Microwave Combustion for Rapidly Synthesizing Pore‐Size‐Controllable Porous Graphene
Porous graphene has been widely applied in energy storage, electrocatalysis, photoelectron devices, etc. However, the producing process for porous graphene usually needs long time and is a tedious step. In this work, porous graphene is prepared with controllable pore size by using active metal nanop...
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| Published in | Advanced functional materials Vol. 28; no. 22 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Hoboken
Wiley Subscription Services, Inc
30.05.2018
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Porous graphene has been widely applied in energy storage, electrocatalysis, photoelectron devices, etc. However, the producing process for porous graphene usually needs long time and is a tedious step. In this work, porous graphene is prepared with controllable pore size by using active metal nanoparticles to catalytically oxidize carbon under microwave combustion process within tens of seconds. The ion exchange membrane based on porous graphene with ≈5 nm pore diameter exhibits a great performance for salinity gradient power generation application with a power density output of ≈1.15 W m−2. This work highlights a new strategy for the design and synthesis of pore‐size‐controllable porous graphene and provides new opportunities for 2D porous nanomaterials.
Pore‐size‐controllable porous graphene is rapidly synthesized by utilizing catalytic oxidation combined with microwave combustion. By adjusting the concentration of the precursor and the microwave‐treatment times, the pore size can be easily mediated to ≈5, ≈30, and ≈100 nm. An ion exchange membrane assembled with the porous graphene shows great performance with an output power density of 1.15 W m−2. |
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| AbstractList | Porous graphene has been widely applied in energy storage, electrocatalysis, photoelectron devices, etc. However, the producing process for porous graphene usually needs long time and is a tedious step. In this work, porous graphene is prepared with controllable pore size by using active metal nanoparticles to catalytically oxidize carbon under microwave combustion process within tens of seconds. The ion exchange membrane based on porous graphene with ≈5 nm pore diameter exhibits a great performance for salinity gradient power generation application with a power density output of ≈1.15 W m−2. This work highlights a new strategy for the design and synthesis of pore‐size‐controllable porous graphene and provides new opportunities for 2D porous nanomaterials. Porous graphene has been widely applied in energy storage, electrocatalysis, photoelectron devices, etc. However, the producing process for porous graphene usually needs long time and is a tedious step. In this work, porous graphene is prepared with controllable pore size by using active metal nanoparticles to catalytically oxidize carbon under microwave combustion process within tens of seconds. The ion exchange membrane based on porous graphene with ≈5 nm pore diameter exhibits a great performance for salinity gradient power generation application with a power density output of ≈1.15 W m−2. This work highlights a new strategy for the design and synthesis of pore‐size‐controllable porous graphene and provides new opportunities for 2D porous nanomaterials. Pore‐size‐controllable porous graphene is rapidly synthesized by utilizing catalytic oxidation combined with microwave combustion. By adjusting the concentration of the precursor and the microwave‐treatment times, the pore size can be easily mediated to ≈5, ≈30, and ≈100 nm. An ion exchange membrane assembled with the porous graphene shows great performance with an output power density of 1.15 W m−2. Porous graphene has been widely applied in energy storage, electrocatalysis, photoelectron devices, etc. However, the producing process for porous graphene usually needs long time and is a tedious step. In this work, porous graphene is prepared with controllable pore size by using active metal nanoparticles to catalytically oxidize carbon under microwave combustion process within tens of seconds. The ion exchange membrane based on porous graphene with ≈5 nm pore diameter exhibits a great performance for salinity gradient power generation application with a power density output of ≈1.15 W m −2 . This work highlights a new strategy for the design and synthesis of pore‐size‐controllable porous graphene and provides new opportunities for 2D porous nanomaterials. |
| Author | Huang, Liang Wu, Jiabin Zhou, Jun Wan, Jun Xiong, Liukang Hu, Zhimi Li, Tianqi Yu, Huimin |
| Author_xml | – sequence: 1 givenname: Jun surname: Wan fullname: Wan, Jun organization: Huazhong University of Science and Technology – sequence: 2 givenname: Liang surname: Huang fullname: Huang, Liang organization: Huazhong University of Science and Technology – sequence: 3 givenname: Jiabin surname: Wu fullname: Wu, Jiabin organization: Huazhong University of Science and Technology – sequence: 4 givenname: Liukang surname: Xiong fullname: Xiong, Liukang organization: Huazhong University of Science and Technology – sequence: 5 givenname: Zhimi surname: Hu fullname: Hu, Zhimi organization: Huazhong University of Science and Technology – sequence: 6 givenname: Huimin surname: Yu fullname: Yu, Huimin organization: Huazhong University of Science and Technology – sequence: 7 givenname: Tianqi surname: Li fullname: Li, Tianqi organization: Huazhong University of Science and Technology – sequence: 8 givenname: Jun orcidid: 0000-0003-4799-8165 surname: Zhou fullname: Zhou, Jun email: jun.zhou@mail.hust.edu.cn organization: Huazhong University of Science and Technology |
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| Snippet | Porous graphene has been widely applied in energy storage, electrocatalysis, photoelectron devices, etc. However, the producing process for porous graphene... |
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| SubjectTerms | Electric power generation Energy storage Graphene Ion exchange Materials science microwave combustion Nanomaterials Pore size Porosity porous graphene |
| Title | Microwave Combustion for Rapidly Synthesizing Pore‐Size‐Controllable Porous Graphene |
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