Single Atom Ru Monolithic Electrode for Efficient Chlorine Evolution and Nitrate Reduction
Fabricating single‐atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab‐to‐fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand‐free isolated Ru a...
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| Published in | Angewandte Chemie International Edition Vol. 61; no. 41; pp. e202208215 - n/a |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
Wiley Subscription Services, Inc
10.10.2022
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| Edition | International ed. in English |
| Subjects | |
| Online Access | Get full text |
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| Abstract | Fabricating single‐atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab‐to‐fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand‐free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal‐support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher mass activity than that of commercial dimensionally stable anode, and also selectively reduced nitrate to ammonia with an unprecedented ammonia yield rate of 22.2 mol g−1 h−1 at −0.3 V. Furthermore, the Ru single atom monolithic electrode can be scaled up from 2×2 cm to 25×15 cm at least, thus demonstrating great potential for industrial electrocatalytic applications.
We report an inherent oxide anchoring strategy to synthesize monolithic single atom electrodes. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution and nitrate reduction performances. The scalability and bifunctionality of Ru single atom electrode highlight its great potential of electrochemical applications. |
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| AbstractList | Fabricating single‐atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab‐to‐fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand‐free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal‐support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher mass activity than that of commercial dimensionally stable anode, and also selectively reduced nitrate to ammonia with an unprecedented ammonia yield rate of 22.2 mol g
−1
h
−1
at −0.3 V. Furthermore, the Ru single atom monolithic electrode can be scaled up from 2×2 cm to 25×15 cm at least, thus demonstrating great potential for industrial electrocatalytic applications. Fabricating single-atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab-to-fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand-free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal-support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher mass activity than that of commercial dimensionally stable anode, and also selectively reduced nitrate to ammonia with an unprecedented ammonia yield rate of 22.2 mol g-1 h-1 at -0.3 V. Furthermore, the Ru single atom monolithic electrode can be scaled up from 2×2 cm to 25×15 cm at least, thus demonstrating great potential for industrial electrocatalytic applications.Fabricating single-atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab-to-fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand-free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal-support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher mass activity than that of commercial dimensionally stable anode, and also selectively reduced nitrate to ammonia with an unprecedented ammonia yield rate of 22.2 mol g-1 h-1 at -0.3 V. Furthermore, the Ru single atom monolithic electrode can be scaled up from 2×2 cm to 25×15 cm at least, thus