Recent advances in transition-metal-sulfide-based bifunctional electrocatalysts for overall water splitting
Hydrogen produced via water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency, solving the problems of conventional fossil fuel exhaustion and environmental contamination. Transition metal sulfides (TMS) have been extens...
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| Published in | Journal of materials chemistry. A, Materials for energy and sustainability Vol. 9; no. 9; pp. 532 - 5363 |
|---|---|
| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
09.03.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Hydrogen produced
via
water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency, solving the problems of conventional fossil fuel exhaustion and environmental contamination. Transition metal sulfides (TMS) have been extensively explored as effective, widely available alternatives to precious metals in overall water splitting. Herein, recent advances, covering preparation methods, intrinsic electrocatalytic performance, and optimization strategies, relating to TMS-based bifunctional electrocatalysts have been summarized systematically and comprehensively. Firstly, a general introduction to the reaction mechanisms and key parameters of the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is provided. Next, the physicochemical properties of TMS and typical synthesis methods are introduced to give guidance for fabricating TMS materials with well-defined structures, controllable compositions, and excellent performance. Importantly, the intrinsic activities of TMS-based electrocatalysts and several strategies for improving their bifunctional electrocatalytic performance during water electrolysis are discussed in detail. Finally, perspectives covering the challenges and opportunities related to the further development of TMS-based materials with high activity and long-term durability for overall water splitting are given. The aim herein is to provide guidelines for the design and fabrication of TMS-based bifunctional electrocatalysts with excellent performance and to accelerate their large-scale practical application in water electrolysis.
This review summarizes recent advances relating to transition metal sulfide (TMS)-based bifunctional electrocatalysts, providing guidelines for the design and fabrication of TMS-based catalysts for practical application in water electrolysis. |
|---|---|
| AbstractList | Hydrogen produced via water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency, solving the problems of conventional fossil fuel exhaustion and environmental contamination. Transition metal sulfides (TMS) have been extensively explored as effective, widely available alternatives to precious metals in overall water splitting. Herein, recent advances, covering preparation methods, intrinsic electrocatalytic performance, and optimization strategies, relating to TMS-based bifunctional electrocatalysts have been summarized systematically and comprehensively. Firstly, a general introduction to the reaction mechanisms and key parameters of the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is provided. Next, the physicochemical properties of TMS and typical synthesis methods are introduced to give guidance for fabricating TMS materials with well-defined structures, controllable compositions, and excellent performance. Importantly, the intrinsic activities of TMS-based electrocatalysts and several strategies for improving their bifunctional electrocatalytic performance during water electrolysis are discussed in detail. Finally, perspectives covering the challenges and opportunities related to the further development of TMS-based materials with high activity and long-term durability for overall water splitting are given. The aim herein is to provide guidelines for the design and fabrication of TMS-based bifunctional electrocatalysts with excellent performance and to accelerate their large-scale practical application in water electrolysis. Hydrogen produced via water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency, solving the problems of conventional fossil fuel exhaustion and environmental contamination. Transition metal sulfides (TMS) have been extensively explored as effective, widely available alternatives to precious metals in overall water splitting. Herein, recent advances, covering preparation methods, intrinsic electrocatalytic performance, and optimization strategies, relating to TMS-based bifunctional electrocatalysts have been summarized systematically and comprehensively. Firstly, a general introduction to the reaction mechanisms and key parameters of the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is provided. Next, the physicochemical properties of TMS and typical synthesis methods are introduced to give guidance for fabricating TMS materials with well-defined structures, controllable compositions, and excellent performance. Importantly, the intrinsic activities of TMS-based electrocatalysts and several strategies for improving their bifunctional electrocatalytic performance during water electrolysis are discussed in detail. Finally, perspectives covering the challenges and opportunities related to the