Van der Waals engineering of ferromagnetic semiconductor heterostructures for spin and valleytronics
A van der Waals heterostructure of monolayer WSe 2 and ferromagnetic CrI 3 enables exceptional control of valley pseudospin. The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration...
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| Published in | Science advances Vol. 3; no. 5; p. e1603113 |
|---|---|
| Main Authors | , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
AAAS
01.05.2017
American Association for the Advancement of Science |
| Subjects | |
| Online Access | Get full text |
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| Abstract | A van der Waals heterostructure of monolayer WSe
2
and ferromagnetic CrI
3
enables exceptional control of valley pseudospin.
The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI
3
and a monolayer of WSe
2
. We observe unprecedented control of the spin and valley pseudospin in WSe
2
, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe
2
valley splitting and polarization via flipping of the CrI
3
magnetization. The WSe
2
photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe
2
and the CrI
3
magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure. |
|---|---|
| AbstractList | The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI
and a monolayer of WSe
. We observe unprecedented control of the spin and valley pseudospin in WSe
, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe
valley splitting and polarization via flipping of the CrI
magnetization. The WSe
photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe
and the CrI
magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure. A van der Waals heterostructure of monolayer WSe 2 and ferromagnetic CrI 3 enables exceptional control of valley pseudospin. The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI 3 and a monolayer of WSe 2 . We observe unprecedented control of the spin and valley pseudospin in WSe 2 , where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe 2 valley splitting and polarization via flipping of the CrI 3 magnetization. The WSe 2 photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe 2 and the CrI 3 magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure. The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI3 and a monolayer of WSe2. We observe unprecedented control of the spin and valley pseudospin in WSe2, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe2 valley splitting and polarization via flipping of the CrI3 magnetization. The WSe2 photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe2 and the CrI3 magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure. The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI3 and a monolayer of WSe2. We observe unprecedented control of the spin and valley pseudospin in WSe2, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe2 valley splitting and polarization via flipping of the CrI3 magnetization. The WSe2 photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe2 and the CrI3 magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure.The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the seamless integration of information processing and storage. We create van der Waals heterostructures formed by an ultrathin ferromagnetic semiconductor CrI3 and a monolayer of WSe2. We observe unprecedented control of the spin and valley pseudospin in WSe2, where we detect a large magnetic exchange field of nearly 13 T and rapid switching of the WSe2 valley splitting and polarization via flipping of the CrI3 magnetization. The WSe2 photoluminescence intensity strongly depends on the relative alignment between photoexcited spins in WSe2 and the CrI3 magnetization, because of ultrafast spin-dependent charge hopping across the heterostructure interface. The photoluminescence detection of valley pseudospin provides a simple and sensitive method to probe the intriguing domain dynamics in the ultrathin magnet, as well as the rich spin interactions within the heterostructure. |
| Author | Sivadas, Nikhil Taniguchi, Takashi Fu, Kai-Mei C. Zhong, Ding Yao, Wang Linpeng, Xiayu Xiao, Di Schmidgall, Emma Huang, Bevin Cheng, Ran Watanabe, Kenji Seyler, Kyle L. McGuire, Michael A. Xu, Xiaodong |
| Author_xml | – sequence: 1 givenname: Ding orcidid: 0000-0003-3149-2071 surname: Zhong fullname: Zhong, Ding organization: Department of Physics, University of Washington, Seattle, WA 98195, USA – sequence: 2 givenname: Kyle L. surname: Seyler fullname: Seyler, Kyle L. organization: Department of Physics, University of Washington, Seattle, WA 98195, USA – sequence: 3 givenname: Xiayu surname: Linpeng fullname: Linpeng, Xiayu organization: Department of Physics, University of Washington, Seattle, WA 98195, USA – sequence: 4 givenname: Ran orcidid: 0000-0003-0166-2172 surname: Cheng fullname: Cheng, Ran organization: Department of Physics, Carnegie Mellon University, Pittsburg, PA 15213, USA – sequence: 5 givenname: Nikhil surname: Sivadas fullname: Sivadas, Nikhil organization: Department of Physics, Carnegie Mellon University, Pittsburg, PA 15213, USA – sequence: 6 givenname: Bevin surname: Huang fullname: Huang, Bevin organization: Department of Physics, University of Washington, Seattle, WA 98195, USA – sequence: 7 givenname: Emma orcidid: 0000-0001-6809-1808 surname: Schmidgall fullname: Schmidgall, Emma organization: Department of Physics, University of Washington, Seattle, WA 98195, USA – sequence: 8 givenname: Takashi surname: Taniguchi fullname: Taniguchi, Takashi organization: National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan – sequence: 9 givenname: Kenji orcidid: 0000-0003-3701-8119 surname: Watanabe fullname: Watanabe, Kenji organization: National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan – sequence: 10 givenname: Michael A. surname: McGuire fullname: McGuire, Michael A. organization: Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA – sequence: 11 givenname: Wang orcidid: 0000-0003-2883-4528 surname: Yao fullname: Yao, Wang organization: Department of Physics and Center of Theoretical and Computational Physics, University of Hong Kong, Hong Kong, China – sequence: 12 givenname: Di surname: Xiao fullname: Xiao, Di organization: Department of Physics, Carnegie Mellon University, Pittsburg, PA 15213, USA – sequence: 13 givenname: Kai-Mei C. surname: Fu fullname: Fu, Kai-Mei C. organization: Department of Physics, University of Washington, Seattle, WA 98195, USA., Department of Electrical Engineering, University of Washington, Seattle, WA 98195, USA – sequence: 14 givenname: Xiaodong surname: Xu fullname: Xu, Xiaodong organization: Department of Physics, University of Washington, Seattle, WA 98195, USA., Department of Materials Science and Engineering, University of Washington, Seattle, WA 98195, USA |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/28580423$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1376521$$D View this record in Osti.gov |
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| Keywords | magnetic proximity effect van der Waals heterostructure Exchange interaction 2D materials ultrafast charge transfer Valleytronics ferromagnetic semiconductor monolayer semiconductor Spintronics |
| Language | English |
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| Snippet | A van der Waals heterostructure of monolayer WSe
2
and ferromagnetic CrI
3
enables exceptional control of valley pseudospin.
The integration of magnetic... The integration of magnetic material with semiconductors has been fertile ground for fundamental science as well as of great practical interest toward the... |
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| Title | Van der Waals engineering of ferromagnetic semiconductor heterostructures for spin and valleytronics |
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