Rapid Lithium Diffusion in Order@Disorder Pathways for Fast‐Charging Graphite Anodes

The use of graphite anode renders practical lithium‐ion batteries for effective energy storage. However, graphite anode is the bottleneck to achieve the fast charging of a battery, ascribed to its low operating potential and corresponding incidental lithium plating. Herein the principle of a thin na...

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Published inSmall structures Vol. 1; no. 1
Main Authors Cai, Wenlong, Yan, Chong, Yao, Yu-Xing, Xu, Lei, Xu, Rui, Jiang, Li-Li, Huang, Jia-Qi, Zhang, Qiang
Format Journal Article
LanguageEnglish
Published Weinheim John Wiley & Sons, Inc 01.10.2020
Subjects
Anode effect
Charging
Diffusion coating
Diffusion layers
Diffusion rate
Electrode polarization
Energy storage
fast charging
Graphite
graphite anodes
Lithium-ion batteries
lithium-ion diffusion
porous carbon layers
Storage batteries
three-electrode measurements
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Abstract The use of graphite anode renders practical lithium‐ion batteries for effective energy storage. However, graphite anode is the bottleneck to achieve the fast charging of a battery, ascribed to its low operating potential and corresponding incidental lithium plating. Herein the principle of a thin nanoscale layer on the graphite surface to improve charging capability is investigated by applying a three‐electrode device to precisely record the working behavior. The Li+ diffusion rate is significantly improved by coating a nanoscale turbostratic carbon layer, in which abundant active sites and additional fast Li+ diffusion pathways at the basal‐plane side of graphite sheets render small polarization in a working battery. This fresh understanding enriches the fundamental insights into enhancing the rate performance and facilitating the practical applications of graphite in fast‐charging batteries. The turbostratic carbon layer on the graphite anode affords abundant active sites and fast diffusion pathways to accelerate the transportation of Li ions in a working battery. This renders a reduced polarization and significantly improved rate performance.
AbstractList The use of graphite anode renders practical lithium‐ion batteries for effective energy storage. However, graphite anode is the bottleneck to achieve the fast charging of a battery, ascribed to its low operating potential and corresponding incidental lithium plating. Herein the principle of a thin nanoscale layer on the graphite surface to improve charging capability is investigated by applying a three‐electrode device to precisely record the working behavior. The Li+ diffusion rate is significantly improved by coating a nanoscale turbostratic carbon layer, in which abundant active sites and additional fast Li+ diffusion pathways at the basal‐plane side of graphite sheets render small polarization in a working battery. This fresh understanding enriches the fundamental insights into enhancing the rate performance and facilitating the practical applications of graphite in fast‐charging batteries.
The use of graphite anode renders practical lithium‐ion batteries for effective energy storage. However, graphite anode is the bottleneck to achieve the fast charging of a battery, ascribed to its low operating potential and corresponding incidental lithium plating. Herein the principle of a thin nanoscale layer on the graphite surface to improve charging capability is investigated by applying a three‐electrode device to precisely record the working behavior. The Li+ diffusion rate is significantly improved by coating a nanoscale turbostratic carbon layer, in which abundant active sites and additional fast Li+ diffusion pathways at the basal‐plane side of graphite sheets render small polarization in a working battery. This fresh understanding enriches the fundamental insights into enhancing the rate performance and facilitating the practical applications of graphite in fast‐charging batteries. The turbostratic carbon layer on the graphite anode affords abundant active sites and fast diffusion pathways to accelerate the transportation of Li ions in a working battery. This renders a reduced polarization and significantly improved rate performance.
Author Yao, Yu-Xing
Xu, Rui
Jiang, Li-Li
Zhang, Qiang
Xu, Lei
Cai, Wenlong
Huang, Jia-Qi
Yan, Chong
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  organization: Tsinghua University
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Snippet The use of graphite anode renders practical lithium‐ion batteries for effective energy storage. However, graphite anode is the bottleneck to achieve the fast...
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SubjectTerms Anode effect
Charging
Diffusion coating
Diffusion layers
Diffusion rate
Electrode polarization
Energy storage
fast charging
Graphite
graphite anodes
Lithium-ion batteries
lithium-ion diffusion
porous carbon layers
Storage batteries
three-electrode measurements
Title Rapid Lithium Diffusion in Order@Disorder Pathways for Fast‐Charging Graphite Anodes
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fsstr.202000010
https://www.proquest.com/docview/2509280815
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