC) under visible-light illumination. Results exhibited the increased photocatalytic efficiency of BiVO4/N-CQDs/Ag3PO4-10 (Ag3PO4 with the mass ratio of BiVO4/N-CQDs/Ag3PO4 = 10%) to photodegrade TC is up to 88.9% in 30 min and 59.8% mineralization in 90 min. The degradation reaction coefficient (k) is about 6.00, 2.78 and 1.80 times higher than that of BiVO4, N-CQDs/BiVO4 and Ag3PO4/BiVO4, respectively. The excellent photocatalytic performance of the Z-scheme BiVO4/N-CQDs/Ag3PO4 was attributed to the construction of Z-scheme system, increased light harvesting capacity and improved molecular oxygen activation ability. Moreover, the photocatalytic activity of BiVO4/N-CQDs/Ag3PO4 remained 79.9% after five cycling runs, indicating the high stability and reusability of the as-prepared photocatalyst. Additionally, a possible photocatalytic mechanism of the novel Z-scheme BiVO4/N-CQDs/Ag3PO4 was proposed.
AbstractList A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, scanning electron microscopy, transmission electron micrograph, UV-vis diffuse reflection spectroscopy, vis photoluminescence and electron spin resonance analysis. The photocatalytic performances of as-prepared photocatalysts were used for degradation of tetracycline (TC) under visible-light illumination. Results exhibited the increased photocatalytic efficiency of BiVO4/N-CQDs/Ag3PO4-10 (Ag3PO4 with the mass ratio of BiVO4/N-CQDs/Ag3PO4 = 10%) to photodegrade TC is up to 88.9% in 30 min and 59.8% mineralization in 90 min. The degradation reaction coefficient (k) is about 6.00, 2.78 and 1.80 times higher than that of BiVO4, N-CQDs/BiVO4 and Ag3PO4/BiVO4, respectively. The excellent photocatalytic performance of the Z-scheme BiVO4/N-CQDs/Ag3PO4 was attributed to the construction of Z-scheme system, increased light harvesting capacity and improved molecular oxygen activation ability. Moreover, the photocatalytic activity of BiVO4/N-CQDs/Ag3PO4 remained 79.9% after five cycling runs, indicating the high stability and reusability of the as-prepared photocatalyst. Additionally, a possible photocatalytic mechanism of the novel Z-scheme BiVO4/N-CQDs/Ag3PO4 was proposed.A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, scanning electron microscopy, transmission electron micrograph, UV-vis diffuse reflection spectroscopy, vis photoluminescence and electron spin resonance analysis. The photocatalytic performances of as-prepared photocatalysts were used for degradation of tetracycline (TC) under visible-light illumination. Results exhibited the increased photocatalytic efficiency of BiVO4/N-CQDs/Ag3PO4-10 (Ag3PO4 with the mass ratio of BiVO4/N-CQDs/Ag3PO4 = 10%) to photodegrade TC is up to 88.9% in 30 min and 59.8% mineralization in 90 min. The degradation reaction coefficient (k) is about 6.00, 2.78 and 1.80 times higher than that of BiVO4, N-CQDs/BiVO4 and Ag3PO4/BiVO4, respectively. The excellent photocatalytic performance of the Z-scheme BiVO4/N-CQDs/Ag3PO4 was attributed to the construction of Z-scheme system, increased light harvesting capacity and improved molecular oxygen activation ability. Moreover, the photocatalytic activity of BiVO4/N-CQDs/Ag3PO4 remained 79.9% after five cycling runs, indicating the high stability and reusability of the as-prepared photocatalyst. Additionally, a possible photocatalytic mechanism of the novel Z-scheme BiVO4/N-CQDs/Ag3PO4 was proposed.
A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag PO /BiVO Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, scanning electron microscopy, transmission electron micrograph, UV-vis diffuse reflection spectroscopy, vis photoluminescence and electron spin resonance analysis. The photocatalytic performances of as-prepared photocatalysts were used for degradation of tetracycline (TC) under visible-light illumination. Results exhibited the increased photocatalytic efficiency of BiVO /N-CQDs/Ag PO -10 (Ag PO with the mass ratio of BiVO /N-CQDs/Ag PO  = 10%) to photodegrade TC is up to 88.9% in 30 min and 59.8% mineralization in 90 min. The degradation reaction coefficient (k) is about 6.00, 2.78 and 1.80 times higher than that of BiVO N-CQDs/BiVO and Ag PO /BiVO , respectively. The excellent photocatalytic performance of the Z-scheme BiVO /N-CQDs/Ag PO was attributed to the construction of Z-scheme system, increased light harvesting capacity and improved molecular oxygen activation ability. Moreover, the photocatalytic activity of BiVO /N-CQDs/Ag PO remained 79.9% after five cycling runs, indicating the high stability and reusability of the as-prepared photocatalyst. Additionally, a possible photocatalytic mechanism of the novel Z-scheme BiVO /N-CQDs/Ag PO was proposed.
