Detecting Mercury (II) and Thiocyanate Using “Turn-on” Fluorescence of Graphene Quantum Dots
In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The fluorescence of the GQDs could be almost completely quenched (about 96%) by adding Hg 2+ . Quenching was far less efficient with other similar heavy...
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Published in | Journal of fluorescence Vol. 30; no. 5; pp. 1181 - 1187 |
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Main Authors | , , , |
Format | Journal Article |
Language | English |
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01.09.2020
Springer Nature B.V |
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Abstract | In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The fluorescence of the GQDs could be almost completely quenched (about 96%) by adding Hg
2+
. Quenching was far less efficient with other similar heavy metals, Tl
+
, Pb
2+
and Bi
3+
. Fluorescence could be near quantitatively restored through the introduction of thiocyanate. This “turn-on” fluorescence can thus be used to detect both or either environmental and physiological contaminants mercury and thiocyanate and could prove useful for the development of simple point-of-care diagnostics in the future.
Graphical Abstract |
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AbstractList | In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The fluorescence of the GQDs could be almost completely quenched (about 96%) by adding Hg
2+
. Quenching was far less efficient with other similar heavy metals, Tl
+
, Pb
2+
and Bi
3+
. Fluorescence could be near quantitatively restored through the introduction of thiocyanate. This “turn-on” fluorescence can thus be used to detect both or either environmental and physiological contaminants mercury and thiocyanate and could prove useful for the development of simple point-of-care diagnostics in the future.
Graphical Abstract In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The fluorescence of the GQDs could be almost completely quenched (about 96%) by adding Hg2+. Quenching was far less efficient with other similar heavy metals, Tl+, Pb2+ and Bi3+. Fluorescence could be near quantitatively restored through the introduction of thiocyanate. This “turn-on” fluorescence can thus be used to detect both or either environmental and physiological contaminants mercury and thiocyanate and could prove useful for the development of simple point-of-care diagnostics in the future. In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The fluorescence of the GQDs could be almost completely quenched (about 96%) by adding Hg . Quenching was far less efficient with other similar heavy metals, Tl , Pb and Bi . Fluorescence could be near quantitatively restored through the introduction of thiocyanate. This "turn-on" fluorescence can thus be used to detect both or either environmental and physiological contaminants mercury and thiocyanate and could prove useful for the development of simple point-of-care diagnostics in the future. Graphical Abstract. |
Author | Rahdar, Abbas Askari, Faezeh Dashti, Mohadeseh Trant, John F. |
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BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32691262$$D View this record in MEDLINE/PubMed |
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Snippet | In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The... In this work, 1.8 nm graphene quantum dots (GQDs), exhibiting bright blue fluorescence, were prepared using a bottom-up synthesis from citric acid. The... |
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SubjectTerms | Analytical Chemistry Biochemistry Biological and Medical Physics Biomedical and Life Sciences Biomedicine Biophysics Biotechnology Citric acid Contaminants Fluorescence Fluorescent Dyes - chemical synthesis Fluorescent Dyes - chemistry Graphene Graphite - chemistry Heavy metals Lead Mercury (metal) Mercury - analysis Original Article Quantum dots Quantum Dots - chemistry Spectrometry, Fluorescence Thiocyanates Thiocyanates - analysis |
Title | Detecting Mercury (II) and Thiocyanate Using “Turn-on” Fluorescence of Graphene Quantum Dots |
URI | https://link.springer.com/article/10.1007/s10895-020-02586-z https://www.ncbi.nlm.nih.gov/pubmed/32691262 https://www.proquest.com/docview/2437147511 https://search.proquest.com/docview/2425898530 |
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