Ordered macroporous Co3O4-supported Ru nanoparticles: A robust catalyst for efficient hydrodeoxygenation of anisole
A three-dimensional ordered macroporous Co3O4 (OM-Co3O4) supported Ru catalyst was developed for the efficient hydrodeoxygenation (HDO) of anisole. It is revealed that small-sized Ru nanoparticles evenly distributed over the surface of OM-Co3O4 with large quantities of oxygen vacancies could strongl...
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| Published in | Catalysis communications Vol. 153; p. 106302 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
01.05.2021
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| Abstract | A three-dimensional ordered macroporous Co3O4 (OM-Co3O4) supported Ru catalyst was developed for the efficient hydrodeoxygenation (HDO) of anisole. It is revealed that small-sized Ru nanoparticles evenly distributed over the surface of OM-Co3O4 with large quantities of oxygen vacancies could strongly capture Ru0 species, thereby resulting in strong Ru-Co3O4 interactions. Compared with commercial Co3O4 supported Ru catalyst, Ru/OM-Co3O4 displays a better catalytic HDO performance, with a high cyclohexane yield of 92.4% at 250 °C and 0.5 MPa hydrogen pressure after 5 h on stream. Such a significant efficiency of Ru/OM-Co3O4 is mainly attributed to both high dispersion of Ru0 species and an enhanced formation of surface defects, as well as the unique macroporous framework of OM-Co3O4 support.
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•Ordered macroporous Co3O4 supported Ru catalyst was constructed.•Such Ru-based nanocatalyst was highly active for the hydrodeoxygenation of anisole.•Macroporous Co3O4 facilitated the formation of highly dispersed Ru nanoparticles.•Highly dispersion Ru NPs together with surface defects and macroporous framework contributed to high efficiency. |
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| AbstractList | A three-dimensional ordered macroporous Co3O4 (OM-Co3O4) supported Ru catalyst was developed for the efficient hydrodeoxygenation (HDO) of anisole. It is revealed that small-sized Ru nanoparticles evenly distributed over the surface of OM-Co3O4 with large quantities of oxygen vacancies could strongly capture Ru0 species, thereby resulting in strong Ru-Co3O4 interactions. Compared with commercial Co3O4 supported Ru catalyst, Ru/OM-Co3O4 displays a better catalytic HDO performance, with a high cyclohexane yield of 92.4% at 250 °C and 0.5 MPa hydrogen pressure after 5 h on stream. Such a significant efficiency of Ru/OM-Co3O4 is mainly attributed to both high dispersion of Ru0 species and an enhanced formation of surface defects, as well as the unique macroporous framework of OM-Co3O4 support.
[Display omitted]
•Ordered macroporous Co3O4 supported Ru catalyst was constructed.•Such Ru-based nanocatalyst was highly active for the hydrodeoxygenation of anisole.•Macroporous Co3O4 facilitated the formation of highly dispersed Ru nanoparticles.•Highly dispersion Ru NPs together with surface defects and macroporous framework contributed to high efficiency. A three-dimensional ordered macroporous Co3O4 (OM-Co3O4) supported Ru catalyst was developed for the efficient hydrodeoxygenation (HDO) of anisole. It is revealed that small-sized Ru nanoparticles evenly distributed over the surface of OM-Co3O4 with large quantities of oxygen vacancies could strongly capture Ru0 species, thereby resulting in strong Ru-Co3O4 interactions. Compared with commercial Co3O4 supported Ru catalyst, Ru/OM-Co3O4 displays a better catalytic HDO performance, with a high cyclohexane yield of 92.4% at 250 °C and 0.5 MPa hydrogen pressure after 5 h on stream. Such a significant efficiency of Ru/OM-Co3O4 is mainly attributed to both high dispersion of Ru0 species and an enhanced formation of surface defects, as well as the unique macroporous framework of OM-Co3O4 support. |
| ArticleNumber | 106302 |
| Author | Li, Feng Wang, An Yang, Lan Shi, Yisheng Fan, Guoli |
| Author_xml | – sequence: 1 givenname: An surname: Wang fullname: Wang, An – sequence: 2 givenname: Yisheng surname: Shi fullname: Shi, Yisheng – sequence: 3 givenname: Lan surname: Yang fullname: Yang, Lan email: yanglan@mail.buct.edu.cn – sequence: 4 givenname: Guoli surname: Fan fullname: Fan, Guoli – sequence: 5 givenname: Feng surname: Li fullname: Li, Feng email: lifeng@mail.buct.edu.cn |
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| CitedBy_id | crossref_primary_10_1016_j_cjche_2022_07_009 crossref_primary_10_1016_j_fuel_2021_123060 crossref_primary_10_1016_j_fuel_2023_128084 crossref_primary_10_1016_j_cclet_2022_108085 crossref_primary_10_1016_j_jhazmat_2022_130058 crossref_primary_10_3390_catal12121625 crossref_primary_10_1016_j_rser_2023_113700 crossref_primary_10_1039_D1GC04592J |
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| Keywords | Defective structure Hydrodeoxygenation Biomass conversion Ordered macroporous Co3O4 Highly dispersed Ru species |
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| Snippet | A three-dimensional ordered macroporous Co3O4 (OM-Co3O4) supported Ru catalyst was developed for the efficient hydrodeoxygenation (HDO) of anisole. It is... |
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| SubjectTerms | Biomass conversion Defective structure Highly dispersed Ru species Hydrodeoxygenation Ordered macroporous Co3O4 |
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| Title | Ordered macroporous Co3O4-supported Ru nanoparticles: A robust catalyst for efficient hydrodeoxygenation of anisole |
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