Ferroelectricity and Large Rashba Splitting in Two-Dimensional Tellurium
Two-dimensional (2D) ferroelectric (FE) systems are promising candidates for non-volatile nanodevices. Previous studies mainly focused on 2D compounds. Though counter-intuitive, here we propose several new phases of tellurium with (anti)ferroelectricity. Two-dimensional films can be viewed as a coll...
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| Published in | Chinese physics letters Vol. 40; no. 11; pp. 117102 - 129 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Chinese Physical Society and IOP Publishing Ltd
01.11.2023
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| Online Access | Get full text |
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| Abstract | Two-dimensional (2D) ferroelectric (FE) systems are promising candidates for non-volatile nanodevices. Previous studies mainly focused on 2D compounds. Though counter-intuitive, here we propose several new phases of tellurium with (anti)ferroelectricity. Two-dimensional films can be viewed as a collection of one-dimensional chains, and lone-pair instability is responsible for the (anti)ferroelectricity. The total polarization is determined to be 0.34 × 10
−10
C/m for the FE ground state. Due to the local polarization field in the FE film, we show a large Rashba splitting (
α
R
∼ 2 eV⋅Å) with nonzero spin Hall conductivity for experimental detection. Furthermore, a dipole-like distribution of Berry curvature is verified, which may facilitate a nonlinear Hall effect. Because Rashba-splitting/Berry-curvature distributions are fully coupled with a polarization field, they can be reversed through FE phase transition. Our results not only broaden the elemental FE materials, but also shed light on their intriguing transport phenomena. |
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| AbstractList | Two-dimensional(2D)ferroelectric(FE)systems are promising candidates for non-volatile nanodevices.Pre-vious studies mainly focused on 2D compounds.Though counter-intuitive,here we propose several new phases of tellurium with(anti)ferroelectricity.Two-dimensional films can be viewed as a collection of one-dimensional chains,and lone-pair instability is responsible for the(anti)ferroelectricity.The total polarization is determined to be 0.34 × 10-10 C/m for the FE ground state.Due to the local polarization field in the FE film,we show a large Rashba splitting(αR～2 eV·?)with nonzero spin Hall conductivity for experimental detection.Furthermore,a dipole-like distribution of Berry curvature is verified,which may facilitate a nonlinear Hall effect.Because Rashba-splitting/Berry-curvature distributions are fully coupled with a polarization field,they can be reversed through FE phase transition.Our results not only broaden the elemental FE materials,but also shed light on their intriguing transport phenomena. Two-dimensional (2D) ferroelectric (FE) systems are promising candidates for non-volatile nanodevices. Previous studies mainly focused on 2D compounds. Though counter-intuitive, here we propose several new phases of tellurium with (anti)ferroelectricity. Two-dimensional films can be viewed as a collection of one-dimensional chains, and lone-pair instability is responsible for the (anti)ferroelectricity. The total polarization is determined to be 0.34 × 10 −10 C/m for the FE ground state. Due to the local polarization field in the FE film, we show a large Rashba splitting ( α R ∼ 2 eV⋅Å) with nonzero spin Hall conductivity for experimental detection. Furthermore, a dipole-like distribution of Berry curvature is verified, which may facilitate a nonlinear Hall effect. Because Rashba-splitting/Berry-curvature distributions are fully coupled with a polarization field, they can be reversed through FE phase transition. Our results not only broaden the elemental FE materials, but also shed light on their intriguing transport phenomena. |
| Author | Wang, Yao Lu, Yunhao Zhang, Jinsen Hua, Chenqiang Lei, Zhenzhen Tao, Xinyong |
| Author_xml | – sequence: 1 givenname: Yao surname: Wang fullname: Wang, Yao organization: Moganshan Research Institute at Deqing County Zhejiang University of Technology , China – sequence: 2 givenname: Zhenzhen surname: Lei fullname: Lei, Zhenzhen organization: College of Materials Science and Engineering, Zhejiang University of Technology , China – sequence: 3 givenname: Jinsen surname: Zhang fullname: Zhang, Jinsen organization: College of Materials Science and Engineering, Zhejiang University of Technology , China – sequence: 4 givenname: Xinyong surname: Tao fullname: Tao, Xinyong organization: College of Materials Science and Engineering, Zhejiang University of Technology , China – sequence: 5 givenname: Chenqiang surname: Hua fullname: Hua, Chenqiang organization: Zhongfa Aviation Institute of Beihang University , China – sequence: 6 givenname: Yunhao surname: Lu fullname: Lu, Yunhao organization: School of Physics, Zhejiang University , China |
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| Snippet | Two-dimensional (2D) ferroelectric (FE) systems are promising candidates for non-volatile nanodevices. Previous studies mainly focused on 2D compounds. Though... Two-dimensional(2D)ferroelectric(FE)systems are promising candidates for non-volatile nanodevices.Pre-vious studies mainly focused on 2D compounds.Though... |
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| Title | Ferroelectricity and Large Rashba Splitting in Two-Dimensional Tellurium |
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