Inkjet printing of single-walled carbon nanotube/RuO2 nanowire supercapacitors on cloth fabrics and flexible substrates

Single-walled carbon nanotube (SWNT) thin film electrodes have been printed on flexible substrates and cloth fabrics by using SWNT inks and an off-the-shelf inkjet printer, with features of controlled pattern geometry (0.4–6 cm 2 ), location, controllable thickness (20–200 nm), and tunable electrica...

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Published in	Nano research Vol. 3; no. 8; pp. 594 - 603
Main Authors	Chen, Pochiang, Chen, Haitian, Qiu, Jing, Zhou, Chongwu
Format	Journal Article
Language	English
Published	Heidelberg Tsinghua Press 01.08.2010 Tsinghua University Press
Subjects	Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Carbon Chemical vapor deposition Chemistry and Materials Science Condensed Matter Physics Electrodes Electrolytes Energy storage Fabrics Geometry Ink jet printers Materials Science Nanotechnology Nanowires Polymers Research Article Ruthenium Thin films Los Angeles California United States > US California Nanowires carbon nanotubes printed and wearable energy devices supercapacitors
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Abstract	Single-walled carbon nanotube (SWNT) thin film electrodes have been printed on flexible substrates and cloth fabrics by using SWNT inks and an off-the-shelf inkjet printer, with features of controlled pattern geometry (0.4–6 cm 2 ), location, controllable thickness (20–200 nm), and tunable electrical conductivity. The as-printed SWNT films were then sandwiched together with a piece of printable polymer electrolyte to form flexible and wearable supercapacitors, which displayed good capacitive behavior even after 1,000 charge/discharge cycles. Furthermore, a simple and efficient route to produce ruthenium oxide (RuO 2 ) nanowire/SWNT hybrid films has been developed, and it was found that the knee frequency of the hybrid thin film electrodes can reach 1,500 Hz, which is much higher than the knee frequency of the bare SWNT electrodes (˜158 Hz). In addition, with the integration of RuO 2 nanowires, the performance of the printed SWNT supercapacitor was significantly improved in terms of its specific capacitance of 138 F/g, power density of 96 kW/kg, and energy density of 18.8 Wh/kg. The results indicate the potential of printable energy storage devices and their significant promise for application in wearable energy storage devices.
AbstractList	Single-walled carbon nanotube (SWNT) thin film electrodes have been printed on flexible substrates and cloth fabrics by using SWNT inks and an off-the-shelf inkjet printer, with features of controlled pattern geometry (0.4–6 cm 2 ), location, controllable thickness (20–200 nm), and tunable electrical conductivity. The as-printed SWNT films were then sandwiched together with a piece of printable polymer electrolyte to form flexible and wearable supercapacitors, which displayed good capacitive behavior even after 1,000 charge/discharge cycles. Furthermore, a simple and efficient route to produce ruthenium oxide (RuO 2 ) nanowire/SWNT hybrid films has been developed, and it was found that the knee frequency of the hybrid thin film electrodes can reach 1,500 Hz, which is much higher than the knee frequency of the bare SWNT electrodes (˜158 Hz). In addition, with the integration of RuO 2 nanowires, the performance of the printed SWNT supercapacitor was significantly improved in terms of its specific capacitance of 138 F/g, power density of 96 kW/kg, and energy density of 18.8 Wh/kg. The results indicate the potential of printable energy storage devices and their significant promise for application in wearable energy storage devices. Single-walled carbon nanotube (SWNT) thin film electrodes have been printed on flexible substrates and cloth fabrics by using SWNT inks and an off-the-shelf inkjet printer, with features of controlled pattern geometry (0.4-6 cm^sup 2^), location, controllable thickness (20-200 nm), and tunable electrical conductivity. The as-printed SWNT films were then sandwiched together with a piece of printable polymer electrolyte to form flexible and wearable supercapacitors, which displayed good capacitive behavior even after 1,000 charge/discharge cycles. Furthermore, a simple and efficient route to produce ruthenium oxide (RuO2) nanowire/SWNT hybrid films has been developed, and it was found that the knee frequency of the hybrid thin film electrodes can reach 1,500 Hz, which is much higher than the knee frequency of the bare SWNT electrodes ( 158 Hz). In addition, with the integration of RuO2 nanowires, the performance of the printed SWNT supercapacitor was significantly improved in terms of its specific capacitance of 138 F/g, power density of 96 kW/kg, and energy density of 18.8 Wh/kg. The results indicate the potential of printable energy storage devices and their significant promise for application in wearable energy storage devices. [PUBLICATION ABSTRACT]
Author	Chen, Pochiang Chen, Haitian Qiu, Jing Zhou, Chongwu
Author_xml	– sequence: 1 givenname: Pochiang surname: Chen fullname: Chen, Pochiang organization: Chemical Engineering Department and Materials Science, University of Southern California – sequence: 2 givenname: Haitian surname: Chen fullname: Chen, Haitian organization: Department of Electrical Engineering, University of Southern California – sequence: 3 givenname: Jing surname: Qiu fullname: Qiu, Jing organization: Chemical Engineering Department and Materials Science, University of Southern California – sequence: 4 givenname: Chongwu surname: Zhou fullname: Zhou, Chongwu email: chongwuz@usc.edu organization: Chemical Engineering Department and Materials Science, University of Southern California, Department of Electrical Engineering, University of Southern California
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Snippet	Single-walled carbon nanotube (SWNT) thin film electrodes have been printed on flexible substrates and cloth fabrics by using SWNT inks and an off-the-shelf...
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SubjectTerms	Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Carbon Chemical vapor deposition Chemistry and Materials Science Condensed Matter Physics Electrodes Electrolytes Energy storage Fabrics Geometry Ink jet printers Materials Science Nanotechnology Nanowires Polymers Research Article Ruthenium Thin films
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Title	Inkjet printing of single-walled carbon nanotube/RuO2 nanowire supercapacitors on cloth fabrics and flexible substrates
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