further development of TMS-based materials with high activity and long-term durability for overall water splitting are given. The aim herein is to provide guidelines for the design and fabrication of TMS-based bifunctional electrocatalysts with excellent performance and to accelerate their large-scale practical application in water electrolysis. Hydrogen produced via water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency, solving the problems of conventional fossil fuel exhaustion and environmental contamination. Transition metal sulfides (TMS) have been extensively explored as effective, widely available alternatives to precious metals in overall water splitting. Herein, recent advances, covering preparation methods, intrinsic electrocatalytic performance, and optimization strategies, relating to TMS-based bifunctional electrocatalysts have been summarized systematically and comprehensively. Firstly, a general introduction to the reaction mechanisms and key parameters of the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is provided. Next, the physicochemical properties of TMS and typical synthesis methods are introduced to give guidance for fabricating TMS materials with well-defined structures, controllable compositions, and excellent performance. Importantly, the intrinsic activities of TMS-based electrocatalysts and several strategies for improving their bifunctional electrocatalytic performance during water electrolysis are discussed in detail. Finally, perspectives covering the challenges and opportunities related to the further development of TMS-based materials with high activity and long-term durability for overall water splitting are given. The aim herein is to provide guidelines for the design and fabrication of TMS-based bifunctional electrocatalysts with excellent performance and to accelerate their large-scale practical application in water electrolysis. This review summarizes recent advances relating to transition metal sulfide (TMS)-based bifunctional electrocatalysts, providing guidelines for the design and fabrication of TMS-based catalysts for practical application in water electrolysis. |
| Author | Wang, Min He, Yijia Zhang, Li Zhu, Hongwei |
| AuthorAffiliation | Key Laboratory of Photochemical Conversion and Optoelectronic Materials Chinese Academy of Sciences China Ship Information Center School of Materials Science and Engineering Tsinghua University State Key Lab of New Ceramics and Fine Processing Technical Institute of Physics and Chemistry |
| AuthorAffiliation_xml | – name: Key Laboratory of Photochemical Conversion and Optoelectronic Materials – name: China Ship Information Center – name: Technical Institute of Physics and Chemistry – name: Chinese Academy of Sciences – name: State Key Lab of New Ceramics and Fine Processing – name: School of Materials Science and Engineering – name: Tsinghua University |
| Author_xml | – sequence: 1 givenname: Min surname: Wang fullname: Wang, Min – sequence: 2 givenname: Li surname: Zhang fullname: Zhang, Li – sequence: 3 givenname: Yijia surname: He fullname: He, Yijia – sequence: 4 givenname: Hongwei surname: Zhu fullname: Zhu, Hongwei |
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| Notes | Min Wang is a PhD candidate at the School of Materials Science and Engineering, Tsinghua University, China. She received her B.S. degree in Materials Science and Engineering from Jilin University in 2016. Her research focuses on advanced nanomaterials related to electrocatalysis for energy conversion. Hongwei Zhu is a Professor at the School of Materials Science and Engineering, Tsinghua University, China. He received his B.S. degree in Mechanical Engineering (1998) and his PhD degree in Materials Processing Engineering (2003) from Tsinghua University. After postdoctoral studies in Japan and the USA, he began his independent career as a faculty member at Tsinghua University (2008 to present). His current research interests involve low-dimensional materials and materials informatics. ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 content type line 23 |
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| PublicationTitle | Journal of materials chemistry. A, Materials for energy and sustainability |
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| Snippet | Hydrogen produced
via
water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency,... Hydrogen produced via water electrolysis can act as an ideal clean chemical fuel with superb gravimetric energy density and high energy conversion efficiency,... |
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| SubjectTerms | Chemical fuels Clean energy Contamination durability Electrocatalysts Electrolysis Energy conversion Energy conversion efficiency energy density Fabrication Flux density Fossil fuels Gravimetry hydrogen Hydrogen evolution reactions hydrogen production Metal sulfides Metals Optimization Oxygen evolution reactions oxygen production Physicochemical properties pollution Reaction mechanisms Splitting Sulfides Transition metals Water splitting |
| Title | Recent advances in transition-metal-sulfide-based bifunctional electrocatalysts for overall water splitting |
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