demonstrating great potential for industrial electrocatalytic applications. Fabricating single‐atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab‐to‐fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand‐free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal‐support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher mass activity than that of commercial dimensionally stable anode, and also selectively reduced nitrate to ammonia with an unprecedented ammonia yield rate of 22.2 mol g−1 h−1 at −0.3 V. Furthermore, the Ru single atom monolithic electrode can be scaled up from 2×2 cm to 25×15 cm at least, thus demonstrating great potential for industrial electrocatalytic applications. We report an inherent oxide anchoring strategy to synthesize monolithic single atom electrodes. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution and nitrate reduction performances. The scalability and bifunctionality of Ru single atom electrode highlight its great potential of electrochemical applications. Fabricating single‐atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the lab‐to‐fab translation of the electrochemical technologies. Here, we report an inherent oxide anchoring strategy to fasten ligand‐free isolated Ru atoms on the amorphous layer of monolithic Ti support by regulating the electronic metal‐support interactions. The prepared Ru single atom electrode exhibited exceptional electrochemical chlorine evolution activity, three orders of magnitude higher mass activity than that of commercial dimensionally stable anode, and also selectively reduced nitrate to ammonia with an unprecedented ammonia yield rate of 22.2 mol g−1 h−1 at −0.3 V. Furthermore, the Ru single atom monolithic electrode can be scaled up from 2×2 cm to 25×15 cm at least, thus demonstrating great potential for industrial electrocatalytic applications. |
| Author | Wang, Jiaxian Zhang, Lizhi Dai, Jie Hou, Wei Yao, Yancai Zheng, Qian Fang, Chuyang Zhan, Guangming Zhao, Long |
| Author_xml | – sequence: 1 givenname: Yancai surname: Yao fullname: Yao, Yancai organization: Shanghai Jiao Tong University – sequence: 2 givenname: Long surname: Zhao fullname: Zhao, Long organization: Shanghai Jiao Tong University – sequence: 3 givenname: Jie surname: Dai fullname: Dai, Jie organization: Shanghai Jiao Tong University – sequence: 4 givenname: Jiaxian surname: Wang fullname: Wang, Jiaxian organization: Shanghai Jiao Tong University – sequence: 5 givenname: Chuyang surname: Fang fullname: Fang, Chuyang organization: Central China Normal University – sequence: 6 givenname: Guangming surname: Zhan fullname: Zhan, Guangming organization: Central China Normal University – sequence: 7 givenname: Qian surname: Zheng fullname: Zheng, Qian organization: Shanghai Jiao Tong University – sequence: 8 givenname: Wei surname: Hou fullname: Hou, Wei organization: Shanghai Jiao Tong University – sequence: 9 givenname: Lizhi orcidid: 0000-0002-6842-9167 surname: Zhang fullname: Zhang, Lizhi email: zhanglizhi@sjtu.edu.cn, zhanglz@mail.ccnu.edu.cn organization: Central China Normal University |
