Metal‐Free Organocatalyzed Atom Transfer Radical Polymerization: Synthesis, Applications, and Future Perspectives

Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well‐defined structure, properties, and functionalities. Among the available RDRPs, ATRP is the most investigated. However, the necessity of a metal catalyst represents a d...

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Published inMacromolecular rapid communications. Vol. 42; no. 15; pp. e2100221 - n/a
Main Authors Ávila Gonçalves, Sayeny, R. Rodrigues, Plínio, Pioli Vieira, Roniérik
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 01.08.2021
Subjects
Catalysts
Chemical synthesis
controlled polymerization
Deactivation
Functional materials
Irradiation
Light irradiation
metal‐free polymerization
Organic compounds
organic synthesis
O‐ATRP
photocatalysts
Polymerization
Polymers
Radiation
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Abstract Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well‐defined structure, properties, and functionalities. Among the available RDRPs, ATRP is the most investigated. However, the necessity of a metal catalyst represents a drawback and limits its use for some applications. O‐ATRP emerged as an alternative to traditional ATRP that uses organic compounds that catalyze polymerization under light irradiation instead of metal. The friendly nature and the robustness of O‐ATRP allow its use in the synthesis of tailorable advanced materials with unique properties. In this review, the fundamental aspects of the reductive and oxidative quenching mechanism of O‐ATRP are provided, as well as insights into each component and its role in the reaction. Besides, the breakthrough recent studies that applied O‐ATRP for the synthesis of functional materials are presented, which illustrate the significant potential and impact of this technique across diverse fields. O‐ATRP has emerged as an important alternative for controllable polymerizations due to the use of photoredox organic catalysts instead of metals. The robustness and friendly‐nature of O‐ATRP endorse its use in the synthesis of tailorable materials with diverse properties. This review covers the fundamental aspects and progress of O‐ATRP, as well as developments in O‐ATRP‐based materials for several areas.
AbstractList Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well‐defined structure, properties, and functionalities. Among the available RDRPs, ATRP is the most investigated. However, the necessity of a metal catalyst represents a drawback and limits its use for some applications. O‐ATRP emerged as an alternative to traditional ATRP that uses organic compounds that catalyze polymerization under light irradiation instead of metal. The friendly nature and the robustness of O‐ATRP allow its use in the synthesis of tailorable advanced materials with unique properties. In this review, the fundamental aspects of the reductive and oxidative quenching mechanism of O‐ATRP are provided, as well as insights into each component and its role in the reaction. Besides, the breakthrough recent studies that applied O‐ATRP for the synthesis of functional materials are presented, which illustrate the significant potential and impact of this technique across diverse fields. O‐ATRP has emerged as an important alternative for controllable polymerizations due to the use of photoredox organic catalysts instead of metals. The robustness and friendly‐nature of O‐ATRP endorse its use in the synthesis of tailorable materials with diverse properties. This review covers the fundamental aspects and progress of O‐ATRP, as well as developments in O‐ATRP‐based materials for several areas.
Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well-defined structure, properties, and functionalities. Among the available RDRPs, ATRP is the most investigated. However, the necessity of a metal catalyst represents a drawback and limits its use for some applications. O-ATRP emerged as an alternative to traditional ATRP that uses organic compounds that catalyze polymerization under light irradiation instead of metal. The friendly nature and the robustness of O-ATRP allow its use in the synthesis of tailorable advanced materials with unique properties. In this review, the fundamental aspects of the reductive and oxidative quenching mechanism of O-ATRP are provided, as well as insights into each component and its role in the reaction. Besides, the breakthrough recent studies that applied O-ATRP for the synthesis of functional materials are presented, which illustrate the significant potential and impact of this technique across diverse fields.Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well-defined structure, properties, and functionalities. Among the available RDRPs, ATRP is the most investigated. However, the necessity of a metal catalyst represents a drawback and limits its use for some applications. O-ATRP emerged as an alternative to traditional ATRP that uses organic compounds that catalyze polymerization under light irradiation instead of metal. The friendly nature and the robustness of O-ATRP allow its use in the synthesis of tailorable advanced materials with unique properties. In this review, the fundamental aspects of the reductive and oxidative quenching mechanism of O-ATRP are provided, as well as insights into each component and its role in the reaction. Besides, the breakthrough recent studies that applied O-ATRP for the synthesis of functional materials are presented, which illustrate the significant potential and impact of this technique across diverse fields.
Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well‐defined structure, properties, and functionalities. Among the available RDRPs, ATRP is the most investigated. However, the necessity of a metal catalyst represents a drawback and limits its use for some applications. O‐ATRP emerged as an alternative to traditional ATRP that uses organic compounds that catalyze polymerization under light irradiation instead of metal. The friendly nature and the robustness of O‐ATRP allow its use in the synthesis of tailorable advanced materials with unique properties. In this review, the fundamental aspects of the reductive and oxidative quenching mechanism of O‐ATRP are provided, as well as insights into each component and its role in the reaction. Besides, the breakthrough recent studies that applied O‐ATRP for the synthesis of functional materials are presented, which illustrate the significant potential and impact of this technique across diverse fields.
Author R. Rodrigues, Plínio
Pioli Vieira, Roniérik
Ávila Gonçalves, Sayeny
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  surname: Ávila Gonçalves
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  organization: University of Campinas
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  surname: R. Rodrigues
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  givenname: Roniérik
  orcidid: 0000-0002-1887-3120
  surname: Pioli Vieira
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e_1_2_9_129_1
e_1_2_9_144_1
e_1_2_9_106_1
e_1_2_9_125_1
e_1_2_9_15_1
e_1_2_9_38_1
e_1_2_9_140_1
e_1_2_9_121_1
e_1_2_9_19_1
e_1_2_9_42_1
e_1_2_9_88_1
e_1_2_9_61_1
e_1_2_9_46_1
e_1_2_9_84_1
e_1_2_9_23_1
e_1_2_9_80_1
e_1_2_9_5_1
e_1_2_9_1_1
e_1_2_9_114_1
e_1_2_9_137_1
e_1_2_9_118_1
e_1_2_9_133_1
e_1_2_9_156_1
e_1_2_9_9_1
Capek I. (e_1_2_9_27_1) 2011
e_1_2_9_152_1
e_1_2_9_69_1
e_1_2_9_110_1
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e_1_2_9_50_1
e_1_2_9_73_1
e_1_2_9_35_1
e_1_2_9_77_1
e_1_2_9_96_1
e_1_2_9_12_1
e_1_2_9_54_1
e_1_2_9_92_1
e_1_2_9_109_1
e_1_2_9_101_1
e_1_2_9_128_1
e_1_2_9_105_1
e_1_2_9_124_1
e_1_2_9_147_1
e_1_2_9_39_1
e_1_2_9_120_1
e_1_2_9_16_1
e_1_2_9_58_1
e_1_2_9_143_1
e_1_2_9_20_1
e_1_2_9_62_1
e_1_2_9_89_1
e_1_2_9_24_1
e_1_2_9_43_1
e_1_2_9_66_1
e_1_2_9_85_1
e_1_2_9_81_1
e_1_2_9_4_1
e_1_2_9_113_1
e_1_2_9_117_1
e_1_2_9_155_1
e_1_2_9_136_1
e_1_2_9_151_1
e_1_2_9_28_1
e_1_2_9_47_1
e_1_2_9_132_1
e_1_2_9_74_1
e_1_2_9_51_1
e_1_2_9_78_1
Nicolas J. (e_1_2_9_8_1) 2013; 30
e_1_2_9_13_1
e_1_2_9_32_1
e_1_2_9_55_1
e_1_2_9_97_1
e_1_2_9_93_1
e_1_2_9_108_1
e_1_2_9_70_1
e_1_2_9_127_1
e_1_2_9_100_1
e_1_2_9_123_1
e_1_2_9_104_1
e_1_2_9_146_1
e_1_2_9_17_1
e_1_2_9_36_1
e_1_2_9_59_1
e_1_2_9_142_1
Tran H. M. (e_1_2_9_41_1) 2019; 43
e_1_2_9_63_1
e_1_2_9_40_1
Tran H. M. (e_1_2_9_65_1) 2019; 43
e_1_2_9_21_1
e_1_2_9_67_1
e_1_2_9_44_1
e_1_2_9_86_1
e_1_2_9_7_1
e_1_2_9_82_1
e_1_2_9_3_1
e_1_2_9_112_1
e_1_2_9_139_1
e_1_2_9_116_1
e_1_2_9_135_1
e_1_2_9_158_1
e_1_2_9_25_1
e_1_2_9_131_1
e_1_2_9_154_1
e_1_2_9_48_1
e_1_2_9_29_1
e_1_2_9_150_1
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Snippet Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well‐defined structure,...
Reversible deactivation radical polymerization (RDRP) is a class of powerful techniques capable of synthesizing polymers with a well-defined structure,...
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StartPage e2100221
SubjectTerms Catalysts
Chemical synthesis
controlled polymerization
Deactivation
Functional materials
Irradiation
Light irradiation
metal‐free polymerization
Organic compounds
organic synthesis
O‐ATRP
photocatalysts
Polymerization
Polymers
Radiation
Title Metal‐Free Organocatalyzed Atom Transfer Radical Polymerization: Synthesis, Applications, and Future Perspectives
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fmarc.202100221
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Volume 42
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