Pore structure evolution during lignite pyrolysis based on nuclear magnetic resonance
Increasing attention is being paid to the clean and efficient mining and utilization of coal resources. Lignite is a major component of coal; however, its high moisture and volatile contents and low calorific value cause it to have low mining and utilization efficiencies. During the dehydration, upg...
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Published in | Case studies in thermal engineering Vol. 26; p. 101125 |
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Format | Journal Article |
Language | English |
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01.08.2021
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Abstract | Increasing attention is being paid to the clean and efficient mining and utilization of coal resources. Lignite is a major component of coal; however, its high moisture and volatile contents and low calorific value cause it to have low mining and utilization efficiencies. During the dehydration, upgrading and in-situ heat injection or underground coal gasification of lignite, its pore structure plays an important role in the pyrolysis and product transfer processes. Therefore, it is necessary to systematically study the high-temperature pore structure of lignite. The evolution of pore fissures in gas-pyrolyzed lignite was studied by nuclear magnetic resonance combined with a gas heating reactor and test device. We found that the total connectivity, porosity and permeability of lignite increased between temperatures of 25 °C and 250 °C, then decreased at 350 °C and increased again at 450 °C. At 450 °C, the porosity, effective porosity and permeability of lignite were 18.32%, 30.22% and 856.98 md, respectively. The evolution in the pore structure parameters of lignite with temperature was observed to determine the changes in seepage channels that occur during the processes of lignite mining and utilization. |
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AbstractList | Increasing attention is being paid to the clean and efficient mining and utilization of coal resources. Lignite is a major component of coal; however, its high moisture and volatile contents and low calorific value cause it to have low mining and utilization efficiencies. During the dehydration, upgrading and in-situ heat injection or underground coal gasification of lignite, its pore structure plays an important role in the pyrolysis and product transfer processes. Therefore, it is necessary to systematically study the high-temperature pore structure of lignite. The evolution of pore fissures in gas-pyrolyzed lignite was studied by nuclear magnetic resonance combined with a gas heating reactor and test device. We found that the total connectivity, porosity and permeability of lignite increased between temperatures of 25 °C and 250 °C, then decreased at 350 °C and increased again at 450 °C. At 450 °C, the porosity, effective porosity and permeability of lignite were 18.32%, 30.22% and 856.98 md, respectively. The evolution in the pore structure parameters of lignite with temperature was observed to determine the changes in seepage channels that occur during the processes of lignite mining and utilization. |
ArticleNumber | 101125 |
Author | Niu, Shiwei Liu, Weizhen Tang, Haibo Zhou, Ke |
Author_xml | – sequence: 1 givenname: Weizhen orcidid: 0000-0002-1465-5409 surname: Liu fullname: Liu, Weizhen organization: College of Energy and Mining Engineering, Shandong University of Science and Technology, Qingdao, 266590, China – sequence: 2 givenname: Shiwei surname: Niu fullname: Niu, Shiwei email: nshiwei1123@sdust.edu.cn organization: College of Energy and Mining Engineering, Shandong University of Science and Technology, Qingdao, 266590, China – sequence: 3 givenname: Haibo surname: Tang fullname: Tang, Haibo organization: Mining Technology Institute, Taiyuan University of Technology, Taiyuan, 030024, China – sequence: 4 givenname: Ke surname: Zhou fullname: Zhou, Ke organization: College of Energy and Mining Engineering, Shandong University of Science and Technology, Qingdao, 266590, China |
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CitedBy_id | crossref_primary_10_1155_2022_8378062 crossref_primary_10_1016_j_petrol_2022_111150 crossref_primary_10_1016_j_compstruct_2023_117433 crossref_primary_10_1016_j_conbuildmat_2023_133278 crossref_primary_10_1016_j_joei_2021_09_014 crossref_primary_10_1038_s41598_022_09113_z crossref_primary_10_1021_acsomega_2c00157 crossref_primary_10_1007_s11053_023_10194_4 crossref_primary_10_1016_j_jnggs_2021_11_001 crossref_primary_10_1007_s10064_023_03315_z crossref_primary_10_1016_j_cec_2022_100006 crossref_primary_10_3390_w14030330 |
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Keywords | Pyrolysis Lignite Pore structure Nuclear magnetic resonance (NMR) |
Language | English |
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Title | Pore structure evolution during lignite pyrolysis based on nuclear magnetic resonance |
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