Structural characterizations of organic-based materials with extensive mechanoluminescence properties
The organic mechanoluminescent (ML) material europium-doped dibenzoylmethide triethylammonium (EuD4TEA) is known as a triboluminescent material. Our group has synthesized a novel ML material with the addition of 1-ethenylpyrrolidin-2-one [(polyvinylpyrrolidone) (PVP)], which changed the ligand of th...
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| Published in | Journal of luminescence Vol. 190; pp. 413 - 423 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
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Elsevier B.V
01.10.2017
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| Abstract | The organic mechanoluminescent (ML) material europium-doped dibenzoylmethide triethylammonium (EuD4TEA) is known as a triboluminescent material. Our group has synthesized a novel ML material with the addition of 1-ethenylpyrrolidin-2-one [(polyvinylpyrrolidone) (PVP)], which changed the ligand of the mechanoluminescent material. This research investigated the ML material structure, molecular orbital electron distributions of the ligands, ML mechanism and enhancement in the photoluminescence (PL) intensity with PVP. For the first time, the ML material structure was characterized using nuclear magnetic resonance spectroscopy (NMR), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and Gaussian DFT/B3LYP/6–31G(d,p) software. The ML properties were characterized using a Hamamatsu Photonic Multichannel Analyzer (PMA). The material can be applied to the real-time visualization of the stress field near the tip of a crack, an ML light source, determination of laser and ultrasonic powers, secret message writing and earthquake detection sensors. |
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| AbstractList | The organic mechanoluminescent (ML) material europium-doped dibenzoylmethide triethylammonium (EuD4TEA) is known as a triboluminescent material. Our group has synthesized a novel ML material with the addition of 1-ethenylpyrrolidin-2-one [(polyvinylpyrrolidone) (PVP)], which changed the ligand of the mechanoluminescent material. This research investigated the ML material structure, molecular orbital electron distributions of the ligands, ML mechanism and enhancement in the photoluminescence (PL) intensity with PVP. For the first time, the ML material structure was characterized using nuclear magnetic resonance spectroscopy (NMR), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS) and Gaussian DFT/B3LYP/6–31G(d,p) software. The ML properties were characterized using a Hamamatsu Photonic Multichannel Analyzer (PMA). The material can be applied to the real-time visualization of the stress field near the tip of a crack, an ML light source, determination of laser and ultrasonic powers, secret message writing and earthquake detection sensors. |
| Author | Okuya, Masayuki Shimomura, Masaru Murakami, Kenji Ranasinghe, R.A.D.M. Tanaka, Yasutaka |
| Author_xml | – sequence: 1 givenname: R.A.D.M. surname: Ranasinghe fullname: Ranasinghe, R.A.D.M. organization: Graduate School of Science and Technology, Shizuoka University, Japan – sequence: 2 givenname: Yasutaka surname: Tanaka fullname: Tanaka, Yasutaka organization: Graduate School of Integrated Science and Technology, Shizuoka University, Japan – sequence: 3 givenname: Masayuki surname: Okuya fullname: Okuya, Masayuki organization: Graduate School of Integrated Science and Technology, Shizuoka University, Japan – sequence: 4 givenname: Masaru surname: Shimomura fullname: Shimomura, Masaru organization: Graduate School of Integrated Science and Technology, Shizuoka University, Japan – sequence: 5 givenname: Kenji surname: Murakami fullname: Murakami, Kenji email: murakami.kenji@shizuoka.ac.jp organization: Graduate School of Integrated Science and Technology, Shizuoka University, Japan |
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| Keywords | Structure Polyvinylpyrrolidone Organic polymer-based mechanoluminescence |
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| Snippet | The organic mechanoluminescent (ML) material europium-doped dibenzoylmethide triethylammonium (EuD4TEA) is known as a triboluminescent material. Our group has... |
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| SubjectTerms | Organic polymer-based mechanoluminescence Polyvinylpyrrolidone Structure |
| Title | Structural characterizations of organic-based materials with extensive mechanoluminescence properties |
| URI | https://dx.doi.org/10.1016/j.jlumin.2017.05.073 |
| Volume | 190 |
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