TADF‐Type Organic Afterglow
We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing (kRISC) to simultaneously improve afterglow quantum yields and maintain afterglow emission li...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 31; pp. 17138 - 17147 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
26.07.2021
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing (kRISC) to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. Difluoroboron β‐diketonate (BF2bdk) compounds are designed with multiple electron‐donating groups to possess moderate kRISC values and are selected as luminescent dopants. The matrices with carbonyl functional groups such as phenyl benzoate (PhB) have been found to interact with and perturb BF2bdk excited states by dipole–dipole interactions and thus enhance the intersystem crossing of BF2bdk excited states. Through dopant‐matrix collaboration, the efficient TADF‐type afterglow materials have been achieved to exhibit excellent processability into desired shapes and large‐area films by melt casting, as well as aqueous afterglow dispersions for potential bioimaging applications.
Due to the spin‐forbidden nature, it remains challenging to achieve room‐temperature organic phosphorescence and afterglow materials with high quantum yields. We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. |
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| AbstractList | We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing (kRISC) to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. Difluoroboron β‐diketonate (BF2bdk) compounds are designed with multiple electron‐donating groups to possess moderate kRISC values and are selected as luminescent dopants. The matrices with carbonyl functional groups such as phenyl benzoate (PhB) have been found to interact with and perturb BF2bdk excited states by dipole–dipole interactions and thus enhance the intersystem crossing of BF2bdk excited states. Through dopant‐matrix collaboration, the efficient TADF‐type afterglow materials have been achieved to exhibit excellent processability into desired shapes and large‐area films by melt casting, as well as aqueous afterglow dispersions for potential bioimaging applications. We report a highly efficient dopant-matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60-70 %, which features a moderate rate constant for reverse intersystem crossing (kRISC ) to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. Difluoroboron β-diketonate (BF2 bdk) compounds are designed with multiple electron-donating groups to possess moderate kRISC values and are selected as luminescent dopants. The matrices with carbonyl functional groups such as phenyl benzoate (PhB) have been found to interact with and perturb BF2 bdk excited states by dipole-dipole interactions and thus enhance the intersystem crossing of BF2 bdk excited states. Through dopant-matrix collaboration, the efficient TADF-type afterglow materials have been achieved to exhibit excellent processability into desired shapes and large-area films by melt casting, as well as aqueous afterglow dispersions for potential bioimaging applications.We report a highly efficient dopant-matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60-70 %, which features a moderate rate constant for reverse intersystem crossing (kRISC ) to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. Difluoroboron β-diketonate (BF2 bdk) compounds are designed with multiple electron-donating groups to possess moderate kRISC values and are selected as luminescent dopants. The matrices with carbonyl functional groups such as phenyl benzoate (PhB) have been found to interact with and perturb BF2 bdk excited states by dipole-dipole interactions and thus enhance the intersystem crossing of BF2 bdk excited states. Through dopant-matrix collaboration, the efficient TADF-type afterglow materials have been achieved to exhibit excellent processability into desired shapes and large-area films by melt casting, as well as aqueous afterglow dispersions for potential bioimaging applications. We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing ( k RISC ) to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. Difluoroboron β‐diketonate (BF 2 bdk) compounds are designed with multiple electron‐donating groups to possess moderate k RISC values and are selected as luminescent dopants. The matrices with carbonyl functional groups such as phenyl benzoate (PhB) have been found to interact with and perturb BF 2 bdk excited states by dipole–dipole interactions and thus enhance the intersystem crossing of BF 2 bdk excited states. Through dopant‐matrix collaboration, the efficient TADF‐type afterglow materials have been achieved to exhibit excellent processability into desired shapes and large‐area films by melt casting, as well as aqueous afterglow dispersions for potential bioimaging applications. We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing (kRISC) to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. Difluoroboron β‐diketonate (BF2bdk) compounds are designed with multiple electron‐donating groups to possess moderate kRISC values and are selected as luminescent dopants. The matrices with carbonyl functional groups such as phenyl benzoate (PhB) have been found to interact with and perturb BF2bdk excited states by dipole–dipole interactions and thus enhance the intersystem crossing of BF2bdk excited states. Through dopant‐matrix collaboration, the efficient TADF‐type afterglow materials have been achieved to exhibit excellent processability into desired shapes and large‐area films by melt casting, as well as aqueous afterglow dispersions for potential bioimaging applications. Due to the spin‐forbidden nature, it remains challenging to achieve room‐temperature organic phosphorescence and afterglow materials with high quantum yields. We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate rate constant for reverse intersystem crossing to simultaneously improve afterglow quantum yields and maintain afterglow emission lifetime. |
| Author | Wang, Guangming Li, Xun Zhang, Kaka Sun, Yan Li, Jiuyang Wang, Xuepu |
| Author_xml | – sequence: 1 givenname: Xuepu surname: Wang fullname: Wang, Xuepu organization: Chinese Academy of Sciences – sequence: 2 givenname: Yan surname: Sun fullname: Sun, Yan organization: Chinese Academy of Sciences – sequence: 3 givenname: Guangming surname: Wang fullname: Wang, Guangming organization: Chinese Academy of Sciences – sequence: 4 givenname: Jiuyang surname: Li fullname: Li, Jiuyang organization: Chinese Academy of Sciences – sequence: 5 givenname: Xun surname: Li fullname: Li, Xun organization: Chinese Academy of Sciences – sequence: 6 givenname: Kaka orcidid: 0000-0002-8176-6205 surname: Zhang fullname: Zhang, Kaka email: zhangkaka@sioc.ac.cn organization: Chinese Academy of Sciences |
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| Snippet | We report a highly efficient dopant‐matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60–70 %, which features a moderate... We report a highly efficient dopant-matrix afterglow system enabled by TADF mechanism to realize afterglow quantum yields of 60-70 %, which features a moderate... |
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| SubjectTerms | afterglow Benzoates Benzoic acid Carbonyl compounds Carbonyls Dipole interactions Dopants Excitation Functional groups Medical imaging organic materials phosphorescence thermally activated delayed fluorescence triplet excited state |
| Title | TADF‐Type Organic Afterglow |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fanie.202105628 https://www.proquest.com/docview/2552810511 https://www.proquest.com/docview/2535827758 |
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