Radiation generated by the ultrafast migration of a positive charge following the ionization of a molecular system

Electronic many-body effects alone can be the driving force for an ultrafast migration of a positive charge created upon ionization of molecular systems. Here we show that this purely electronic phenomenon generates a characteristic IR radiation. The situation when the initial ionic wave packet is p...

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Published inPhysical review letters Vol. 106; no. 5; p. 053001
Main Authors Kuleff, Alexander I, Cederbaum, Lorenz S
Format Journal Article
LanguageEnglish
Published United States 31.01.2011
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Abstract Electronic many-body effects alone can be the driving force for an ultrafast migration of a positive charge created upon ionization of molecular systems. Here we show that this purely electronic phenomenon generates a characteristic IR radiation. The situation when the initial ionic wave packet is produced by a sudden removal of an electron is also studied. It is shown that in this case a much stronger UV emission is generated. This emission appears as an ultrafast response of the remaining electrons to the perturbation caused by the sudden ionization and as such is a universal phenomenon to be expected in every multielectron system.
AbstractList Electronic many-body effects alone can be the driving force for an ultrafast migration of a positive charge created upon ionization of molecular systems. Here we show that this purely electronic phenomenon generates a characteristic IR radiation. The situation when the initial ionic wave packet is produced by a sudden removal of an electron is also studied. It is shown that in this case a much stronger UV emission is generated. This emission appears as an ultrafast response of the remaining electrons to the perturbation caused by the sudden ionization and as such is a universal phenomenon to be expected in every multielectron system.
Author Kuleff, Alexander I
Cederbaum, Lorenz S
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  givenname: Lorenz S
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Snippet Electronic many-body effects alone can be the driving force for an ultrafast migration of a positive charge created upon ionization of molecular systems. Here...
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Title Radiation generated by the ultrafast migration of a positive charge following the ionization of a molecular system
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