Dilute Doping, Defects, and Ferromagnetism in Metal Oxide Systems

Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic impurities on the physical properties of functional non‐magnetic metal oxides such as TiO2 and ZnO. This effort is aimed at inducing spin functi...

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Bibliographic Details
Published inAdvanced materials (Weinheim) Vol. 22; no. 29; pp. 3125 - 3155
Main Author Ogale, Satishchandra B.
Format Journal Article
LanguageEnglish
Published Weinheim WILEY-VCH Verlag 03.08.2010
WILEY‐VCH Verlag
Subjects
Defects
Dilution
Doping
Ferromagnetism
Impurities
Magnetics
Metal oxides
Models, Molecular
Models, Theoretical
Oxides
Oxides - chemistry
Semiconductors
Titanium dioxide
Transition Elements - chemistry
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Abstract Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic impurities on the physical properties of functional non‐magnetic metal oxides such as TiO2 and ZnO. This effort is aimed at inducing spin functionality (magnetism, spin polarization) and thereby novel magneto‐transport and magneto‐optic effects in such oxides. After an early excitement and in spite of some very promising results reported in the literature, this field of diluted magnetic semiconducting oxides (DMSO) has continued to be dogged by concerns regarding uniformity of dopant incorporation, the possibilities of secondary ferromagnetic phases, and contamination issues. The rather sensitive dependence of magnetism of the DMSO systems on growth methods and conditions has led to interesting questions regarding the specific role played by defects in the attendant phenomena. Indeed, it has also led to the rapid re‐emergence of the field of defect ferromagnetism. Many theoretical studies have contributed to the analysis of diverse experimental observations in this field and in some cases to the predictions of new systems and scenarios. In this review an attempt is made to capture the scope and spirit of this effort highlighting the successes, concerns, and questions. The realization of ferromagnetism in functional non‐magnetic metal oxides, such as TiO2 and ZnO, by dilute doping of magnetic impurities or controlled introduction of specific defect types is reviewed. An attempt is made to capture the scope and spirit of this field as it developed over the past decade highlighting the successes, concerns, and new questions. Future research directions are discussed as well.
AbstractList Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic impurities on the physical properties of functional non‐magnetic metal oxides such as TiO2 and ZnO. This effort is aimed at inducing spin functionality (magnetism, spin polarization) and thereby novel magneto‐transport and magneto‐optic effects in such oxides. After an early excitement and in spite of some very promising results reported in the literature, this field of diluted magnetic semiconducting oxides (DMSO) has continued to be dogged by concerns regarding uniformity of dopant incorporation, the possibilities of secondary ferromagnetic phases, and contamination issues. The rather sensitive dependence of magnetism of the DMSO systems on growth methods and conditions has led to interesting questions regarding the specific role played by defects in the attendant phenomena. Indeed, it has also led to the rapid re‐emergence of the field of defect ferromagnetism. Many theoretical studies have contributed to the analysis of diverse experimental observations in this field and in some cases to the predictions of new systems and scenarios. In this review an attempt is made to capture the scope and spirit of this effort highlighting the successes, concerns, and questions. The realization of ferromagnetism in functional non‐magnetic metal oxides, such as TiO2 and ZnO, by dilute doping of magnetic impurities or controlled introduction of specific defect types is reviewed. An attempt is made to capture the scope and spirit of this field as it developed over the past decade highlighting the successes, concerns, and new questions. Future research directions are discussed as well.
Abstract Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic impurities on the physical properties of functional non‐magnetic metal oxides such as TiO 2 and ZnO. This effort is aimed at inducing spin functionality (magnetism, spin polarization) and thereby novel magneto‐transport and magneto‐optic effects in such oxides. After an early excitement and in spite of some very promising results reported in the literature, this field of diluted magnetic semiconducting oxides (DMSO) has continued to be dogged by concerns regarding uniformity of dopant incorporation, the possibilities of secondary ferromagnetic phases, and contamination issues. The rather sensitive dependence of magnetism of the DMSO systems on growth methods and conditions has led to interesting questions regarding the specific role played by defects in the attendant phenomena. Indeed, it has also led to the rapid re‐emergence of the field of defect ferromagnetism. Many theoretical studies have contributed to the analysis of diverse experimental observations in this field and in some cases to the predictions of new systems and scenarios. In this review an attempt is made to capture the scope and spirit of this effort highlighting the successes, concerns, and questions.
Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic impurities on the physical properties of functional non-magnetic metal oxides such as TiO sub(2) and ZnO. This effort is aimed at inducing spin functionality (magnetism, spin polarization) and thereby novel magneto-transport and magneto-optic effects in such oxides. After an early excitement and in spite of some very promising results reported in the literature, this field of diluted magnetic semiconducting oxides (DMSO) has continued to be dogged by concerns regarding uniformity of dopant incorporation, the possibilities of secondary ferromagnetic phases, and contamination issues. The rather sensitive dependence of magnetism of the DMSO systems on growth methods and conditions has led to interesting questions regarding the specific role played by defects in the attendant phenomena. Indeed, it has also led to the rapid re-emergence of the field of defect ferromagnetism. Many theoretical studies have contributed to the analysis of diverse experimental observations in this field and in some cases to the predictions of new systems and scenarios. In this review an attempt is made to capture the scope and spirit of this effort highlighting the successes, concerns, and questions. The realization of ferromagnetism in functional non-magnetic metal oxides, such as TiO sub(2) and ZnO, by dilute doping of magnetic impurities or controlled introduction of specific defect types is reviewed. An attempt is made to capture the scope and spirit of this field as it developed over the past decade highlighting the successes, concerns, and new questions. Future research directions are discussed as well.
Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic impurities on the physical properties of functional non-magnetic metal oxides such as TiO(2) and ZnO. This effort is aimed at inducing spin functionality (magnetism, spin polarization) and thereby novel magneto-transport and magneto-optic effects in such oxides. After an early excitement and in spite of some very promising results reported in the literature, this field of diluted magnetic semiconducting oxides (DMSO) has continued to be dogged by concerns regarding uniformity of dopant incorporation, the possibilities of secondary ferromagnetic phases, and contamination issues. The rather sensitive dependence of magnetism of the DMSO systems on growth methods and conditions has led to interesting questions regarding the specific role played by defects in the attendant phenomena. Indeed, it has also led to the rapid re-emergence of the field of defect ferromagnetism. Many theoretical studies have contributed to the analysis of diverse experimental observations in this field and in some cases to the predictions of new systems and scenarios. In this review an attempt is made to capture the scope and spirit of this effort highlighting the successes, concerns, and questions.
Author Ogale, Satishchandra B.
Author_xml – sequence: 1
  givenname: Satishchandra B.
  surname: Ogale
  fullname: Ogale, Satishchandra B.
  email: sb.ogale@ncl.res.in, satishogale@gmail.com
  organization: Physical and Materials Chemistry Division, National Chemical Laboratory, Council of Scientific and Industrial Research, Dr. Homi Bhabha Road, Pashan, Pune 411008 (India) Indian Institute of Science Education and Research (IISER), Pune (India) Phone: 91-20-25902260, 91-9822628242, Fax: 91-20-25902636
BackLink https://www.ncbi.nlm.nih.gov/pubmed/20535732$$D View this record in MEDLINE/PubMed
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Snippet Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of magnetic...
Abstract Over the past decade intensive research efforts have been carried out by researchers around the globe on exploring the effects of dilute doping of...
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SubjectTerms Defects
Dilution
Doping
Ferromagnetism
Impurities
Magnetics
Metal oxides
Models, Molecular
Models, Theoretical
Oxides
Oxides - chemistry
Semiconductors
Titanium dioxide
Transition Elements - chemistry
Title Dilute Doping, Defects, and Ferromagnetism in Metal Oxide Systems
URI https://api.istex.fr/ark:/67375/WNG-Q7C7MLP3-1/fulltext.pdf
https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.200903891
https://www.ncbi.nlm.nih.gov/pubmed/20535732
https://search.proquest.com/docview/1884125283
https://search.proquest.com/docview/748925179
Volume 22
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