Simultaneously improved electromagnetic interference shielding and mechanical performance of segregated carbon nanotube/polypropylene composite via solid phase molding

Conductive polymer composite with segregated structure has been well demonstrated to achieve high electromagnetic interference shielding effectiveness (EMI SE) due to the selectively distributed electrical nanofillers to establish desirable conductive networks. Nevertheless, the formation of segrega...

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Published in	Composites science and technology Vol. 156; pp. 87 - 94
Main Authors	Wu, Hong-Yuan, Jia, Li-Chuan, Yan, Ding-Xiang, Gao, Jie-feng, Zhang, Xiao-Peng, Ren, Peng-Gang, Li, Zhong-Ming
Format	Journal Article
Language	English
Published	Barking Elsevier Ltd 01.03.2018 Elsevier BV
Subjects	Carbon nanotubes Compressive strength Construction materials Crystal structure Crystallinity Electric power distribution Electromagnetic interference shielding Electromagnetic shielding Low-melt-viscosity polymer Mechanical properties Nanotubes Polymer matrix composites Polymers Polypropylene Pressure Pressure effects Segregated structure Temperature effects Viscosity Electromagnetic interference shielding Mechanical properties Low-melt-viscosity polymer Segregated structure
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Abstract	Conductive polymer composite with segregated structure has been well demonstrated to achieve high electromagnetic interference shielding effectiveness (EMI SE) due to the selectively distributed electrical nanofillers to establish desirable conductive networks. Nevertheless, the formation of segregated structure in low-melt-viscosity semi-crystalline polymer is still challenged and the segregated composite always suffers poor mechanical performance. Herein, elevated pressure and temperature were utilized to make a typical semi-crystalline polymer, polypropylene (PP), hold solid phase to restrict the diffusion of carbon nanotube (CNT) into its interior. Segregated CNT networks were facilely constructed in the resultant CNT/PP composite and imparted it with a superior EMI SE of 48.3 dB at 2.2 mm thickness and 5.0 wt% CNT loading, the highest EMI shielding level among the reported CNT/polymer composites at equivalent material thickness and CNT loading. Moreover, the elevated pressure and temperature effect dramatically increase the compressive, tensile, and flexural strength (modulus) of the CNT/PP composite by 133% (65%), 74% (130%) and 53% (50%), respectively, in comparison to those for conventional segregated CNT/PP composite, really overcoming the major mechanical shortcoming in the development of segregated composites for EMI shielding. Our work provides a facile strategy to fabricate the efficient EMI shielding and robust material with the construction of typical segregated structure in low-melt-viscosity semi-crystalline polymers.
AbstractList	Conductive polymer composite with segregated structure has been well demonstrated to achieve high electromagnetic interference shielding effectiveness (EMI SE) due to the selectively distributed electrical nanofillers to establish desirable conductive networks. Nevertheless, the formation of segregated structure in low-melt-viscosity semi-crystalline polymer is still challenged and the segregated composite always suffers poor mechanical performance. Herein, elevated pressure and temperature were utilized to make a typical semi-crystalline polymer, polypropylene (PP), hold solid phase to restrict the diffusion of carbon nanotube (CNT) into its interior. Segregated CNT networks were facilely constructed in the resultant CNT/PP composite and imparted it with a superior EMI SE of 48.3 dB at 2.2 mm thickness and 5.0 wt% CNT loading, the highest EMI shielding level among the reported CNT/polymer composites at equivalent material thickness and CNT loading. Moreover, the elevated pressure and temperature effect dramatically increase the compressive, tensile, and flexural strength (modulus) of the CNT/PP composite by 133% (65%), 74% (130%) and 53% (50%), respectively, in comparison to those for conventional segregated CNT/PP composite, really overcoming the major mechanical shortcoming in the development of segregated composites for EMI shielding. Our work provides a facile strategy to fabricate the efficient EMI shielding and robust material with the construction of typical segregated structure in low-melt-viscosity semi-crystalline polymers.
Author	Ren, Peng-Gang Yan, Ding-Xiang Zhang, Xiao-Peng Jia, Li-Chuan Li, Zhong-Ming Gao, Jie-feng Wu, Hong-Yuan
Author_xml	– sequence: 1 givenname: Hong-Yuan surname: Wu fullname: Wu, Hong-Yuan organization: College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu 610065, China – sequence: 2 givenname: Li-Chuan surname: Jia fullname: Jia, Li-Chuan organization: College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu 610065, China – sequence: 3 givenname: Ding-Xiang surname: Yan fullname: Yan, Ding-Xiang email: yandingxiang@scu.edu.cn organization: School of Aeronautics and Astronautics, Sichuan University, Chengdu 610065, China – sequence: 4 givenname: Jie-feng surname: Gao fullname: Gao, Jie-feng organization: The College of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou, 225009, China – sequence: 5 givenname: Xiao-Peng surname: Zhang fullname: Zhang, Xiao-Peng organization: College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu 610065, China – sequence: 6 givenname: Peng-Gang surname: Ren fullname: Ren, Peng-Gang organization: Institute of Printing, Packaging Engineering and Digital Media Technology, Xi'an University of Technology, Xi'an, Shaanxi 710048, China – sequence: 7 givenname: Zhong-Ming surname: Li fullname: Li, Zhong-Ming organization: College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University, Chengdu 610065, China
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Snippet	Conductive polymer composite with segregated structure has been well demonstrated to achieve high electromagnetic interference shielding effectiveness (EMI SE)...
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SubjectTerms	Carbon nanotubes Compressive strength Construction materials Crystal structure Crystallinity Electric power distribution Electromagnetic interference shielding Electromagnetic shielding Low-melt-viscosity polymer Mechanical properties Nanotubes Polymer matrix composites Polymers Polypropylene Pressure Pressure effects Segregated structure Temperature effects Viscosity
Title	Simultaneously improved electromagnetic interference shielding and mechanical performance of segregated carbon nanotube/polypropylene composite via solid phase molding
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