Porous Co3O4 nanofibers surface-modified by reduced graphene oxide as a durable, high-rate anode for lithium ion battery

[Display omitted] Here we report our findings in synthesis and characterization of porous Co3O4 nanofibers coated with a surface-modification layer, reduced graphene oxide. The unique porous Co3O4@rGO architecture enables efficient stress relaxation and fast Li+ ions and electron transport during di...

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Published inElectrochimica acta Vol. 228; pp. 241 - 250
Main Authors Hu, Renzong, Zhang, Houpo, Bu, Yunfei, Zhang, Hanyin, Zhao, Bote, Yang, Chenghao
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 20.02.2017
Subjects
Cobalt oxides
conversion reaction
Full cell performance
Lithium ion batteries
Reduced graphene oxide
Lithium ion batteries
Full cell performance
Cobalt oxides
Reduced graphene oxide
conversion reaction
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Abstract [Display omitted] Here we report our findings in synthesis and characterization of porous Co3O4 nanofibers coated with a surface-modification layer, reduced graphene oxide. The unique porous Co3O4@rGO architecture enables efficient stress relaxation and fast Li+ ions and electron transport during discharge/charge cycling. When tested in a half cell, the Co3O4@rGO electrodes display high Coulombic efficiency, enhanced cyclic stability, and high rate capability (∼900mAh/g at 1A/g, and ∼600mAh/g at 5A/g). The high capacity is contributed by a stable capacity yielded from reversible conversion reactions above 0.8V vs. Li/Li+, and a increasing capacity induced by the electrolyte decomposition and interfacial storage between 0.8 0.01V during discahrge. A full cell constructed from a Co3O4@rGO anode and a LiMn2O4 cathode delivers good capacity retention with operation voltage of ∼2.0V. These performances are better than those of other full cells using alloy or metal oxide anodes. Our work is a preliminary attempt for practicality of high capacity metal oxide anodes in Li-ion batteries used for the electronic devices.
AbstractList [Display omitted] Here we report our findings in synthesis and characterization of porous Co3O4 nanofibers coated with a surface-modification layer, reduced graphene oxide. The unique porous Co3O4@rGO architecture enables efficient stress relaxation and fast Li+ ions and electron transport during discharge/charge cycling. When tested in a half cell, the Co3O4@rGO electrodes display high Coulombic efficiency, enhanced cyclic stability, and high rate capability (∼900mAh/g at 1A/g, and ∼600mAh/g at 5A/g). The high capacity is contributed by a stable capacity yielded from reversible conversion reactions above 0.8V vs. Li/Li+, and a increasing capacity induced by the electrolyte decomposition and interfacial storage between 0.8 0.01V during discahrge. A full cell constructed from a Co3O4@rGO anode and a LiMn2O4 cathode delivers good capacity retention with operation voltage of ∼2.0V. These performances are better than those of other full cells using alloy or metal oxide anodes. Our work is a preliminary attempt for practicality of high capacity metal oxide anodes in Li-ion batteries used for the electronic devices.
Author Zhao, Bote
Hu, Renzong
Bu, Yunfei
Zhang, Houpo
Zhang, Hanyin
Yang, Chenghao
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  organization: School of Environment and Energy, South China University of Technology, Guangzhou, 510006, China
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Full cell performance
Cobalt oxides
Reduced graphene oxide
conversion reaction
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Snippet [Display omitted] Here we report our findings in synthesis and characterization of porous Co3O4 nanofibers coated with a surface-modification layer, reduced...
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SubjectTerms Cobalt oxides
conversion reaction
Full cell performance
Lithium ion batteries
Reduced graphene oxide
Title Porous Co3O4 nanofibers surface-modified by reduced graphene oxide as a durable, high-rate anode for lithium ion battery
URI https://dx.doi.org/10.1016/j.electacta.2017.01.067
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