NiS and MoS2 nanosheet co-modified graphitic C3N4 ternary heterostructure for high efficient visible light photodegradation of antibiotic
[Display omitted] The development of efficient solar driven catalytic system for the degradation of antibiotics has become increasingly important in environmental protection and remediation. Non-noble-metal NiS and MoS2 nanosheet co-modified graphitic C3N4 ternary heterostructure has been synthesize...
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| Published in | Journal of hazardous materials Vol. 341; pp. 10 - 19 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
05.01.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
The development of efficient solar driven catalytic system for the degradation of antibiotics has become increasingly important in environmental protection and remediation. Non-noble-metal NiS and MoS2 nanosheet co-modified graphitic C3N4 ternary heterostructure has been synthesized via a facile combination of hydrothermal and ultrasound method, and the ternary heterostructure has been utilized for photocatalytic degradation of antibiotic agents. The antibiotics of ciprofloxacin (CIP) and tetracycline hydrochloride (TC) were photodegraded by the hybrid under the visible light. The optimal photodegradation rate of the ternary heterostructure reaches about 96% after 2h irradiation, which is 2.1 times higher than that of pure g-C3N4 for TC degradation. The photocatalytic degradation rates of the ternary heterostructure for both CIP and TC obey the pseudo-first-order kinetic model. The enhanced visible light adsorption and charge separation efficiency contribute to the photocatalytic performance of the ternary heterostructure. This work provides new insights and pathways by which efficient degradation of antibiotics can be achieved and will stimulate further studies in this important field. |
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| AbstractList | [Display omitted]
The development of efficient solar driven catalytic system for the degradation of antibiotics has become increasingly important in environmental protection and remediation. Non-noble-metal NiS and MoS2 nanosheet co-modified graphitic C3N4 ternary heterostructure has been synthesized via a facile combination of hydrothermal and ultrasound method, and the ternary heterostructure has been utilized for photocatalytic degradation of antibiotic agents. The antibiotics of ciprofloxacin (CIP) and tetracycline hydrochloride (TC) were photodegraded by the hybrid under the visible light. The optimal photodegradation rate of the ternary heterostructure reaches about 96% after 2h irradiation, which is 2.1 times higher than that of pure g-C3N4 for TC degradation. The photocatalytic degradation rates of the ternary heterostructure for both CIP and TC obey the pseudo-first-order kinetic model. The enhanced visible light adsorption and charge separation efficiency contribute to the photocatalytic performance of the ternary heterostructure. This work provides new insights and pathways by which efficient degradation of antibiotics can be achieved and will stimulate further studies in this important field. The development of efficient solar driven catalytic system for the degradation of antibiotics has become increasingly important in environmental protection and remediation. Non-noble-metal NiS and MoS2 nanosheet co-modified graphitic C3N4 ternary heterostructure has been synthesized via a facile combination of hydrothermal and ultrasound method, and the ternary heterostructure has been utilized for photocatalytic degradation of antibiotic agents. The antibiotics of ciprofloxacin (CIP) and tetracycline hydrochloride (TC) were photodegraded by the hybrid under the visible light. The optimal photodegradation rate of the ternary heterostructure reaches about 96% after 2h irradiation, which is 2.1 times higher than that of pure g-C3N4 for TC degradation. The photocatalytic degradation rates of the ternary heterostructure for both CIP and TC obey the pseudo-first-order kinetic model. The enhanced visible light adsorption and charge separation efficiency contribute to the photocatalytic performance of the ternary heterostructure. This work provides new insights and pathways by which efficient degradation of antibiotics can be achieved and will stimulate further studies in this important field. |
| Author | Xu, Guangqing Lu, Xuejun Zheng, Zhixiang Wang, Yu Lv, Jun Zhang, Xinyi Wang, Dongmei Wu, Yucheng |
| Author_xml | – sequence: 1 givenname: Xuejun surname: Lu fullname: Lu, Xuejun organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China – sequence: 2 givenname: Yu surname: Wang fullname: Wang, Yu organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China – sequence: 3 givenname: Xinyi surname: Zhang fullname: Zhang, Xinyi organization: School of Chemistry, Monash University, Clayton, VIC3800, Australia – sequence: 4 givenname: Guangqing surname: Xu fullname: Xu, Guangqing organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China – sequence: 5 givenname: Dongmei surname: Wang fullname: Wang, Dongmei organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China – sequence: 6 givenname: Jun surname: Lv fullname: Lv, Jun email: lvjun117@126.com organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China – sequence: 7 givenname: Zhixiang surname: Zheng fullname: Zheng, Zhixiang organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China – sequence: 8 givenname: Yucheng surname: Wu fullname: Wu, Yucheng email: ycwu@hfut.edu.cn organization: Laboratory of Functional Nanomaterials and Devices, School of Materials Sciences and Engineering, Hefei University of Technology, Hefei 230009, China |
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