Photocatalytic hydrogen generation on low-bandgap black zirconia (ZrO) produced by high-pressure torsion

Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO 2 ) is a semiconductor oxide, it is not generally considered as a photocatalyst owing to its poor light absorbance and wide bandgap (over 5 eV). In...

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Published inJournal of materials chemistry. A, Materials for energy and sustainability Vol. 8; no. 7; pp. 3643 - 365
Main Authors Wang, Qing, Edalati, Kaveh, Koganemaru, Yuta, Nakamura, Shohei, Watanabe, Motonori, Ishihara, Tatsumi, Horita, Zenji
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 01.01.2020
Subjects
Catalytic activity
Clean energy
Clean technology
Conduction
Conduction bands
Crystal defects
Electromagnetic absorption
Electronics industry
Energy gap
Energy sources
Hydrogen
Hydrogen evolution
Hydrogen production
Lattice vacancies
Oxygen
Phase transitions
Photocatalysis
Photocatalysts
Pressure
Solar energy
Water splitting
Zirconia
Zirconium dioxide
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Abstract Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO 2 ) is a semiconductor oxide, it is not generally considered as a photocatalyst owing to its poor light absorbance and wide bandgap (over 5 eV). In this study, black ZrO 2 with a large concentration of lattice defects such as oxygen vacancies, dislocations and nanograin boundaries is stabilized by high-pressure torsion (HPT) straining. The black ZrO 2 , which experiences monoclinic-tetragonal phase transformations during the HPT process, shows large light absorption, a small bandgap, reduced conduction band energy and high photocatalytic activity for hydrogen evolution due the presence of oxygen vacancies. These results confirm that the introduction of strain-induced oxygen vacancies is a potential method to produce low-bandgap photocatalysts. Photocatalytic hydrogen generation on low-bandgap black ZrO 2 produced by high-pressure torsion.
AbstractList Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO 2 ) is a semiconductor oxide, it is not generally considered as a photocatalyst owing to its poor light absorbance and wide bandgap (over 5 eV). In this study, black ZrO 2 with a large concentration of lattice defects such as oxygen vacancies, dislocations and nanograin boundaries is stabilized by high-pressure torsion (HPT) straining. The black ZrO 2 , which experiences monoclinic–tetragonal phase transformations during the HPT process, shows large light absorption, a small bandgap, reduced conduction band energy and high photocatalytic activity for hydrogen evolution due the presence of oxygen vacancies. These results confirm that the introduction of strain-induced oxygen vacancies is a potential method to produce low-bandgap photocatalysts.
Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO 2 ) is a semiconductor oxide, it is not generally considered as a photocatalyst owing to its poor light absorbance and wide bandgap (over 5 eV). In this study, black ZrO 2 with a large concentration of lattice defects such as oxygen vacancies, dislocations and nanograin boundaries is stabilized by high-pressure torsion (HPT) straining. The black ZrO 2 , which experiences monoclinic-tetragonal phase transformations during the HPT process, shows large light absorption, a small bandgap, reduced conduction band energy and high photocatalytic activity for hydrogen evolution due the presence of oxygen vacancies. These results confirm that the introduction of strain-induced oxygen vacancies is a potential method to produce low-bandgap photocatalysts. Photocatalytic hydrogen generation on low-bandgap black ZrO 2 produced by high-pressure torsion.
Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO2) is a semiconductor oxide, it is not generally considered as a photocatalyst owing to its poor light absorbance and wide bandgap (over 5 eV). In this study, black ZrO2 with a large concentration of lattice defects such as oxygen vacancies, dislocations and nanograin boundaries is stabilized by high-pressure torsion (HPT) straining. The black ZrO2, which experiences monoclinic–tetragonal phase transformations during the HPT process, shows large light absorption, a small bandgap, reduced conduction band energy and high photocatalytic activity for hydrogen evolution due the presence of oxygen vacancies. These results confirm that the introduction of strain-induced oxygen vacancies is a potential method to produce low-bandgap photocatalysts.
Author Nakamura, Shohei
Ishihara, Tatsumi
Wang, Qing
Edalati, Kaveh
Koganemaru, Yuta
Watanabe, Motonori
Horita, Zenji
AuthorAffiliation 2
Faculty of Engineering
Department of Applied Chemistry
CNER
Kyushu Institute of Technology
WPI, International Institute for Carbon-Neutral Energy Research (WPI-I
School of Engineering
Kyushu University
AuthorAffiliation_xml – name: Faculty of Engineering
– name: CNER
– name: Kyushu University
– name: WPI, International Institute for Carbon-Neutral Energy Research (WPI-I
– name: Kyushu Institute of Technology
– name: Department of Applied Chemistry
– name: School of Engineering
– name: 2
Author_xml – sequence: 1
  givenname: Qing
  surname: Wang
  fullname: Wang, Qing
– sequence: 2
  givenname: Kaveh
  surname: Edalati
  fullname: Edalati, Kaveh
– sequence: 3
  givenname: Yuta
  surname: Koganemaru
  fullname: Koganemaru, Yuta
– sequence: 4
  givenname: Shohei
  surname: Nakamura
  fullname: Nakamura, Shohei
– sequence: 5
  givenname: Motonori
  surname: Watanabe
  fullname: Watanabe, Motonori
– sequence: 6
  givenname: Tatsumi
  surname: Ishihara
  fullname: Ishihara, Tatsumi
– sequence: 7
  givenname: Zenji
  surname: Horita
  fullname: Horita, Zenji
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Snippet Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO 2 ) is...
Photocatalysis on semiconductors using solar energy sources provides a clean technology to produce hydrogen from water splitting. Although zirconia (ZrO2) is a...
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SubjectTerms Catalytic activity
Clean energy
Clean technology
Conduction
Conduction bands
Crystal defects
Electromagnetic absorption
Electronics industry
Energy gap
Energy sources
Hydrogen
Hydrogen evolution
Hydrogen production
Lattice vacancies
Oxygen
Phase transitions
Photocatalysis
Photocatalysts
Pressure
Solar energy
Water splitting
Zirconia
Zirconium dioxide
Title Photocatalytic hydrogen generation on low-bandgap black zirconia (ZrO) produced by high-pressure torsion
URI https://www.proquest.com/docview/2356612911/abstract/
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