High Mechanical Performance Composite Conductor: Multi-Walled Carbon Nanotube Sheet/Bismaleimide Nanocomposites
Multi‐walled carbon nanotube (MWNT)‐sheet‐reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (∼60 wt%) of aligned MWNTs are successfully fabricated. Applying simple mechanical stretching and prepregging (pre‐resin impregnation) processes on initially randomly dispersed, comm...
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| Published in | Advanced functional materials Vol. 19; no. 20; pp. 3219 - 3225 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
23.10.2009
WILEY‐VCH Verlag |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Multi‐walled carbon nanotube (MWNT)‐sheet‐reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (∼60 wt%) of aligned MWNTs are successfully fabricated. Applying simple mechanical stretching and prepregging (pre‐resin impregnation) processes on initially randomly dispersed, commercially available sheets of millimeter‐long MWNTs leads to substantial alignment enhancement, good dispersion, and high packing density of nanotubes in the resultant nanocomposites. The tensile strength and Young's modulus of the nanocomposites reaches 2 088 MPa and 169 GPa, respectively, which are very high experimental results and comparable to the state‐of‐the‐art unidirectional IM7 carbon‐fiber‐reinforced composites for high‐performance structural applications. The nanocomposites demonstrate unprecedentedly high electrical conductivity of 5 500 S cm−1 along the alignment direction. Such unique integration of high mechanical properties and electrical conductance opens the door for developing polymeric composite conductors and eventually structural composites with multifunctionalities. New fracture morphology and failure modes due to self‐assembly and spreading of MWNT bundles are also observed.
High concentration (∼60wt%) multi‐walled carbon nanotube sheet/bismaleimide composites are fabricated using simple mechanical stretching and prepregging methods, resulting in unprecedentedly high electrical conductivity (5 500 S cm−1) and mechanical properties (strength of 2 088 MPa and modulus of 169 GPa) comparable to those of unidirectional carbon fiber‐reinforced composites for high‐performance structural and multifunctional applications. |
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| AbstractList | Multi-walled carbon nanotube (MWNT)-sheet-reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (60 wt%) of aligned MWNTs are successfully fabricated. Applying simple mechanical stretching and prepregging (pre-resin impregnation) processes on initially randomly dispersed, commercially available sheets of millimeter-long MWNTs leads to substantial alignment enhancement, good dispersion, and high packing density of nanotubes in the resultant nanocomposites. The tensile strength and Young's modulus of the nanocomposites reaches 2 088 MPa and 169 GPa, respectively, which are very high experimental results and comparable to the state-of-the-art unidirectional IM7 carbon-fiber-reinforced composites for high-performance structural applications. The nanocomposites demonstrate unprecedentedly high electrical conductivity of 5 500 S cm-1 along the alignment direction. Such unique integration of high mechanical properties and electrical conductance opens the door for developing polymeric composite conductors and eventually structural composites with multifunctionalities. New fracture morphology and failure modes due to self-assembly and spreading of MWNT bundles are also observed. Multi‐walled carbon nanotube (MWNT)‐sheet‐reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (∼60 wt%) of aligned MWNTs are successfully fabricated. Applying simple mechanical stretching and prepregging (pre‐resin impregnation) processes on initially randomly dispersed, commercially available sheets of millimeter‐long MWNTs leads to substantial alignment enhancement, good dispersion, and high packing density of nanotubes in the resultant nanocomposites. The tensile strength and Young's modulus of the nanocomposites reaches 2 088 MPa and 169 GPa, respectively, which are very high experimental results and comparable to the state‐of‐the‐art unidirectional IM7 carbon‐fiber‐reinforced composites for high‐performance structural applications. The nanocomposites demonstrate unprecedentedly high electrical conductivity of 5 500 S cm−1 along the alignment direction. Such unique integration of high mechanical properties and electrical conductance opens the door for developing polymeric composite conductors and eventually structural composites with multifunctionalities. New fracture morphology and failure modes due to self‐assembly and spreading of MWNT bundles are also observed. High concentration (∼60wt%) multi‐walled carbon nanotube sheet/bismaleimide composites are fabricated using simple mechanical stretching and prepregging methods, resulting in unprecedentedly high electrical conductivity (5 500 S cm−1) and mechanical properties (strength of 2 088 MPa and modulus of 169 GPa) comparable to those of unidirectional carbon fiber‐reinforced composites for high‐performance structural and multifunctional applications. Multi‐walled carbon nanotube (MWNT)‐sheet‐reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (∼60 wt%) of aligned MWNTs are successfully fabricated. Applying simple mechanical stretching and prepregging (pre‐resin impregnation) processes on initially randomly dispersed, commercially available sheets of millimeter‐long MWNTs leads to substantial alignment enhancement, good dispersion, and high packing density of nanotubes in the resultant nanocomposites. The tensile strength and Young's modulus of the nanocomposites reaches 2 088 MPa and 169 GPa, respectively, which are very high experimental results and comparable to the state‐of‐the‐art unidirectional IM7 carbon‐fiber‐reinforced composites for high‐performance structural applications. The nanocomposites demonstrate unprecedentedly high electrical conductivity of 5 500 S cm −1 along the alignment direction. Such unique integration of high mechanical properties and electrical conductance opens the door for developing polymeric composite conductors and eventually structural composites with multifunctionalities. New fracture morphology and failure modes due to self‐assembly and spreading of MWNT bundles are also observed. |
| Author | Cheng, Qunfeng Liang, Zhiyong Bao, Jianwen Wang, Ben Park, JinGyu Zhang, Chuck |
| Author_xml | – sequence: 1 givenname: Qunfeng surname: Cheng fullname: Cheng, Qunfeng organization: High-Performance Materials Institute (HPMI) Florida State University Tallahassee, FL 32310 (USA) – sequence: 2 givenname: Jianwen surname: Bao fullname: Bao, Jianwen organization: High-Performance Materials Institute (HPMI) Florida State University Tallahassee, FL 32310 (USA) – sequence: 3 givenname: JinGyu surname: Park fullname: Park, JinGyu organization: High-Performance Materials Institute (HPMI) Florida State University Tallahassee, FL 32310 (USA) – sequence: 4 givenname: Zhiyong surname: Liang fullname: Liang, Zhiyong email: liang@eng.fsu.edu organization: High-Performance Materials Institute (HPMI) Florida State University Tallahassee, FL 32310 (USA) – sequence: 5 givenname: Chuck surname: Zhang fullname: Zhang, Chuck organization: High-Performance Materials Institute (HPMI) Florida State University Tallahassee, FL 32310 (USA) – sequence: 6 givenname: Ben surname: Wang fullname: Wang, Ben organization: High-Performance Materials Institute (HPMI) Florida State University Tallahassee, FL 32310 (USA) |
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| Snippet | Multi‐walled carbon nanotube (MWNT)‐sheet‐reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (∼60 wt%) of aligned MWNTs are... Multi-walled carbon nanotube (MWNT)-sheet-reinforced bismaleimide (BMI) resin nanocomposites with high concentrations (60 wt%) of aligned MWNTs are... |
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| SubjectTerms | Bismaleimide resin Carbon nanotubes Composites Electrical conductivity Mechanical properties Nanotube alignment |
| Title | High Mechanical Performance Composite Conductor: Multi-Walled Carbon Nanotube Sheet/Bismaleimide Nanocomposites |
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