Polymer based thermoelectric nanocomposite materials and devices: Fabrication and characteristics

Organic thermoelectric (TE) materials capitalize on advantages such as low thermal conductivity, low-cost, eco-friendly, versatile processability, light-weight, mechanical flexibility, roll-to-roll production, which are advantageous for the development of portable and wearable self-powered electroni...

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Published inNano energy Vol. 78; p. 105186
Main Authors Nandihalli, Nagaraj, Liu, Chia-Jyi, Mori, Takao
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.12.2020
Subjects
Carbon nanotube
Conjugated polymer
Graphene
Hybrid material
Thermoelectric
Thermoelectric generator
Carbon nanotube
Conjugated polymer
Thermoelectric
Thermoelectric generator
Graphene
Hybrid material
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Abstract Organic thermoelectric (TE) materials capitalize on advantages such as low thermal conductivity, low-cost, eco-friendly, versatile processability, light-weight, mechanical flexibility, roll-to-roll production, which are advantageous for the development of portable and wearable self-powered electronics. On the negative side, the figure-of-merit of polymer TE materials is low, mainly owing to typical low electrical conductivity. Various efforts have been made to enhance the TE performance of organic TE materials, i.e. chemical or electrochemical doping, modification of molecular structure, and fabrication of polymer-based composites or blends, which is the simplest and most cost-effective method for modifying polymer properties. Solution-processed polymer/inorganic or organic hybrids pave the way for formulation of functional TE inks/paste which can be used to fabricate large scale cost-effective manufacturing of TE generators. In this review, we briefly summarize the TE properties of conjugated polymers, and focus on recent developments in polymer/carbon nanofillers (e.g. CNT, graphene, GO) composites and polymer/inorganic TE nanoparticles composites along with preparation methods and thermoelectric performance. Finally, we cover recent advances in the development of functional TE inks, processing techniques, and their usage in device fabrication using various printing techniques and review device output characteristics. [Display omitted] •Covers hot topic of thermoelectric materials & devices, suitable for energy harvesting to power IoT sensors and devices.•Review & analysis on advances on enhanced thermoelectric properties of polymer based nanocomposites (CNT, graphene, NP, NW).•Analyzing effect of composite processing mechanisms, and also interchain and cross-domain transport on properties.•Recent progress in the fabrication methods of a variety of functional nanocomposite inks/pastes for different printers.•Analysis of recent nanocomposites TE devices and their output characteristics in dual-mode or single-mode operation.
AbstractList Organic thermoelectric (TE) materials capitalize on advantages such as low thermal conductivity, low-cost, eco-friendly, versatile processability, light-weight, mechanical flexibility, roll-to-roll production, which are advantageous for the development of portable and wearable self-powered electronics. On the negative side, the figure-of-merit of polymer TE materials is low, mainly owing to typical low electrical conductivity. Various efforts have been made to enhance the TE performance of organic TE materials, i.e. chemical or electrochemical doping, modification of molecular structure, and fabrication of polymer-based composites or blends, which is the simplest and most cost-effective method for modifying polymer properties. Solution-processed polymer/inorganic or organic hybrids pave the way for formulation of functional TE inks/paste which can be used to fabricate large scale cost-effective manufacturing of TE generators. In this review, we briefly summarize the TE properties of conjugated polymers, and focus on recent developments in polymer/carbon nanofillers (e.g. CNT, graphene, GO) composites and polymer/inorganic TE nanoparticles composites along with preparation methods and thermoelectric performance. Finally, we cover recent advances in the development of functional TE inks, processing techniques, and their usage in device fabrication using various printing techniques and review device output characteristics. [Display omitted] •Covers hot topic of thermoelectric materials & devices, suitable for energy harvesting to power IoT sensors and devices.•Review & analysis on advances on enhanced thermoelectric properties of polymer based nanocomposites (CNT, graphene, NP, NW).•Analyzing effect of composite processing mechanisms, and also interchain and cross-domain transport on properties.•Recent progress in the fabrication methods of a variety of functional nanocomposite inks/pastes for different printers.•Analysis of recent nanocomposites TE devices and their output characteristics in dual-mode or single-mode operation.
ArticleNumber 105186
Author Mori, Takao
Liu, Chia-Jyi
Nandihalli, Nagaraj
Author_xml – sequence: 1
  givenname: Nagaraj
  surname: Nandihalli
  fullname: Nandihalli, Nagaraj
  email: nnandiha@uwaterloo.ca
  organization: Department of Physics, National Changhua University of Education, Changhua, 500, Taiwan
– sequence: 2
  givenname: Chia-Jyi
  surname: Liu
  fullname: Liu, Chia-Jyi
  organization: Department of Physics, National Changhua University of Education, Changhua, 500, Taiwan
– sequence: 3
  givenname: Takao
  surname: Mori
  fullname: Mori, Takao
  email: mori.takao@nims.go.jp
  organization: National Institute for Materials Science (NIMS), International Center for Materials Nanoarchitectonics (WPI-MANA), Namiki 1-1, Tsukuba, 305-0044, Japan
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Snippet Organic thermoelectric (TE) materials capitalize on advantages such as low thermal conductivity, low-cost, eco-friendly, versatile processability,...
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StartPage 105186
SubjectTerms Carbon nanotube
Conjugated polymer
Graphene
Hybrid material
Thermoelectric
Thermoelectric generator
Title Polymer based thermoelectric nanocomposite materials and devices: Fabrication and characteristics
URI https://dx.doi.org/10.1016/j.nanoen.2020.105186
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