A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag₃PO₄/BiVO₄ Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, scanning electron microscopy, transmission electron micrograph, UV–vis diffuse reflection spectroscopy, vis photoluminescence and electron spin resonance analysis. The photocatalytic performances of as-prepared photocatalysts were used for degradation of tetracycline (TC) under visible-light illumination. Results exhibited the increased photocatalytic efficiency of BiVO₄/N-CQDs/Ag₃PO₄-10 (Ag₃PO₄ with the mass ratio of BiVO₄/N-CQDs/Ag₃PO₄ = 10%) to photodegrade TC is up to 88.9% in 30 min and 59.8% mineralization in 90 min. The degradation reaction coefficient (k) is about 6.00, 2.78 and 1.80 times higher than that of BiVO₄, N-CQDs/BiVO₄ and Ag₃PO₄/BiVO₄, respectively. The excellent photocatalytic performance of the Z-scheme BiVO₄/N-CQDs/Ag₃PO₄ was attributed to the construction of Z-scheme system, increased light harvesting capacity and improved molecular oxygen activation ability. Moreover, the photocatalytic activity of BiVO₄/N-CQDs/Ag₃PO₄ remained 79.9% after five cycling runs, indicating the high stability and reusability of the as-prepared photocatalyst. Additionally, a possible photocatalytic mechanism of the novel Z-scheme BiVO₄/N-CQDs/Ag₃PO₄ was proposed.
[Display omitted] A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method. The as-prepared photocatalysts were comprehensive characterized by X-ray diffraction, X-ray photo-electron spectroscopy, scanning electron microscopy, transmission electron micrograph, UV–vis diffuse reflection spectroscopy, vis photoluminescence and electron spin resonance analysis. The photocatalytic performances of as-prepared photocatalysts were used for degradation of tetracycline (TC) under visible-light illumination. Results exhibited the increased photocatalytic efficiency of BiVO4/N-CQDs/Ag3PO4-10 (Ag3PO4 with the mass ratio of BiVO4/N-CQDs/Ag3PO4 = 10%) to photodegrade TC is up to 88.9% in 30 min and 59.8% mineralization in 90 min. The degradation reaction coefficient (k) is about 6.00, 2.78 and 1.80 times higher than that of BiVO4, N-CQDs/BiVO4 and Ag3PO4/BiVO4, respectively. The excellent photocatalytic performance of the Z-scheme BiVO4/N-CQDs/Ag3PO4 was attributed to the construction of Z-scheme system, increased light harvesting capacity and improved molecular oxygen activation ability. Moreover, the photocatalytic activity of BiVO4/N-CQDs/Ag3PO4 remained 79.9% after five cycling runs, indicating the high stability and reusability of the as-prepared photocatalyst. Additionally, a possible photocatalytic mechanism of the novel Z-scheme BiVO4/N-CQDs/Ag3PO4 was proposed.
Author Zhang, Jin
Zeng, Guangming
Yuan, Xingzhong
Wang, Hou
Si, Mengying
Wu, Zhibin
Yan, Ming
Jiang, Longbo
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  organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China
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  surname: Yan
  fullname: Yan, Ming
  email: ym8188@hnu.edu.cn
  organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China
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  givenname: Xingzhong
  surname: Yuan
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  organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China
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  fullname: Si, Mengying
  organization: School of Metallurgy and Environment, Central South University, Changsha 410083, PR China
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  orcidid: 0000-0002-4230-7647
  surname: Zeng
  fullname: Zeng, Guangming
  organization: College of Environmental Science and Engineering, Hunan University, Changsha 410082, PR China
BackLink https://www.ncbi.nlm.nih.gov/pubmed/29879678$$D View this record in MEDLINE/PubMed
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Keywords Visible light photocatalysis
Ag3PO4
BiVO4
N-CQDs
Tetracycline
AgPO
BiVO
Language English
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PublicationDate 2018-11-01
PublicationDateYYYYMMDD 2018-11-01
PublicationDate_xml – month: 11
  year: 2018
  text: 2018-11-01
  day: 01
PublicationDecade 2010
PublicationPlace United States
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PublicationTitle Journal of colloid and interface science
PublicationTitleAlternate J Colloid Interface Sci
PublicationYear 2018
Publisher Elsevier Inc
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Snippet [Display omitted] A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a...
A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag PO /BiVO Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method....
A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag3PO4/BiVO4 Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method....
A novel nitrogen doped carbon quantum dots (N-CQDs) mediated Ag₃PO₄/BiVO₄ Z-scheme photocatalyst was synthesized through a solvothermal-precipitation method....
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StartPage 11
SubjectTerms Ag3PO4
bismuth
BiVO4
carbon quantum dots
electron paramagnetic resonance spectroscopy
lighting
mineralization
N-CQDs
nitrogen
oxygen
phosphates
photocatalysis
photocatalysts
photoluminescence
scanning electron microscopy
silver
Tetracycline
Visible light photocatalysis
X-ray diffraction
X-ray photoelectron spectroscopy
Title Nitrogen doped carbon quantum dots mediated silver phosphate/bismuth vanadate Z-scheme photocatalyst for enhanced antibiotic degradation
URI https://dx.doi.org/10.1016/j.jcis.2018.05.109
https://www.ncbi.nlm.nih.gov/pubmed/29879678
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https://www.proquest.com/docview/2116925575
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