A paper-based electrode using a graphene dot/PEDOT:PSS composite for flexible solar cells
We have synthesized a metal-free composite ink that contains graphene dots (GDs) and poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) that can be used on paper to serve as the counter electrode in a flexible dye-sensitized solar cell (DSSC). This paper-based GD/PEDOT:PSS electrode...
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| Published in | Nano energy Vol. 36; pp. 260 - 267 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.06.2017
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| Subjects | |
| Online Access | Get full text |
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| Abstract | We have synthesized a metal-free composite ink that contains graphene dots (GDs) and poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) that can be used on paper to serve as the counter electrode in a flexible dye-sensitized solar cell (DSSC). This paper-based GD/PEDOT:PSS electrode is low-cost, light-weight, flexible, environmentally friendly, and easy to cut and process for device fabrication. We determined the GD/PEDOT:PSS composite effectively fills the dense micro-pores in the paper substrate, which leads to improved carrier transport in the electrode and a 3-fold enhanced cell efficiency as compared to the paper electrode made with sputtered Pt. Moreover, the DSSC with the paper electrode featuring the GD/PEDOT:PSS composite did not fail in photovoltaic tests even after bending the electrode 150 times, whereas the device made with the Pt-based paper electrode decreased in efficiency by 45% after such manipulation. These exceptional properties make the metal-free GD/PEDOT:PSS composite ink a promising electrode material for a wide variety of flexible electronic applications.
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•Water–soluble GDs and PEDOT:PSS are used for preparing Pt–free counter electrode.•GD/PEDOT:PSS–coated paper electrode exhibits higher performance than that with the paper with sputtered Pt.•GD/PEDOT:PSS–coated paper electrode shows unfailing performance after 150 bending cycles.•GD/PEDOT:PSS–coated paper electrode is low–cost, light–weight, and environmental friendly. |
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| AbstractList | We have synthesized a metal-free composite ink that contains graphene dots (GDs) and poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) that can be used on paper to serve as the counter electrode in a flexible dye-sensitized solar cell (DSSC). This paper-based GD/PEDOT:PSS electrode is low-cost, light-weight, flexible, environmentally friendly, and easy to cut and process for device fabrication. We determined the GD/PEDOT:PSS composite effectively fills the dense micro-pores in the paper substrate, which leads to improved carrier transport in the electrode and a 3-fold enhanced cell efficiency as compared to the paper electrode made with sputtered Pt. Moreover, the DSSC with the paper electrode featuring the GD/PEDOT:PSS composite did not fail in photovoltaic tests even after bending the electrode 150 times, whereas the device made with the Pt-based paper electrode decreased in efficiency by 45% after such manipulation. These exceptional properties make the metal-free GD/PEDOT:PSS composite ink a promising electrode material for a wide variety of flexible electronic applications.
[Display omitted]
•Water–soluble GDs and PEDOT:PSS are used for preparing Pt–free counter electrode.•GD/PEDOT:PSS–coated paper electrode exhibits higher performance than that with the paper with sputtered Pt.•GD/PEDOT:PSS–coated paper electrode shows unfailing performance after 150 bending cycles.•GD/PEDOT:PSS–coated paper electrode is low–cost, light–weight, and environmental friendly. |
| Author | Wu, Chih-I Lee, Chuan-Pei Ho, Kuo-Chuan Lai, Kun-Yu Lau, Shu-Ping He, Jr-Hau Lin, Chin-An Li, Chun-Ting |
| Author_xml | – sequence: 1 givenname: Chuan-Pei surname: Lee fullname: Lee, Chuan-Pei organization: Computer, Electrical and Mathematical Sciences and Engineering (CEMSE) Division, King Abdullah, University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia – sequence: 2 givenname: Kun-Yu surname: Lai fullname: Lai, Kun-Yu organization: Department of Optics and Photonics, National Central University, Chung-Li 32001, Taiwan, ROC – sequence: 3 givenname: Chin-An surname: Lin fullname: Lin, Chin-An organization: Computer, Electrical and Mathematical Sciences and Engineering (CEMSE) Division, King Abdullah, University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia – sequence: 4 givenname: Chun-Ting surname: Li fullname: Li, Chun-Ting organization: Department of Chemical Engineering, National Taiwan University, Taipei 10617, Taiwan, ROC – sequence: 5 givenname: Kuo-Chuan surname: Ho fullname: Ho, Kuo-Chuan organization: Department of Chemical Engineering, National Taiwan University, Taipei 10617, Taiwan, ROC – sequence: 6 givenname: Chih-I surname: Wu fullname: Wu, Chih-I organization: Institute of Photonics and Optoelectronics and Department of Electrical Engineering, National Taiwan University, Taipei 10617, Taiwan, ROC – sequence: 7 givenname: Shu-Ping surname: Lau fullname: Lau, Shu-Ping organization: Department of Applied Physics, The Hong Kong Polytechnic University, Hong Kong, China – sequence: 8 givenname: Jr-Hau surname: He fullname: He, Jr-Hau email: jrhau.he@kaust.edu.sa organization: Computer, Electrical and Mathematical Sciences and Engineering (CEMSE) Division, King Abdullah, University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia |
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| Snippet | We have synthesized a metal-free composite ink that contains graphene dots (GDs) and poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS) that... |
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| SubjectTerms | Conducting polymer Dye-sensitized solar cell Flexible electrode Graphene dots Metal-free counter electrode Paper electrode |
| Title | A paper-based electrode using a graphene dot/PEDOT:PSS composite for flexible solar cells |
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