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| Cites_doi | 10.1073/pnas.1813605115 10.1021/jacs.6b10435 10.1038/s41563-019-0444-y 10.1002/adma.201803234 10.1038/s41570-018-0010-1 10.1038/s41467-019-09290-y 10.1002/adma.201705369 10.1021/jacs.9b09391 10.1126/sciadv.aax6322 10.1126/science.aaw7515 10.1038/s41929-019-0246-2 10.1002/adma.202105410 10.1038/s41467-019-12510-0 10.1038/s41929-018-0203-5 10.1002/celc.202100147 10.1038/s41557-021-00734-x 10.1002/adma.202003191 10.1002/ange.201911441 10.1038/s41929-017-0008-y 10.1002/anie.201604802 10.1016/j.joule.2018.11.008 10.1038/s41467-019-14272-1 10.1038/s41467-019-13519-1 10.1038/s41467-021-23115-x 10.1016/j.chempr.2018.08.019 10.1021/acssuschemeng.8b01879 10.1038/s41565-021-01022-y 10.1038/s41565-018-0197-9 10.1002/anie.201511804 10.1002/anie.201911441 10.1002/ange.201604802 10.1016/j.xcrp.2019.100004 10.1002/ange.202000016 10.1021/acs.accounts.9b00412 10.1016/j.coelec.2022.100979 10.1002/celc.201900834 10.1039/C9GC01099H 10.1038/s41467-019-12859-2 10.1002/ange.201511804 10.1007/s10853-018-2961-5 10.1002/ange.201703720 10.1038/s41929-021-00621-1 10.1021/jacs.9b04907 10.1021/acs.accounts.8b00490 10.1021/jacs.1c10814 10.1002/anie.202000016 10.1038/s41467-020-14402-0 10.1002/sstr.202000067 10.1016/j.chempr.2017.12.005 10.1039/C8EE03676D 10.1039/C4NR00402G 10.1021/acscatal.9b01159 10.1073/pnas.1319663111 10.1002/aenm.201901945 10.1002/anie.201703720 10.1038/s41467-020-14984-9 |
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| References | 2021; 8 2019; 9 2019; 3 2021; 4 2019; 6 2019; 5 2021; 2 2019; 52 2019; 2 2019; 10 2019; 54 2019; 12 2020 2020; 59 132 2019; 18 2020; 11 2017 2017; 56 129 2020; 32 2020; 10 2019; 141 2014; 111 2019; 364 2019 2019; 58 131 2017; 139 2022; 144 2021; 13 2018; 6 2018; 2 2016 2016; 55 128 2021; 12 2018; 4 2020; 1 2018; 1 2019; 21 2018; 115 2022; 34 2018; 30 2014; 6 2022; 17 2018; 13 e_1_2_3_50_2 e_1_2_3_4_2 e_1_2_3_16_2 e_1_2_3_37_2 e_1_2_3_2_2 e_1_2_3_18_2 e_1_2_3_39_2 e_1_2_3_12_1 e_1_2_3_56_2 e_1_2_3_8_2 e_1_2_3_33_2 e_1_2_3_58_2 e_1_2_3_6_2 e_1_2_3_14_2 e_1_2_3_35_2 e_1_2_3_31_1 e_1_2_3_52_2 e_1_2_3_10_2 e_1_2_3_54_1 e_1_2_3_60_2 e_1_2_3_49_2 e_1_2_3_28_2 e_1_2_3_45_1 e_1_2_3_24_2 e_1_2_3_47_2 e_1_2_3_24_3 e_1_2_3_26_1 e_1_2_3_41_2 e_1_2_3_64_2 e_1_2_3_20_2 e_1_2_3_43_2 e_1_2_3_62_2 e_1_2_3_22_1 e_1_2_3_1_1 e_1_2_3_19_2 e_1_2_3_38_2 e_1_2_3_3_3 e_1_2_3_5_1 e_1_2_3_3_2 e_1_2_3_17_2 e_1_2_3_59_2 e_1_2_3_59_3 e_1_2_3_9_2 e_1_2_3_11_2 e_1_2_3_34_2 e_1_2_3_57_1 e_1_2_3_55_2 e_1_2_3_7_2 e_1_2_3_13_2 e_1_2_3_15_1 e_1_2_3_36_1 e_1_2_3_30_2 e_1_2_3_51_2 e_1_2_3_32_2 e_1_2_3_53_2 e_1_2_3_61_1 e_1_2_3_40_1 e_1_2_3_27_2 e_1_2_3_29_2 e_1_2_3_21_3 e_1_2_3_23_2 e_1_2_3_25_1 e_1_2_3_48_1 e_1_2_3_25_2 e_1_2_3_46_2 e_1_2_3_65_1 e_1_2_3_44_1 e_1_2_3_21_2 e_1_2_3_42_2 e_1_2_3_63_2 |
| References_xml | – volume: 10 year: 2020 publication-title: Adv. Energy Mater. – volume: 2 start-page: 65 year: 2018 end-page: 81 publication-title: Nat. Chem. Rev. – volume: 1 year: 2020 publication-title: Cell Rep. Phys. Sci. – volume: 12 start-page: 1241 year: 2019 end-page: 1248 publication-title: Energy Environ. Sci. – volume: 21 start-page: 3256 year: 2019 end-page: 3262 publication-title: Green Chem. – volume: 2 start-page: 134 year: 2019 end-page: 141 publication-title: Nat. Catal. – volume: 59 132 start-page: 12612 12712 year: 2020 2020 end-page: 12622 12722 publication-title: Angew. Chem. Int. Ed. Angew. Chem. – volume: 4 start-page: 285 year: 2018 end-page: 297 publication-title: Chem – volume: 144 start-page: 2171 year: 2022 end-page: 2178 publication-title: J. Am. Chem. Soc. – volume: 3 start-page: 584 year: 2019 end-page: 594 publication-title: Joule – volume: 54 start-page: 949 year: 2019 end-page: 973 publication-title: J. Mater. Sci. – volume: 139 start-page: 1885 year: 2017 end-page: 1893 publication-title: J. Am. Chem. Soc. – volume: 9 start-page: 8561 year: 2019 end-page: 8574 publication-title: ACS Catal. – volume: 115 start-page: 12692 year: 2018 