Impact of SO2 on elemental mercury oxidation over CeO2–TiO2 catalyst
[Display omitted] ► SO2 exhibited different, even contrary, effects on Hg0 oxidation in different conditions. ► With O2, few SO2 promoted Hg0 oxidation, while excess SO2 inhibited Hg0 oxidation. ► There is a balance SO2 concentration, where no obvious effect of SO2 can be observed. ► NO catalyzed SO...
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| Published in | Chemical engineering journal (Lausanne, Switzerland : 1996) Vol. 219; pp. 319 - 326 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.03.2013
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| Subjects | |
| Online Access | Get full text |
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| Abstract | [Display omitted]
► SO2 exhibited different, even contrary, effects on Hg0 oxidation in different conditions. ► With O2, few SO2 promoted Hg0 oxidation, while excess SO2 inhibited Hg0 oxidation. ► There is a balance SO2 concentration, where no obvious effect of SO2 can be observed. ► NO catalyzed SO2 conversion to SO3, and thus relieved the inhibitive effect of SO2.
Effect of SO2 on elemental mercury (Hg0) oxidation over a highly active CeO2–TiO2 catalyst was systematically investigated. SO2 was found to have different, even contrary, effects on Hg0 oxidation under different flue gas conditions. In pure N2 atmosphere, SO2 inhibited Hg0 oxidation. In N2 plus O2 atmosphere, low concentration of SO2 promoted Hg0 oxidation, while high concentration of SO2 deteriorated Hg0 oxidation. The promotional effect of SO2 on Hg0 oxidation was probably due to SO3 generated from SO2 oxidation, and the inhibitive effect of SO2 on Hg0 oxidation was attributed to the competitive adsorption between SO2 and Hg0. The results suggest a balance point for SO2 concentration, where the promotional effect on Hg0 oxidation by SO3 originated from SO2 is equal to the inhibitive effect of SO2 on Hg0 adsorption and subsequent oxidation via the Langmuir–Hinshelwood mechanism. In the presence of NO, SO2 with the aid of O2 exhibited promotional effect on Hg0 oxidation through NO-catalyzed oxidation to form SO3 and hence a balance point of higher SO2 concentration. However, without O2, SO2 greatly limited Hg0 oxidation in the presence of NO. When HCl was present, most Hg0 oxidation was due to reactions between active chlorine species and adsorbed Hg0. SO2 inhibited Hg0 adsorption and therefore deteriorated Hg0 oxidation by chlorine species. When both NO and HCl were present, NO accelerated the conversion of SO2 to SO3, and hence relieved the prohibitive effect of SO2 on Hg0 oxidation by HCl. |
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| AbstractList | Effect of SO₂ on elemental mercury (Hg⁰) oxidation over a highly active CeO₂–TiO₂ catalyst was systematically investigated. SO₂ was found to have different, even contrary, effects on Hg⁰ oxidation under different flue gas conditions. In pure N₂ atmosphere, SO₂ inhibited Hg⁰ oxidation. In N₂ plus O₂ atmosphere, low concentration of SO₂ promoted Hg⁰ oxidation, while high concentration of SO₂ deteriorated Hg⁰ oxidation. The promotional effect of SO₂ on Hg⁰ oxidation was probably due to SO₃ generated from SO₂ oxidation, and the inhibitive effect of SO₂ on Hg⁰ oxidation was attributed to the competitive adsorption between SO₂ and Hg⁰. The results suggest a balance point for SO₂ concentration, where the promotional effect on Hg⁰ oxidation by SO₃ originated from SO₂ is equal to the inhibitive effect of SO₂ on Hg⁰ adsorption and subsequent oxidation via the Langmuir–Hinshelwood mechanism. In the presence of NO, SO₂ with the aid of O₂ exhibited promotional effect on Hg⁰ oxidation through NO-catalyzed oxidation to form SO₃ and hence a balance point of higher SO₂ concentration. However, without O₂, SO₂ greatly limited Hg⁰ oxidation in the presence of NO. When HCl was present, most Hg⁰ oxidation was due to reactions between active chlorine species and adsorbed Hg⁰. SO₂ inhibited Hg⁰ adsorption