Electroreduction of oxygen on Pd catalysts supported on Ti-modified carbon
Carbon supports modified with well dispersed anatase TiO2 (C–Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were synthesized with various Ti loadings and used to support Pd catalysts for oxygen reduction. The anatase nanoparticles increased in size with increasin...
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| Published in | Current applied physics Vol. 12; no. 6; pp. 1476 - 1480 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.11.2012
한국물리학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1567-1739 1878-1675 |
| DOI | 10.1016/j.cap.2012.04.011 |
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| Abstract | Carbon supports modified with well dispersed anatase TiO2 (C–Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were synthesized with various Ti loadings and used to support Pd catalysts for oxygen reduction. The anatase nanoparticles increased in size with increasing Ti loading. Pd dispersion improved with increasing Ti loading up to the C–Ti-0.75, which resulted in the best catalytic activity. Although the Pd dispersion was lowest on the C–Ti-1.0, it showed better catalytic performance than the catalysts supported on C–Ti-0.25 and C–Ti-0.5. At 0.8V (vs. RHE), the best catalytic activity achieved was respectively 2.7 and 2.7 times the mass and specific activities of Pd supported on un-modified carbon. The interaction between Pd and highly dispersed TiO2 is believed to improve the catalytic activity of Pd supported on TiO2-modified carbons.
► TiO2-modified carbon as support of Pd for oxygen reduction reaction. ► Different Pd dispersion depending on Ti contents. ► Positive effect of interaction between Pd and TiO2 on oxygen reduction. |
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| AbstractList | Carbon supports modified with well dispersed anatase TiO2 (CeTi-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were synthesized with various Ti loadings and used to support Pd catalysts for oxygen reduction. The anatase nanoparticles increased in size with increasing Ti loading.
Pd dispersion improved with increasing Ti loading up to the CeTi-0.75, which resulted in the best catalytic activity. Although the Pd dispersion was lowest on the CeTi-1.0, it showed better catalytic performance than the catalysts supported on CeTi-0.25 and CeTi-0.5. At 0.8 V (vs. RHE), the best catalytic activity achieved was respectively 2.7 and 2.7 times the mass and specific activities of Pd supported on un-modified carbon. The interaction between Pd and highly dispersed TiO2 is believed to improve the catalytic activity of Pd supported on TiO2-modified carbons. KCI Citation Count: 8 Carbon supports modified with well dispersed anatase TiO2 (C–Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were synthesized with various Ti loadings and used to support Pd catalysts for oxygen reduction. The anatase nanoparticles increased in size with increasing Ti loading. Pd dispersion improved with increasing Ti loading up to the C–Ti-0.75, which resulted in the best catalytic activity. Although the Pd dispersion was lowest on the C–Ti-1.0, it showed better catalytic performance than the catalysts supported on C–Ti-0.25 and C–Ti-0.5. At 0.8V (vs. RHE), the best catalytic activity achieved was respectively 2.7 and 2.7 times the mass and specific activities of Pd supported on un-modified carbon. The interaction between Pd and highly dispersed TiO2 is believed to improve the catalytic activity of Pd supported on TiO2-modified carbons. ► TiO2-modified carbon as support of Pd for oxygen reduction reaction. ► Different Pd dispersion depending on Ti contents. ► Positive effect of interaction between Pd and TiO2 on oxygen reduction. Carbon supports modified with well dispersed anatase TiO2 (C-Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were synthesized with various Ti loadings and used to support Pd catalysts for oxygen reduction. The anatase nanoparticles increased in size with increasing Ti loading. Pd dispersion improved with increasing Ti loading up to the C-Ti-0.75, which resulted in the best catalytic activity. Although the Pd dispersion was lowest on the C-Ti-1.0, it showed better catalytic performance than the catalysts supported on C-Ti-0.25 and C-Ti-0.5. At 0.8 V (vs. RHE), the best catalytic activity achieved was respectively 2.7 and 2.7 times the mass and specific activities of Pd supported on un-modified carbon. The interaction between Pd and highly dispersed TiO2 is believed to improve the catalytic activity of Pd supported on TiO2-modified carbons. Carbon supports modified with well dispersed anatase TiO₂ (C–Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were synthesized with various Ti loadings and used to support Pd catalysts for oxygen reduction. The anatase nanoparticles increased in size with increasing Ti loading. Pd dispersion improved with increasing Ti loading up to the C–Ti-0.75, which resulted in the best catalytic activity. Although the Pd dispersion was lowest on the C–Ti-1.0, it showed better catalytic performance than the catalysts supported on C–Ti-0.25 and C–Ti-0.5. At 0.8V (vs. RHE), the best catalytic activity achieved was respectively 2.7 and 2.7 times the mass and specific activities of Pd supported on un-modified carbon. The interaction between Pd and highly dispersed TiO₂ is believed to improve the catalytic activity of Pd supported on TiO₂-modified carbons. |
| Author | Kim, Pil Nahm, Kee Suk Bae, Sung Jong |
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| CitedBy_id | crossref_primary_10_1016_j_jwpe_2024_105880 crossref_primary_10_1080_19443994_2014_903205 crossref_primary_10_1016_j_cap_2015_04_031 crossref_primary_10_1002_jctb_5056 crossref_primary_10_1016_j_mseb_2015_03_016 crossref_primary_10_1007_s11164_018_3375_3 crossref_primary_10_3390_catal5031221 crossref_primary_10_1016_j_sajce_2017_11_001 crossref_primary_10_1016_j_jelechem_2016_09_034 |
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| Keywords | Polymer electrolyte fuel cells (PEMFCs) Carbon-TiO2 composite Oxygen reduction reaction Pd catalyst |
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| Snippet | Carbon supports modified with well dispersed anatase TiO2 (C–Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were... Carbon supports modified with well dispersed anatase TiO₂ (C–Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were... Carbon supports modified with well dispersed anatase TiO2 (C-Ti-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were... Carbon supports modified with well dispersed anatase TiO2 (CeTi-X; X (0.25, 0.5, 0.75, and 1.0) represents mass ratio of Ti precursor to carbon) were... |
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| SubjectTerms | Anatase Carbon Carbon-TiO2 composite Catalysis Catalysts Catalytic activity nanoparticles oxygen Oxygen reduction reaction Palladium Pd catalyst physics Polymer electrolyte fuel cells (PEMFCs) Titanium Titanium dioxide 물리학 |
| Title | Electroreduction of oxygen on Pd catalysts supported on Ti-modified carbon |
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