end-page: 12697 publication-title: Proc. Natl. Acad. Sci. USA – volume: 141 start-page: 12717 year: 2019 end-page: 12723 publication-title: J. Am. Chem. Soc. – volume: 52 start-page: 237 year: 2019 end-page: 247 publication-title: Acc. Chem. Res. – volume: 34 year: 2022 publication-title: Adv. Mater. – volume: 10 start-page: 1278 year: 2019 publication-title: Nat. Commun. – volume: 52 start-page: 2858 year: 2019 end-page: 2869 publication-title: Acc. Chem. Res. – volume: 111 start-page: 45 year: 2014 end-page: 50 publication-title: Proc. Natl. Acad. Sci. USA – volume: 13 start-page: 887 year: 2021 end-page: 894 publication-title: Nat. Chem. – volume: 56 129 start-page: 7847 7955 year: 2017 2017 end-page: 7852 7960 publication-title: Angew. Chem. Int. Ed. Angew. Chem. – volume: 8 start-page: 1204 year: 2021 end-page: 1210 publication-title: ChemElectroChem – volume: 10 start-page: 4585 year: 2019 publication-title: Nat. Commun. – volume: 11 start-page: 1263 year: 2020 publication-title: Nat. Commun. – volume: 34 year: 2022 publication-title: Curr. Opin. Electrochem. – volume: 6 start-page: 9566 year: 2018 end-page: 9571 publication-title: ACS Sustainable Chem. Eng. – volume: 10 start-page: 5692 year: 2019 publication-title: Nat. Commun. – volume: 13 start-page: 856 year: 2018 end-page: 861 publication-title: Nat. Nanotechnol. – volume: 55 128 start-page: 10800 10958 year: 2016 2016 end-page: 10805 10963 publication-title: Angew. Chem. Int. Ed. Angew. Chem. – volume: 6 start-page: 3401 year: 2019 end-page: 3409 publication-title: ChemElectroChem – volume: 17 start-page: 174 year: 2022 end-page: 181 publication-title: Nat. Nanotechnol. – volume: 2 year: 2021 publication-title: Small Struct. – volume: 11 start-page: 412 year: 2020 publication-title: Nat. Commun. – volume: 12 start-page: 2870 year: 2021 publication-title: Nat. Commun. – volume: 2 start-page: 304 year: 2019 end-page: 313 publication-title: Nat. Catal. – volume: 141 start-page: 19964 year: 2019 end-page: 19968 publication-title: J. Am. Chem. Soc. – volume: 18 start-page: 1215 year: 2019 end-page: 1221 publication-title: Nat. Mater. – volume: 4 start-page: 469 year: 2021 end-page: 478 publication-title: Nat. Catal. – volume: 30 year: 2018 publication-title: Adv. Mater. – volume: 58 131 start-page: 18883 19059 year: 2019 2019 end-page: 18887 19063 publication-title: Angew. Chem. Int. Ed. Angew. Chem. – volume: 10 start-page: 4855 year: 2019 publication-title: Nat. Commun. – volume: 32 year: 2020 publication-title: Adv. Mater. – volume: 1 start-page: 63 year: 2018 end-page: 72 publication-title: Nat. Catal. – volume: 6 start-page: 5063 year: 2014 end-page: 5074 publication-title: Nanoscale – volume: 5 year: 2019 publication-title: Sci. Adv. – volume: 364 start-page: 1091 year: 2019 end-page: 1094 publication-title: Science – volume: 4 start-page: 2571 year: 2018 end-page: 2586 publication-title: Chem – volume: 11 start-page: 593 year: 2020 publication-title: Nat. Commun. – volume: 55 128 start-page: 7501 7627 year: 2016 2016 end-page: 7504 7630 publication-title: Angew. Chem. Int. Ed. Angew. Chem. – ident: e_1_2_3_19_2 doi: 10.1073/pnas.1813605115 – ident: e_1_2_3_47_2 doi: 10.1021/jacs.6b10435 – ident: e_1_2_3_53_2 doi: 10.1038/s41563-019-0444-y – ident: e_1_2_3_51_2 doi: 10.1002/adma.201803234 – ident: e_1_2_3_13_2 doi: 10.1038/s41570-018-0010-1 – ident: e_1_2_3_29_2 doi: 10.1038/s41467-019-09290-y – ident: e_1_2_3_52_2 doi: 10.1002/adma.201705369 – ident: e_1_2_3_6_2 doi: 10.1021/jacs.9b09391 – ident: e_1_2_3_12_1 – ident: e_1_2_3_37_2 