MXene‐Based Composites: Synthesis and Applications in Rechargeable Batteries and Supercapacitors

The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti3C2Tx (MXene). The surface of MXenes etched by hydrofluoric acid has hydrophilic groups (F, OH, and O), which leads the surface to be negativel...

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Published inAdvanced materials interfaces Vol. 6; no. 8
Main Authors Yang, Jian, Bao, Weizhai, Jaumaux, Pauline, Zhang, Songtao, Wang, Chengyin, Wang, Guoxiu
Format Journal Article
LanguageEnglish
Published Weinheim John Wiley & Sons, Inc 01.04.2019
Subjects
Batteries
Carbon nitride
Composite materials
Electrochemical analysis
Electrode materials
Hydrofluoric acid
Lithium
lithium‐ion batteries
Metal carbides
MXenes
MXene‐based composites
Rechargeable batteries
sodium‐ion batteries
Supercapacitors
Synthesis
Transition metals
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Abstract The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti3C2Tx (MXene). The surface of MXenes etched by hydrofluoric acid has hydrophilic groups (F, OH, and O), which leads the surface to be negatively charged. Consequently, the negatively charged surface can facilitate the compounding of MXenes with other positively charged materials and prevent MXenes from aggregating with some negatively charged substances, thus promoting the formation of a stable dispersion. The MXene‐based composites have better electrochemical performance than both precursors due to synergistic effects. This review elaborates and discusses the development of MXene‐based composites. It is aimed to summarize the various methods of fabricating MXene‐based composites. The applications of MXene‐based composites in batteries and supercapacitors are presented along with analysis of their excellent electrochemical performances. Finally, the authors propose the approach for further enhancing the electrochemical performances of MXene‐based composite electrode materials. After the discussion of synthesis methods, structures, and properties of MXenes, different kinds of MXene‐based composites are introduced. Thereafter, the article focuses on their synthesis methods and applications in batteries and supercapacitors. Furthermore, the ways to improve the electrochemical performance of MXene‐based composites are also analyzed. Finally, some suggestions for improving the electrochemical performance of MXenes are proposed.
AbstractList The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti3C2Tx (MXene). The surface of MXenes etched by hydrofluoric acid has hydrophilic groups (F, OH, and O), which leads the surface to be negatively charged. Consequently, the negatively charged surface can facilitate the compounding of MXenes with other positively charged materials and prevent MXenes from aggregating with some negatively charged substances, thus promoting the formation of a stable dispersion. The MXene‐based composites have better electrochemical performance than both precursors due to synergistic effects. This review elaborates and discusses the development of MXene‐based composites. It is aimed to summarize the various methods of fabricating MXene‐based composites. The applications of MXene‐based composites in batteries and supercapacitors are presented along with analysis of their excellent electrochemical performances. Finally, the authors propose the approach for further enhancing the electrochemical performances of MXene‐based composite electrode materials.
The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti 3 C 2 T x (MXene). The surface of MXenes etched by hydrofluoric acid has hydrophilic groups (F, OH, and O), which leads the surface to be negatively charged. Consequently, the negatively charged surface can facilitate the compounding of MXenes with other positively charged materials and prevent MXenes from aggregating with some negatively charged substances, thus promoting the formation of a stable dispersion. The MXene‐based composites have better electrochemical performance than both precursors due to synergistic effects. This review elaborates and discusses the development of MXene‐based composites. It is aimed to summarize the various methods of fabricating MXene‐based composites. The applications of MXene‐based composites in batteries and supercapacitors are presented along with analysis of their excellent electrochemical performances. Finally, the authors propose the approach for further enhancing the electrochemical performances of MXene‐based composite electrode materials.
The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti3C2Tx (MXene). The surface of MXenes etched by hydrofluoric acid has hydrophilic groups (F, OH, and O), which leads the surface to be negatively charged. Consequently, the negatively charged surface can facilitate the compounding of MXenes with other positively charged materials and prevent MXenes from aggregating with some negatively charged substances, thus promoting the formation of a stable dispersion. The MXene‐based composites have better electrochemical performance than both precursors due to synergistic effects. This review elaborates and discusses the development of MXene‐based composites. It is aimed to summarize the various methods of fabricating MXene‐based composites. The applications of MXene‐based composites in batteries and supercapacitors are presented along with analysis of their excellent electrochemical performances. Finally, the authors propose the approach for further enhancing the electrochemical performances of MXene‐based composite electrode materials. After the discussion of synthesis methods, structures, and properties of MXenes, different kinds of MXene‐based composites are introduced. Thereafter, the article focuses on their synthesis methods and applications in batteries and supercapacitors. Furthermore, the ways to improve the electrochemical performance of MXene‐based composites are also analyzed. Finally, some suggestions for improving the electrochemical performance of MXenes are proposed.
Author Bao, Weizhai
Jaumaux, Pauline
Wang, Guoxiu
Yang, Jian
Zhang, Songtao
Wang, Chengyin
Author_xml – sequence: 1
  givenname: Jian
  surname: Yang
  fullname: Yang, Jian
  organization: Yangzhou University
– sequence: 2
  givenname: Weizhai
  surname: Bao
  fullname: Bao, Weizhai
  organization: University of Technology Sydney
– sequence: 3
  givenname: Pauline
  surname: Jaumaux
  fullname: Jaumaux, Pauline
  organization: University of Technology Sydney
– sequence: 4
  givenname: Songtao
  surname: Zhang
  fullname: Zhang, Songtao
  organization: Yangzhou University
– sequence: 5
  givenname: Chengyin
  surname: Wang
  fullname: Wang, Chengyin
  email: wangcy@yzu.edu.cn
  organization: Yangzhou University
– sequence: 6
  givenname: Guoxiu
  orcidid: 0000-0003-4295-8578
  surname: Wang
  fullname: Wang, Guoxiu
  email: guoxiu.wang@uts.edu.cn
  organization: University of Technology Sydney
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Xue Q. (e_1_2_8_271_1) 2017
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Snippet The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti3C2Tx...
The family of 2D transition metal carbides, nitrides, and carbonitrides (collectively called MXenes) is rapidly studied since the initial synthesis of Ti 3 C 2...
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SubjectTerms Batteries
Carbon nitride
Composite materials
Electrochemical analysis
Electrode materials
Hydrofluoric acid
Lithium
lithium‐ion batteries
Metal carbides
MXenes
MXene‐based composites
Rechargeable batteries
sodium‐ion batteries
Supercapacitors
Synthesis
Transition metals
Title MXene‐Based Composites: Synthesis and Applications in Rechargeable Batteries and Supercapacitors
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadmi.201802004
https://www.proquest.com/docview/2212618018
Volume 6
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