Strain softened bending modulus of graphene oxide
•The flexibility of graphene oxide is regulated by strain.•The strained graphene oxide can be more flexible than graphene.•The mechanism of strain softened bending modulus is revealed. Graphene oxide is attractive in flexible materials due to its biocompatibility. Herein, flexibility of graphene oxi...
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| Published in | Carbon trends Vol. 7; p. 100167 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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Elsevier Ltd
01.04.2022
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| Abstract | •The flexibility of graphene oxide is regulated by strain.•The strained graphene oxide can be more flexible than graphene.•The mechanism of strain softened bending modulus is revealed.
Graphene oxide is attractive in flexible materials due to its biocompatibility. Herein, flexibility of graphene oxide under uniaxial tensile strain has been studied in term of the bending modulus. It is demonstrated that tensile strain plays an effective role in softening the bending modulus of graphene oxide. The strained graphene oxide can be even more flexible than graphene. The mechanism of strain softened bending modulus is discussed where weakened atomic bonding accounts directly for the enhanced flexibility. Particularly, an important factor for softened bending modulus is proposed, i.e. alignment of epoxide groups. The degradation of bending modulus is more prominent when the epoxides are aligned along the bending direction. This work not only proposes an effective method to enhance the flexibility of graphene oxide, but also unveils the mechanism of softened bending modulus, which could be useful in design of highly flexible materials.
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| AbstractList | •The flexibility of graphene oxide is regulated by strain.•The strained graphene oxide can be more flexible than graphene.•The mechanism of strain softened bending modulus is revealed.
Graphene oxide is attractive in flexible materials due to its biocompatibility. Herein, flexibility of graphene oxide under uniaxial tensile strain has been studied in term of the bending modulus. It is demonstrated that tensile strain plays an effective role in softening the bending modulus of graphene oxide. The strained graphene oxide can be even more flexible than graphene. The mechanism of strain softened bending modulus is discussed where weakened atomic bonding accounts directly for the enhanced flexibility. Particularly, an important factor for softened bending modulus is proposed, i.e. alignment of epoxide groups. The degradation of bending modulus is more prominent when the epoxides are aligned along the bending direction. This work not only proposes an effective method to enhance the flexibility of graphene oxide, but also unveils the mechanism of softened bending modulus, which could be useful in design of highly flexible materials.
[Display omitted] Graphene oxide is attractive in flexible materials due to its biocompatibility. Herein, flexibility of graphene oxide under uniaxial tensile strain has been studied in term of the bending modulus. It is demonstrated that tensile strain plays an effective role in softening the bending modulus of graphene oxide. The strained graphene oxide can be even more flexible than graphene. The mechanism of strain softened bending modulus is discussed where weakened atomic bonding accounts directly for the enhanced flexibility. Particularly, an important factor for softened bending modulus is proposed, i.e. alignment of epoxide groups. The degradation of bending modulus is more prominent when the epoxides are aligned along the bending direction. This work not only proposes an effective method to enhance the flexibility of graphene oxide, but also unveils the mechanism of softened bending modulus, which could be useful in design of highly flexible materials. |
| ArticleNumber | 100167 |
| Author | Yu, Songding Liu, Lizhao Jiao, Lei Zhao, Jijun |
| Author_xml | – sequence: 1 givenname: Songding surname: Yu fullname: Yu, Songding – sequence: 2 givenname: Lei surname: Jiao fullname: Jiao, Lei – sequence: 3 givenname: Jijun surname: Zhao fullname: Zhao, Jijun – sequence: 4 givenname: Lizhao surname: Liu fullname: Liu, Lizhao email: lizhao_liu@dlut.edu.cn |
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| Cites_doi | 10.1021/acs.langmuir.6b03032 10.1103/PhysRevLett.96.176101 10.1038/nphoton.2011.318 10.1016/j.scitotenv.2019.134492 10.1103/PhysRevLett.77.3865 10.1103/PhysRevB.70.212103 10.1016/j.apsusc.2017.01.064 10.1039/c2nr31164j 10.1016/j.cocis.2016.09.001 10.1073/pnas.1605121113 10.1016/j.carbon.2011.12.014 10.1039/D0TC05213B 10.1039/C5CP02986D 10.1103/PhysRevB.59.1758 10.1021/nn404889b 10.1038/ncomms14560 10.1002/adma.201000732 10.1021/la1037926 10.1007/s11467-019-0937-9 10.1016/j.sna.2018.10.036 10.1103/PhysRevB.82.161406 10.1021/acs.jpclett.6b01027 10.1126/science.1162369 10.1063/1.4716024 10.1021/acsami.7b13701 10.1039/C9NR07282A 10.1021/acsami.0c01330 10.1103/PhysRevB.50.17953 10.1038/s41528-021-00100-4 10.1016/j.colsurfb.2010.07.035 10.1016/j.carbon.2012.08.048 10.1016/j.susc.2008.02.025 10.1016/0927-0256(96)00008-0 |
| ContentType | Journal Article |
| Copyright | 2022 |
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| Keywords | Graphene oxide Tensile strain Flexibility Bending modulus |
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| Snippet | •The flexibility of graphene oxide is regulated by strain.•The strained graphene oxide can be more flexible than graphene.•The mechanism of strain softened... Graphene oxide is attractive in flexible materials due to its biocompatibility. Herein, flexibility of graphene oxide under uniaxial tensile strain has been... |
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| SubjectTerms | Bending modulus Flexibility Graphene oxide Tensile strain |
| Title | Strain softened bending modulus of graphene oxide |
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