Highly Reversible Zn Anode Enabled by Controllable Formation of Nucleation Sites for Zn‐Based Batteries
Aqueous Zn batteries have drawn tremendous attention for their several advantages. However, the challenges of Zn anodes such as the corrosion and ZnO densification have compromised their application in rechargeable Zn‐based batteries. In this paper, a straightforward strategy is employed to facilita...
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| Published in | Advanced functional materials Vol. 30; no. 13 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Hoboken
Wiley Subscription Services, Inc
01.03.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Aqueous Zn batteries have drawn tremendous attention for their several advantages. However, the challenges of Zn anodes such as the corrosion and ZnO densification have compromised their application in rechargeable Zn‐based batteries. In this paper, a straightforward strategy is employed to facilitate the uniform Zn stripping/plating of the Zn anode through using a ZrO2 coating layer, which contributes to the controllable nucleation sites for Zn2+ and fast Zn2+ transportation through the favorable Maxwell–Wagner polarization. As a result, the low polarization (24 mV at 0.25 mA cm−2), high Coulombic efficiency (99.36% at 20 mA cm−2), and long cycle life (over 3800 h at 0.25 mA cm−2) can be obtained for the ZrO2‐coated Zn anode. It is believed that the ZrO2 coating layer can also act as an inert physical barrier to decrease the contact of the anode and electrolyte, thus reducing both the Zn corrosion and formation of ZnO densification, and then improve the reversibility of Zn anode. The results demonstrated in this work provide an appealing strategy for the future development of rechargeable Zn‐based batteries.
A highly reversible Zn anode is achieved through controllable nucleation sites for Zn2+ and fast Zn2+ transportation under the favorable Maxwell–Wagner polarization, in which a low polarization (24 mV), high Coulombic efficiency (99.36%), and long cycle life (over 3800 h) are obtained by employing a ZrO2‐coating layer. |
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| AbstractList | Aqueous Zn batteries have drawn tremendous attention for their several advantages. However, the challenges of Zn anodes such as the corrosion and ZnO densification have compromised their application in rechargeable Zn‐based batteries. In this paper, a straightforward strategy is employed to facilitate the uniform Zn stripping/plating of the Zn anode through using a ZrO2 coating layer, which contributes to the controllable nucleation sites for Zn2+ and fast Zn2+ transportation through the favorable Maxwell–Wagner polarization. As a result, the low polarization (24 mV at 0.25 mA cm−2), high Coulombic efficiency (99.36% at 20 mA cm−2), and long cycle life (over 3800 h at 0.25 mA cm−2) can be obtained for the ZrO2‐coated Zn anode. It is believed that the ZrO2 coating layer can also act as an inert physical barrier to decrease the contact of the anode and electrolyte, thus reducing both the Zn corrosion and formation of ZnO densification, and then improve the reversibility of Zn anode. The results demonstrated in this work provide an appealing strategy for the future development of rechargeable Zn‐based batteries.
A highly reversible Zn anode is achieved through controllable nucleation sites for Zn2+ and fast Zn2+ transportation under the favorable Maxwell–Wagner polarization, in which a low polarization (24 mV), high Coulombic efficiency (99.36%), and long cycle life (over 3800 h) are obtained by employing a ZrO2‐coating layer. Aqueous Zn batteries have drawn tremendous attention for their several advantages. However, the challenges of Zn anodes such as the corrosion and ZnO densification have compromised their application in rechargeable Zn‐based batteries. In this paper, a straightforward strategy is employed to facilitate the uniform Zn stripping/plating of the Zn anode through using a ZrO2 coating layer, which contributes to the controllable nucleation sites for Zn2+ and fast Zn2+ transportation through the favorable Maxwell–Wagner polarization. As a result, the low polarization (24 mV at 0.25 mA cm−2), high Coulombic efficiency (99.36% at 20 mA cm−2), and long cycle life (over 3800 h at 0.25 mA cm−2) can be obtained for the ZrO2‐coated Zn anode. It is believed that the ZrO2 coating layer can also act as an inert physical barrier to decrease the contact of the anode and electrolyte, thus reducing both the Zn corrosion and formation of ZnO densification, and then improve the reversibility of Zn anode. The results demonstrated in this work provide an appealing strategy for the future development of rechargeable Zn‐based batteries. Aqueous Zn batteries have drawn tremendous attention for their several advantages. However, the challenges of Zn anodes such as the corrosion and ZnO densification have compromised their application in rechargeable Zn‐based batteries. In this paper, a straightforward strategy is employed to facilitate the uniform Zn stripping/plating of the Zn anode through using a ZrO 2 coating layer, which contributes to the controllable nucleation sites for Zn 2+ and fast Zn 2+ transportation through the favorable Maxwell–Wagner polarization. As a result, the low polarization (24 mV at 0.25 mA cm −2 ), high Coulombic efficiency (99.36% at 20 mA cm −2 ), and long cycle life (over 3800 h at 0.25 mA cm −2 ) can be obtained for the ZrO 2 ‐coated Zn anode. It is believed that the ZrO 2 coating layer can also act as an inert physical barrier to decrease the contact of the anode and electrolyte, thus reducing both the Zn corrosion and formation of ZnO densification, and then improve the reversibility of Zn anode. The results demonstrated in this work provide an appealing strategy for the future development of rechargeable Zn‐based batteries. |
| Author | Liu, Xiaoyu Wu, Kai Wang, Yonggang Liu, Yuyu Cui, Jin Wang, Zhuo Zhang, Jiujun Yi, Jin Xia, Yongyao Liang, Pengcheng |
| Author_xml | – sequence: 1 givenname: Pengcheng surname: Liang fullname: Liang, Pengcheng organization: Shanghai University – sequence: 2 givenname: Jin surname: Yi fullname: Yi, Jin email: jin.yi@shu.edu.cn organization: Shanghai University – sequence: 3 givenname: Xiaoyu surname: Liu fullname: Liu, Xiaoyu organization: Shanghai University – sequence: 4 givenname: Kai surname: Wu fullname: Wu, Kai organization: Shanghai University – sequence: 5 givenname: Zhuo surname: Wang fullname: Wang, Zhuo organization: Fudan University – sequence: 6 givenname: Jin surname: Cui fullname: Cui, Jin organization: Shanghai University – sequence: 7 givenname: Yuyu surname: Liu fullname: Liu, Yuyu organization: Shanghai University – sequence: 8 givenname: Yonggang surname: Wang fullname: Wang, Yonggang organization: Fudan University – sequence: 9 givenname: Yongyao orcidid: 0000-0001-6379-9655 surname: Xia fullname: Xia, Yongyao email: yyxia@fudan.edu.cn organization: Fudan University – sequence: 10 givenname: Jiujun surname: Zhang fullname: Zhang, Jiujun organization: Shanghai University |
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| Snippet | Aqueous Zn batteries have drawn tremendous attention for their several advantages. However, the challenges of Zn anodes such as the corrosion and ZnO... |
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| SubjectTerms | Anodes Anodic coatings Barriers controllable nucleation Densification Electrode polarization Materials science Nucleation Rechargeable batteries surface modification Zinc oxide Zirconium dioxide Zn anodes Zn corrosion Zn‐based batteries |
| Title | Highly Reversible Zn Anode Enabled by Controllable Formation of Nucleation Sites for Zn‐Based Batteries |
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