Na[FSA]-[C3C1pyrr][FSA] ionic liquids as electrolytes for sodium secondary batteries: Effects of Na ion concentration and operation temperature

As electrolytes for sodium secondary batteries operating over a wide temperature range, Na[FSA]-[C sub(3)C sub(1)pyrr][FSA] (FSA = bis(fluorosulfonyl)amide, C sub(3)C sub(1)pyrr = N-methyl-N-propylpyrrolidinium) ionic liquids have been investigated. The effects of Na ion concentration (0-60 mol% Na[...

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Published in	Journal of power sources Vol. 269; pp. 124 - 128
Main Authors	Ding, Changsheng, Nohira, Toshiyuki, Hagiwara, Rika, Matsumoto, Kazuhiko, Okamoto, Yu, Fukunaga, Atsushi, Sakai, Shoichiro, Nitta, Koji, Inazawa, Shinji
Format	Journal Article
Language	English
Published	Amsterdam Elsevier 10.12.2014
Subjects	Applied sciences Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Electrolytes Electrolytic cells Exact sciences and technology Ion concentration Ionic conductivity Ionic liquids Optimization Sodium Storage batteries Viscosity Temperature Sodium-ion battery Electrical properties Sodium secondary batteries Na ion concentration Operation temperature Ionic conductivity Ions Secondary cell Concentration Ionic liquid Electrolyte Ionic liquids Rheological properties
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Abstract	As electrolytes for sodium secondary batteries operating over a wide temperature range, Na[FSA]-[C sub(3)C sub(1)pyrr][FSA] (FSA = bis(fluorosulfonyl)amide, C sub(3)C sub(1)pyrr = N-methyl-N-propylpyrrolidinium) ionic liquids have been investigated. The effects of Na ion concentration (0-60 mol% Na[FSA]) and operation temperature (253-363 K) on the viscosity and ionic conductivity and charge-discharge performance of Na/Na[FSA]-[C sub(3)C sub(1)pyrr] [FSA]/NaCrO sub(2) cells are studied. Results show that Na ion concentration strongly affects the rate capability of the cells, and that the best rate capability at 363 K is obtained at 40 mol% Na [FSA]. The operation temperature also significantly influences the charge-discharge performance, especially at low temperatures. At operation temperatures below 273 K, 25 mol% Na[FSA] is found to be the optimum Na ion concentration. There exist different optimum ranges of Na ion concentration depending on the operation temperatures.
AbstractList	As electrolytes for sodium secondary batteries operating over a wide temperature range, Na[FSA]-[C sub(3)C sub(1)pyrr][FSA] (FSA = bis(fluorosulfonyl)amide, C sub(3)C sub(1)pyrr = N-methyl-N-propylpyrrolidinium) ionic liquids have been investigated. The effects of Na ion concentration (0-60 mol% Na[FSA]) and operation temperature (253-363 K) on the viscosity and ionic conductivity and charge-discharge performance of Na/Na[FSA]-[C sub(3)C sub(1)pyrr] [FSA]/NaCrO sub(2) cells are studied. Results show that Na ion concentration strongly affects the rate capability of the cells, and that the best rate capability at 363 K is obtained at 40 mol% Na [FSA]. The operation temperature also significantly influences the charge-discharge performance, especially at low temperatures. At operation temperatures below 273 K, 25 mol% Na[FSA] is found to be the optimum Na ion concentration. There exist different optimum ranges of Na ion concentration depending on the operation temperatures.
Author	Nohira, Toshiyuki Hagiwara, Rika Sakai, Shoichiro Inazawa, Shinji Ding, Changsheng Okamoto, Yu Fukunaga, Atsushi Nitta, Koji Matsumoto, Kazuhiko
Author_xml	– sequence: 1 givenname: Changsheng surname: Ding fullname: Ding, Changsheng – sequence: 2 givenname: Toshiyuki surname: Nohira fullname: Nohira, Toshiyuki – sequence: 3 givenname: Rika surname: Hagiwara fullname: Hagiwara, Rika – sequence: 4 givenname: Kazuhiko surname: Matsumoto fullname: Matsumoto, Kazuhiko – sequence: 5 givenname: Yu surname: Okamoto fullname: Okamoto, Yu – sequence: 6 givenname: Atsushi surname: Fukunaga fullname: Fukunaga, Atsushi – sequence: 7 givenname: Shoichiro surname: Sakai fullname: Sakai, Shoichiro – sequence: 8 givenname: Koji surname: Nitta fullname: Nitta, Koji – sequence: 9 givenname: Shinji surname: Inazawa fullname: Inazawa, Shinji
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Keywords	Viscosity Temperature Sodium-ion battery Electrical properties Sodium secondary batteries Na ion concentration Operation temperature Ionic conductivity Ions Secondary cell Concentration Ionic liquid Electrolyte Ionic liquids Rheological properties
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Snippet	As electrolytes for sodium secondary batteries operating over a wide temperature range, Na[FSA]-[C sub(3)C sub(1)pyrr][FSA] (FSA = bis(fluorosulfonyl)amide, C...
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SubjectTerms	Applied sciences Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Electrolytes Electrolytic cells Exact sciences and technology Ion concentration Ionic conductivity Ionic liquids Optimization Sodium Storage batteries
Title	Na[FSA]-[C3C1pyrr][FSA] ionic liquids as electrolytes for sodium secondary batteries: Effects of Na ion concentration and operation temperature
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