Evolution of the fractal dimension for simultaneous coagulation and sintering
Simulation results on the evolution of aggregate structure in aerosol processes with coagulation and sintering as the dominant mechanisms are presented. A model for simulation of the three-dimensional morphology of nano-structured aggregates formed by concurrent coagulation and sintering is applied....
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| Published in | Chemical engineering science Vol. 61; no. 1; pp. 293 - 305 |
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| Main Authors | , , , |
| Format | Journal Article Conference Proceeding |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.01.2006
Elsevier |
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| Abstract | Simulation results on the evolution of aggregate structure in aerosol processes with coagulation and sintering as the dominant mechanisms are presented. A model for simulation of the three-dimensional morphology of nano-structured aggregates formed by concurrent coagulation and sintering is applied. The model is based on a stochastic diffusion controlled cluster–cluster aggregation algorithm and sintering is modeled as a successive overlapping of spherical primary particles, which are allowed to grow in order to maintain mass conservation. This leads to computer simulated structured aggregates which are then subject to evaluation. Two different methods to determine the fractal dimension are presented which give comparable results. It is shown that even very small particles show the same fractal behavior. Furthermore, equilibrium structures assuming a constant ratio of the characteristic collision time to the characteristic fusion time are considered as well as the kinetics of structural changes due to a change in the ambient conditions. |
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| AbstractList | Simulation results on the evolution of aggregate structure in aerosol processes with coagulation and sintering as the dominant mechanisms are presented. A model for simulation of the three-dimensional morphology of nano-structured aggregates formed by concurrent coagulation and sintering is applied. The model is based on a stochastic diffusion controlled cluster–cluster aggregation algorithm and sintering is modeled as a successive overlapping of spherical primary particles, which are allowed to grow in order to maintain mass conservation. This leads to computer simulated structured aggregates which are then subject to evaluation. Two different methods to determine the fractal dimension are presented which give comparable results. It is shown that even very small particles show the same fractal behavior. Furthermore, equilibrium structures assuming a constant ratio of the characteristic collision time to the characteristic fusion time are considered as well as the kinetics of structural changes due to a change in the ambient conditions. |
| Author | Al-Zaitone, Belal Schmid, Hans-Joachim Artelt, Christian Peukert, Wolfgang |
| Author_xml | – sequence: 1 givenname: Hans-Joachim surname: Schmid fullname: Schmid, Hans-Joachim email: h.schmid@lfg.uni-erlangen.de organization: Institute of Particle Technology, University Erlangen-Nürnberg, 91052 Erlangen, Germany – sequence: 2 givenname: Belal surname: Al-Zaitone fullname: Al-Zaitone, Belal organization: Institute of Particle Technology, University Erlangen-Nürnberg, 91052 Erlangen, Germany – sequence: 3 givenname: Christian surname: Artelt fullname: Artelt, Christian organization: Institute of Particle Technology, Technical University München, 85748 Garching, Germany – sequence: 4 givenname: Wolfgang surname: Peukert fullname: Peukert, Wolfgang organization: Institute of Particle Technology, University Erlangen-Nürnberg, 91052 Erlangen, Germany |
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| Keywords | Fractals Nanostructure Particle formation Simulation Sintering Coagulation Collision Algorithm Modeling Aggregation Fractal Fractal dimension Flocculation Morphology Aerosols Kinetics Aggregate Diffusion |
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| SubjectTerms | Applied sciences Chemical engineering Coagulation Exact sciences and technology Fractals Nanostructure Particle formation Simulation Sintering Sintering, pelletization, granulation Solid-solid systems |
| Title | Evolution of the fractal dimension for simultaneous coagulation and sintering |
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