Enhancing the CH4 yield of anaerobic digestion via endogenous CO2 fixation by exogenous H2
•H2 can be generated from anaerobic iron corrosion in anaerobic digestion (AD).•The generated H2 can be utilized for converting CO2 to CH4.•With CO2 fixation, enhancement up to 61% in the CH4 yield is achieved.•The added iron can also achieve phosphorus removal from the AD supernatant. A large amoun...
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| Published in | Chemosphere (Oxford) Vol. 140; pp. 34 - 39 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.12.2015
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| Abstract | •H2 can be generated from anaerobic iron corrosion in anaerobic digestion (AD).•The generated H2 can be utilized for converting CO2 to CH4.•With CO2 fixation, enhancement up to 61% in the CH4 yield is achieved.•The added iron can also achieve phosphorus removal from the AD supernatant.
A large amount (25–60%) of degraded organics is converted directly to CO2 during anaerobic digestion (AD) process, which substantially lowers the energy (methane, CH4) yield. In this study, endogenous CO2 fixation by H2 from in-situ iron corrosion was explored to enhancing the CH4 yield. The results demonstrated that a substantial enhancement (up to 61%) in the CH4 yield could be achieved with both nano-scale zero-valent iron (NZVI) and waste iron scraps (WIS) being the added iron. Additionally, the added iron could also achieve effective phosphorus removal from the AD supernatant. |
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| AbstractList | A large amount (25-60%) of degraded organics is converted directly to CO2 during anaerobic digestion (AD) process, which substantially lowers the energy (methane, CH4) yield. In this study, endogenous CO2 fixation by H2 from in-situ iron corrosion was explored to enhancing the CH4 yield. The results demonstrated that a substantial enhancement (up to 61%) in the CH4 yield could be achieved with both nano-scale zero-valent iron (NZVI) and waste iron scraps (WIS) being the added iron. Additionally, the added iron could also achieve effective phosphorus removal from the AD supernatant. •H2 can be generated from anaerobic iron corrosion in anaerobic digestion (AD).•The generated H2 can be utilized for converting CO2 to CH4.•With CO2 fixation, enhancement up to 61% in the CH4 yield is achieved.•The added iron can also achieve phosphorus removal from the AD supernatant. A large amount (25–60%) of degraded organics is converted directly to CO2 during anaerobic digestion (AD) process, which substantially lowers the energy (methane, CH4) yield. In this study, endogenous CO2 fixation by H2 from in-situ iron corrosion was explored to enhancing the CH4 yield. The results demonstrated that a substantial enhancement (up to 61%) in the CH4 yield could be achieved with both nano-scale zero-valent iron (NZVI) and waste iron scraps (WIS) being the added iron. Additionally, the added iron could also achieve effective phosphorus removal from the AD supernatant. |
| Author | Zhao, Dan Hao, Xiaodi Fu, Kunming Hu, Yuansheng |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25455677$$D View this record in MEDLINE/PubMed |
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| Keywords | Waste activated sludge Iron corrosion Carbon fixation Hydrogen Anaerobic digestion |
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| Snippet | •H2 can be generated from anaerobic iron corrosion in anaerobic digestion (AD).•The generated H2 can be utilized for converting CO2 to CH4.•With CO2 fixation,... A large amount (25-60%) of degraded organics is converted directly to CO2 during anaerobic digestion (AD) process, which substantially lowers the energy... |
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| SubjectTerms | Anaerobic digestion Anaerobiosis Carbon capture and storage Carbon dioxide Carbon Dioxide - metabolism Carbon fixation Digestion Fixation Hydrogen Hydrogen - metabolism Iron Iron corrosion Methane Methane - metabolism Phosphorus removal Sewage Waste activated sludge Waste Disposal, Fluid - methods Wastes |
| Title | Enhancing the CH4 yield of anaerobic digestion via endogenous CO2 fixation by exogenous H2 |
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