Remarkable Turn-On and Color-Tuned Piezochromic Luminescence: Mechanically Switching Intramolecular Charge Transfer in Molecular Crystals
The molecular crystals of acridonyl‐tetraphenylethene (AD‐TPE) exhibit an intriguing turn‐on and color‐tuned luminescence in response to mechanical grinding and hydrostatic compression. On the basis of in‐depth experimental and computational studies, it is hypothesized that the origin of the piezoch...
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| Published in | Advanced functional materials Vol. 25; no. 26; pp. 4005 - 4010 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Blackwell Publishing Ltd
01.07.2015
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The molecular crystals of acridonyl‐tetraphenylethene (AD‐TPE) exhibit an intriguing turn‐on and color‐tuned luminescence in response to mechanical grinding and hydrostatic compression. On the basis of in‐depth experimental and computational studies, it is hypothesized that the origin of the piezochromic behavior from the D‐phase to the B‐phase is the change of the intramolecular geometrical conformation, especially for the torsion angle between the TPE and AD moiety. The different molecular conformation in the two distinctive solid phases causes the substantial switching of the intramolecular charge transfer (ICT) process, which can be directly correlated with the subsequent fluorescence from locally excited (LE) state and ICT state in both phases. The AD‐TPE molecular system presents a very rare example of high‐contrast reversible fluorescence tuning driven by a switching of the excited state in the solid state under the mechanical stimuli, and thus provides a novel mechanism of the piezochromic behavior.
Tuning the solid state luminescence of organic materials under mechanical stimuli is an attractive subject for both the fundamental research and practical application in the optical recording and sensing. Herein, a structurally well‐defined molecule, acridonyl‐tetraphenylethene is reported, whose molecular crystals exhibit an intriguing turn‐on and color‐tuned luminescence with high contrast in response to the mechanical stimuli such as grinding and hydrostatic pressure. |
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| AbstractList | The molecular crystals of acridonyl‐tetraphenylethene (AD‐TPE) exhibit an intriguing turn‐on and color‐tuned luminescence in response to mechanical grinding and hydrostatic compression. On the basis of in‐depth experimental and computational studies, it is hypothesized that the origin of the piezochromic behavior from the D‐phase to the B‐phase is the change of the intramolecular geometrical conformation, especially for the torsion angle between the TPE and AD moiety. The different molecular conformation in the two distinctive solid phases causes the substantial switching of the intramolecular charge transfer (ICT) process, which can be directly correlated with the subsequent fluorescence from locally excited (LE) state and ICT state in both phases. The AD‐TPE molecular system presents a very rare example of high‐contrast reversible fluorescence tuning driven by a switching of the excited state in the solid state under the mechanical stimuli, and thus provides a novel mechanism of the piezochromic behavior.
Tuning the solid state luminescence of organic materials under mechanical stimuli is an attractive subject for both the fundamental research and practical application in the optical recording and sensing. Herein, a structurally well‐defined molecule, acridonyl‐tetraphenylethene is reported, whose molecular crystals exhibit an intriguing turn‐on and color‐tuned luminescence with high contrast in response to the mechanical stimuli such as grinding and hydrostatic pressure. The molecular crystals of acridonyl‐tetraphenylethene (AD‐TPE) exhibit an intriguing turn‐on and color‐tuned luminescence in response to mechanical grinding and hydrostatic compression. On the basis of in‐depth experimental and computational studies, it is hypothesized that the origin of the piezochromic behavior from the D‐phase to the B‐phase is the change of the intramolecular geometrical conformation, especially for the torsion angle between the TPE and AD moiety. The different molecular conformation in the two distinctive solid phases causes the substantial switching of the intramolecular charge transfer (ICT) process, which can be directly correlated with the subsequent fluorescence from locally excited (LE) state and ICT state in both phases. The AD‐TPE molecular system presents a very rare example of high‐contrast reversible fluorescence tuning driven by a switching of the excited state in the solid state under the mechanical stimuli, and thus provides a novel mechanism of the piezochromic behavior. The molecular crystals of acridonyl-tetraphenylethene (AD-TPE) exhibit an intriguing turn-on and color-tuned luminescence in response to mechanical grinding and hydrostatic compression. On the basis of in-depth experimental and computational studies, it is hypothesized that the origin of the piezochromic behavior from the D-phase to the B-phase is the change of the intramolecular geometrical conformation, especially for the torsion angle between the TPE and AD moiety. The different molecular conformation in the two distinctive solid phases causes the substantial switching of the intra-molecular charge transfer (ICT) process, which can be directly correlated with the subsequent fluorescence from locally excited (LE) state and ICT state in both phases. The AD-TPE molecular system presents a very rare example of high-contrast reversible fluorescence tuning driven by a switching of the excited state in the solid state under the mechanical stimuli, and thus provides a novel mechanism of the piezochromic behavior. Tuning the solid state luminescence of organic materials under mechanical stimuli is an attractive subject for both the fundamental research and practical application in the optical recording and sensing. Herein, a structurally well-defined molecule, acridonyl-tetraphenylethene is reported, whose molecular crystals exhibit an intriguing turn-on and color-tuned luminescence with high contrast in response to the mechanical stimuli such as grinding and hydrostatic pressure. |
| Author | Xu, Bin Tan, Xiao Zou, Bo Tian, Wenjing Zhang, Jibo Qian, Jingyu Qi, Qingkai Wang, Lijuan |
| Author_xml | – sequence: 1 givenname: Qingkai surname: Qi fullname: Qi, Qingkai organization: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry Jilin University, 130012, Changchun, P. R. China – sequence: 2 givenname: Jingyu surname: Qian fullname: Qian, Jingyu organization: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry Jilin University, 130012, Changchun, P. R. China – sequence: 3 givenname: Xiao surname: Tan fullname: Tan, Xiao organization: State Key Laboratory of Superhard Materials, Jilin University, 130012, Changchun, P. R. China – sequence: 4 givenname: Jibo surname: Zhang fullname: Zhang, Jibo organization: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry Jilin University, 130012, Changchun, P. R. China – sequence: 5 givenname: Lijuan surname: Wang fullname: Wang, Lijuan organization: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry Jilin University, 130012, Changchun, P. R. China – sequence: 6 givenname: Bin surname: Xu fullname: Xu, Bin email: xubin@jlu.edu.cn organization: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry Jilin University, 130012, Changchun, P. R. China – sequence: 7 givenname: Bo surname: Zou fullname: Zou, Bo organization: State Key Laboratory of Superhard Materials, Jilin University, 130012, Changchun, P. R. China – sequence: 8 givenname: Wenjing surname: Tian fullname: Tian, Wenjing email: xubin@jlu.edu.cn organization: State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry Jilin University, 130012, Changchun, P. R. China |
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| Snippet | The molecular crystals of acridonyl‐tetraphenylethene (AD‐TPE) exhibit an intriguing turn‐on and color‐tuned luminescence in response to mechanical grinding... The molecular crystals of acridonyl-tetraphenylethene (AD-TPE) exhibit an intriguing turn-on and color-tuned luminescence in response to mechanical grinding... |
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| SubjectTerms | Charge transfer Crystals Excitation Fluorescence high contrast ICT switch Luminescence mechanical stimuli molecular crystals piezochromic luminescence Stimuli Switching Tuning |
| Title | Remarkable Turn-On and Color-Tuned Piezochromic Luminescence: Mechanically Switching Intramolecular Charge Transfer in Molecular Crystals |
| URI | https://api.istex.fr/ark:/67375/WNG-80TFV6CW-8/fulltext.pdf https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadfm.201501224 https://www.proquest.com/docview/1709760746 |
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