doi: 10.1126/sciadv.aax6322 – ident: e_1_2_3_10_2 doi: 10.1126/science.aaw7515 – ident: e_1_2_3_57_1 – ident: e_1_2_3_11_2 doi: 10.1038/s41929-019-0246-2 – ident: e_1_2_3_27_2 doi: 10.1002/adma.202105410 – ident: e_1_2_3_39_2 doi: 10.1038/s41467-019-12510-0 – ident: e_1_2_3_48_1 – ident: e_1_2_3_9_2 doi: 10.1038/s41929-018-0203-5 – ident: e_1_2_3_26_1 – ident: e_1_2_3_60_2 doi: 10.1002/celc.202100147 – ident: e_1_2_3_17_2 doi: 10.1038/s41557-021-00734-x – ident: e_1_2_3_35_2 doi: 10.1002/adma.202003191 – ident: e_1_2_3_24_3 doi: 10.1002/ange.201911441 – ident: e_1_2_3_61_1 – ident: e_1_2_3_14_2 doi: 10.1038/s41929-017-0008-y – ident: e_1_2_3_21_2 doi: 10.1002/anie.201604802 – ident: e_1_2_3_23_2 doi: 10.1016/j.joule.2018.11.008 – ident: e_1_2_3_7_2 doi: 10.1038/s41467-019-14272-1 – ident: e_1_2_3_49_2 doi: 10.1038/s41467-019-13519-1 – ident: e_1_2_3_5_1 – ident: e_1_2_3_8_2 doi: 10.1038/s41467-021-23115-x – ident: e_1_2_3_4_2 doi: 10.1016/j.chempr.2018.08.019 – ident: e_1_2_3_34_2 doi: 10.1021/acssuschemeng.8b01879 – ident: e_1_2_3_18_2 doi: 10.1038/s41565-021-01022-y – ident: e_1_2_3_38_2 doi: 10.1038/s41565-018-0197-9 – ident: e_1_2_3_59_2 doi: 10.1002/anie.201511804 – ident: e_1_2_3_24_2 doi: 10.1002/anie.201911441 – ident: e_1_2_3_1_1 – ident: e_1_2_3_21_3 doi: 10.1002/ange.201604802 – ident: e_1_2_3_40_1 – ident: e_1_2_3_15_1 – ident: e_1_2_3_16_2 doi: 10.1016/j.xcrp.2019.100004 – ident: e_1_2_3_3_3 doi: 10.1002/ange.202000016 – ident: e_1_2_3_2_2 doi: 10.1021/acs.accounts.9b00412 – ident: e_1_2_3_64_2 doi: 10.1016/j.coelec.2022.100979 – ident: e_1_2_3_54_1 – ident: e_1_2_3_63_2 doi: 10.1002/celc.201900834 – ident: e_1_2_3_65_1 doi: 10.1039/C9GC01099H – ident: e_1_2_3_31_1 – ident: e_1_2_3_50_2 doi: 10.1038/s41467-019-12859-2 – ident: e_1_2_3_59_3 doi: 10.1002/ange.201511804 – ident: e_1_2_3_46_2 doi: 10.1007/s10853-018-2961-5 – ident: e_1_2_3_25_2 doi: 10.1002/ange.201703720 – ident: e_1_2_3_43_2 doi: 10.1038/s41929-021-00621-1 – ident: e_1_2_3_30_2 doi: 10.1021/jacs.9b04907 – ident: e_1_2_3_20_2 doi: 10.1021/acs.accounts.8b00490 – ident: e_1_2_3_45_1 – ident: e_1_2_3_22_1 – ident: e_1_2_3_55_2 doi: 10.1021/jacs.1c10814 – ident: e_1_2_3_36_1 – ident: e_1_2_3_3_2 doi: 10.1002/anie.202000016 – ident: e_1_2_3_28_2 doi: 10.1038/s41467-020-14402-0 – ident: e_1_2_3_41_2 doi: 10.1002/sstr.202000067 – ident: e_1_2_3_56_2 doi: 10.1016/j.chempr.2017.12.005 – ident: e_1_2_3_58_2 doi: 10.1039/C8EE03676D – ident: e_1_2_3_33_2 doi: 10.1039/C4NR00402G – ident: e_1_2_3_62_2 doi: 10.1021/acscatal.9b01159 – ident: e_1_2_3_32_2 doi: 10.1073/pnas.1319663111 – ident: e_1_2_3_44_1 doi: 10.1002/aenm.201901945 – ident: e_1_2_3_25_1 doi: 10.1002/anie.201703720 – ident: e_1_2_3_42_2 doi: 10.1038/s41467-020-14984-9 |
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| Snippet | Fabricating single‐atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the... Fabricating single-atom electrodes via atomic dispersion of active metal atoms into monolithic metal supports is of great significance to advancing the... |
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| SubjectTerms | Ammonia Bifunctionality Chlorine Chlorine Evolution Reaction Dimensional stability Dimensionally stable anodes Electrochemistry Electrodes Evolution Inherent Oxide Anchoring Strategy Nitrate reduction Nitrate Reduction Reaction Single Atom Monolithic Electrode Titanium |
| Title | Single Atom Ru Monolithic Electrode for Efficient Chlorine Evolution and Nitrate Reduction |
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