Inorganic Halide Perovskite Solar Cells: Progress and Challenges

All‐inorganic perovskite semiconductors have recently drawn increasing attention owing to their outstanding thermal stability. Although all‐inorganic perovskite solar cells (PSCs) have achieved significant progress in recent years, they still fall behind their prototype organic–inorganic counterpart...

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Published inAdvanced energy materials Vol. 10; no. 23
Main Authors Tian, Jingjing, Xue, Qifan, Yao, Qin, Li, Ning, Brabec, Christoph J., Yip, Hin‐Lap
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 01.06.2020
Subjects
Composition
Electron transport
inorganic perovskite
lead‐based
lead‐free perovskites
Optimization
perovskite solar cells
Perovskites
Photovoltaic cells
Physical properties
Semiconductors
Solar cells
Thermal stability
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Abstract All‐inorganic perovskite semiconductors have recently drawn increasing attention owing to their outstanding thermal stability. Although all‐inorganic perovskite solar cells (PSCs) have achieved significant progress in recent years, they still fall behind their prototype organic–inorganic counterparts owing to severe energy losses. Therefore, there is considerable interest in further improving the performance of all‐inorganic PSCs by synergic optimization of perovskite films and device interfaces. This review article provides an overview of recent progress in inorganic PSCs in terms of lead‐based and lead‐free composition. The physical properties of all‐inorganic perovskite semiconductors as well as the hole/electron transporting materials are discussed to unveil the important role of composition engineering and interface modification. Finally, a discussion of the prospects and challenges for all‐inorganic PSCs in the near future is presented. Recent progress in inorganic lead‐based and lead‐free CsBX3 perovskite solar cells using various strategies is reviewed and their prospects and challenges in the future are discussed in detail.
AbstractList All‐inorganic perovskite semiconductors have recently drawn increasing attention owing to their outstanding thermal stability. Although all‐inorganic perovskite solar cells (PSCs) have achieved significant progress in recent years, they still fall behind their prototype organic–inorganic counterparts owing to severe energy losses. Therefore, there is considerable interest in further improving the performance of all‐inorganic PSCs by synergic optimization of perovskite films and device interfaces. This review article provides an overview of recent progress in inorganic PSCs in terms of lead‐based and lead‐free composition. The physical properties of all‐inorganic perovskite semiconductors as well as the hole/electron transporting materials are discussed to unveil the important role of composition engineering and interface modification. Finally, a discussion of the prospects and challenges for all‐inorganic PSCs in the near future is presented.
All‐inorganic perovskite semiconductors have recently drawn increasing attention owing to their outstanding thermal stability. Although all‐inorganic perovskite solar cells (PSCs) have achieved significant progress in recent years, they still fall behind their prototype organic–inorganic counterparts owing to severe energy losses. Therefore, there is considerable interest in further improving the performance of all‐inorganic PSCs by synergic optimization of perovskite films and device interfaces. This review article provides an overview of recent progress in inorganic PSCs in terms of lead‐based and lead‐free composition. The physical properties of all‐inorganic perovskite semiconductors as well as the hole/electron transporting materials are discussed to unveil the important role of composition engineering and interface modification. Finally, a discussion of the prospects and challenges for all‐inorganic PSCs in the near future is presented. Recent progress in inorganic lead‐based and lead‐free CsBX3 perovskite solar cells using various strategies is reviewed and their prospects and challenges in the future are discussed in detail.
Author Yao, Qin
Li, Ning
Brabec, Christoph J.
Tian, Jingjing
Yip, Hin‐Lap
Xue, Qifan
Author_xml – sequence: 1
  givenname: Jingjing
  surname: Tian
  fullname: Tian, Jingjing
  organization: South China University of Technology
– sequence: 2
  givenname: Qifan
  surname: Xue
  fullname: Xue, Qifan
  email: qfxue@scut.edu.cn
  organization: South China Institute of Collaborative Innovation
– sequence: 3
  givenname: Qin
  surname: Yao
  fullname: Yao, Qin
  organization: South China University of Technology
– sequence: 4
  givenname: Ning
  surname: Li
  fullname: Li, Ning
  organization: Zhengzhou University
– sequence: 5
  givenname: Christoph J.
  surname: Brabec
  fullname: Brabec, Christoph J.
  organization: Forschungszentrum Jülich
– sequence: 6
  givenname: Hin‐Lap
  orcidid: 0000-0002-5750-9751
  surname: Yip
  fullname: Yip, Hin‐Lap
  email: msangusyip@scut.edu.cn
  organization: South China Institute of Collaborative Innovation
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Snippet All‐inorganic perovskite semiconductors have recently drawn increasing attention owing to their outstanding thermal stability. Although all‐inorganic...
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wiley
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SubjectTerms Composition
Electron transport
inorganic perovskite
lead‐based
lead‐free perovskites
Optimization
perovskite solar cells
Perovskites
Photovoltaic cells
Physical properties
Semiconductors
Solar cells
Thermal stability
Title Inorganic Halide Perovskite Solar Cells: Progress and Challenges
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Faenm.202000183
https://www.proquest.com/docview/2413318257
Volume 10
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