A generalized approach for iron catalyzed chemo- and regioselective formation of anti-Markovnikov acetals from styrene derivatives
Fe(BF4)(2)center dot 6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions.
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| Published in | Chemical communications (Cambridge, England) Vol. 48; no. 28; pp. 3448 - 3450 |
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| Main Authors | , |
| Format | Journal Article |
| Language | English |
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Royal Soc Chemistry
01.01.2012
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| Abstract | Fe(BF4)(2)center dot 6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions. |
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| AbstractList | Fe(BF sub(4)) sub(2).6H sub(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc) sub(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions. Fe(BF4)(2)center dot 6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions. Fe(BF₄)₂·6H₂O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)₂ can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions. Fe(BF(4))(2)·6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions.Fe(BF(4))(2)·6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions. Fe(BF(4))(2)·6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals from styrene derivatives with anti-Markovnikov regioselectivity in good to high yields under mild and benign reaction conditions. |
| Author | Dutta Chowdhury, Abhishek Kumar Lahiri, Goutam |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/22358109$$D View this record in MEDLINE/PubMed |
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| Cites_doi | 10.1039/c39830000848 10.1021/ol053110p 10.1021/jo00114a055 10.1016/S0040-4039(98)00371-2 10.1021/jo00385a021 10.1021/jo052192s 10.1021/jo0258249 10.1021/ar00170a006 10.1021/ja2061038 10.1016/j.tetlet.2004.04.126 10.1002/anie.200800012 10.1021/jo025701o 10.1021/ja808893g 10.1039/c1cc13574k 10.1039/B207328E 10.1002/anie.200460545 10.1021/ja0377899 10.1016/j.biortech.2010.02.101 10.1039/b207328e |
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| Keywords | ALKENES KETONES COMPLEX ELECTRON-WITHDRAWING SUBSTITUENTS CONVERSION PALLADIUM(II)-CATALYZED ACETALIZATION ISOMERIZATION ALDEHYDES |
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| Snippet | Fe(BF4)(2)center dot 6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl... Fe(BF(4))(2)·6H(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)(2) can efficiently catalyze the formation of chemoselective dialkyl acetals... Fe(BF sub(4)) sub(2).6H sub(2)O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc) sub(2) can efficiently catalyze the formation of chemoselective... Fe(BF₄)₂·6H₂O in the presence of pyridine-2,6-dicarboxylic acid and PhI(OAc)₂ can efficiently catalyze the formation of chemoselective dialkyl acetals from... |
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| SubjectTerms | Acetals catalytic activity chemical communication chemical reactions Chemistry Chemistry, Multidisciplinary chemoselectivity Derivatives dicarboxylic acids Iron Physical Sciences regioselectivity Science & Technology styrene Styrenes |
| Title | A generalized approach for iron catalyzed chemo- and regioselective formation of anti-Markovnikov acetals from styrene derivatives |
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