and therefore deteriorated Hg⁰ oxidation by chlorine species. When both NO and HCl were present, NO accelerated the conversion of SO₂ to SO₃, and hence relieved the prohibitive effect of SO₂ on Hg⁰ oxidation by HCl. [Display omitted] ► SO2 exhibited different, even contrary, effects on Hg0 oxidation in different conditions. ► With O2, few SO2 promoted Hg0 oxidation, while excess SO2 inhibited Hg0 oxidation. ► There is a balance SO2 concentration, where no obvious effect of SO2 can be observed. ► NO catalyzed SO2 conversion to SO3, and thus relieved the inhibitive effect of SO2. Effect of SO2 on elemental mercury (Hg0) oxidation over a highly active CeO2–TiO2 catalyst was systematically investigated. SO2 was found to have different, even contrary, effects on Hg0 oxidation under different flue gas conditions. In pure N2 atmosphere, SO2 inhibited Hg0 oxidation. In N2 plus O2 atmosphere, low concentration of SO2 promoted Hg0 oxidation, while high concentration of SO2 deteriorated Hg0 oxidation. The promotional effect of SO2 on Hg0 oxidation was probably due to SO3 generated from SO2 oxidation, and the inhibitive effect of SO2 on Hg0 oxidation was attributed to the competitive adsorption between SO2 and Hg0. The results suggest a balance point for SO2 concentration, where the promotional effect on Hg0 oxidation by SO3 originated from SO2 is equal to the inhibitive effect of SO2 on Hg0 adsorption and subsequent oxidation via the Langmuir–Hinshelwood mechanism. In the presence of NO, SO2 with the aid of O2 exhibited promotional effect on Hg0 oxidation through NO-catalyzed oxidation to form SO3 and hence a balance point of higher SO2 concentration. However, without O2, SO2 greatly limited Hg0 oxidation in the presence of NO. When HCl was present, most Hg0 oxidation was due to reactions between active chlorine species and adsorbed Hg0. SO2 inhibited Hg0 adsorption and therefore deteriorated Hg0 oxidation by chlorine species. When both NO and HCl were present, NO accelerated the conversion of SO2 to SO3, and hence relieved the prohibitive effect of SO2 on Hg0 oxidation by HCl. |
| Author | Li, Liqing Zhao, Yongchun Wu, Chang-Yu Li, Ying Zhang, Junying Li, Hailong |
| Author_xml | – sequence: 1 givenname: Hailong surname: Li fullname: Li, Hailong organization: School of Energy Science and Engineering, Central South University, Changsha 410083, China – sequence: 2 givenname: Chang-Yu surname: Wu fullname: Wu, Chang-Yu organization: Department of Environmental Engineering Sciences, University of Florida, Gainesville, FL 32611, United States – sequence: 3 givenname: Ying surname: Li fullname: Li, Ying organization: Department of Mechanical Engineering, University of Wisconsin–Milwaukee, Milwaukee, WI 53211, United States – sequence: 4 givenname: Liqing surname: Li fullname: Li, Liqing email: lienergycsu@gmail.com organization: School of Energy Science and Engineering, Central South University, Changsha 410083, China – sequence: 5 givenname: Yongchun surname: Zhao fullname: Zhao, Yongchun organization: State Key Laboratory of Coal Combustion, Huazhong University of Science and Technology, Wuhan 430074, China – sequence: 6 givenname: Junying surname: Zhang fullname: Zhang, Junying organization: State Key Laboratory of Coal Combustion, Huazhong University of Science and Technology, Wuhan 430074, China |
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► SO2 exhibited different, even contrary, effects on Hg0 oxidation in different conditions. ► With O2, few SO2 promoted Hg0 oxidation, while... Effect of SO₂ on elemental mercury (Hg⁰) oxidation over a highly active CeO₂–TiO₂ catalyst was systematically investigated. SO₂ was found to have different,... |
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| SubjectTerms | adsorption CeO2–TiO2 chemical engineering chlorine Coal combustion Flue gas Mercury oxidation Sulfur dioxide |
| Title | Impact of SO2 on elemental mercury oxidation over CeO2–TiO2 catalyst |
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