Effect of support for alcohol-hydrocarbon synthesis from syngas in Cu-based catalyst
Effects of a Cu-based catalyst on the catalytic performance in alcohol-hydrocarbon synthesis from syngas have been investigated, using various supports. Under the different porosities of three supports (zinc oxide, activation carbon, and titanium dioxide), whereas Cu/ZnO produces one liquid phase of...
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| Published in | The Korean journal of chemical engineering Vol. 30; no. 4; pp. 864 - 870 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Boston
Springer US
01.04.2013
한국화학공학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0256-1115 1975-7220 |
| DOI | 10.1007/s11814-012-0205-y |
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| Abstract | Effects of a Cu-based catalyst on the catalytic performance in alcohol-hydrocarbon synthesis from syngas have been investigated, using various supports. Under the different porosities of three supports (zinc oxide, activation carbon, and titanium dioxide), whereas Cu/ZnO produces one liquid phase of major mixed alcohols, Cu/AC and Cu/TiO
2
create two phases, alcohol (∼75%) and hydrocarbon (∼25%). X-ray diffraction shows that CuO impregnated on supports undergoes a complete reduction of metallic copper Cu
0
, which is the real active phase in the catalytic process. The Cu/TiO
2
catalyst showed the highest ethanol composition in a mixed alcohol phase under GHSV 18,000 h
−1
, 30 bar, and 300 °C. |
|---|---|
| AbstractList | Effects of a Cu-based catalyst on the catalytic performance in alcohol-hydrocarbon synthesis from syngas have been investigated, using various supports. Under the different porosities of three supports (zinc oxide, activation carbon, and titanium dioxide), whereas Cu/ZnO produces one liquid phase of major mixed alcohols, Cu/AC and Cu/TiO2 create two phases, alcohol (~75%) and hydrocarbon (~25%). X-ray diffraction shows that CuO impregnated on supports undergoes a complete reduction of metallic copper Cu0, which is the real active phase in the catalytic process.
The Cu/TiO2 catalyst showed the highest ethanol composition in a mixed alcohol phase under GHSV 18,000 h−1, 30 bar,and 300 oC. KCI Citation Count: 7 Effects of a Cu-based catalyst on the catalytic performance in alcohol-hydrocarbon synthesis from syngas have been investigated, using various supports. Under the different porosities of three supports (zinc oxide, activation carbon, and titanium dioxide), whereas Cu/ZnO produces one liquid phase of major mixed alcohols, Cu/AC and Cu/TiO 2 create two phases, alcohol (∼75%) and hydrocarbon (∼25%). X-ray diffraction shows that CuO impregnated on supports undergoes a complete reduction of metallic copper Cu 0 , which is the real active phase in the catalytic process. The Cu/TiO 2 catalyst showed the highest ethanol composition in a mixed alcohol phase under GHSV 18,000 h −1 , 30 bar, and 300 °C. |
| Author | Shin, Dae-Hyun Shin, Kyoung-Hee Jin, Chang-Soo Nho, Nam-Sun Nam, Sung-Chan Yeon, Sun-Hwa |
| Author_xml | – sequence: 1 givenname: Sun-Hwa surname: Yeon fullname: Yeon, Sun-Hwa email: ys93@kier.re.kr organization: Energy Storage Group, Korea Institute of Energy Research – sequence: 2 givenname: Dae-Hyun surname: Shin fullname: Shin, Dae-Hyun organization: Energy Storage Group, Korea Institute of Energy Research – sequence: 3 givenname: Nam-Sun surname: Nho fullname: Nho, Nam-Sun organization: Energy Storage Group, Korea Institute of Energy Research – sequence: 4 givenname: Kyoung-Hee surname: Shin fullname: Shin, Kyoung-Hee organization: Energy Storage Group, Korea Institute of Energy Research – sequence: 5 givenname: Chang-Soo surname: Jin fullname: Jin, Chang-Soo organization: Energy Storage Group, Korea Institute of Energy Research – sequence: 6 givenname: Sung-Chan surname: Nam fullname: Nam, Sung-Chan organization: Energy Storage Group, Korea Institute of Energy Research |
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| CitedBy_id | crossref_primary_10_1021_acscatal_5b00090 crossref_primary_10_1016_j_molcata_2015_01_008 crossref_primary_10_1039_C6CS00324A crossref_primary_10_1016_j_apsusc_2017_02_164 crossref_primary_10_1016_j_jechem_2017_02_003 crossref_primary_10_1007_s11814_014_0236_7 crossref_primary_10_1016_j_molcata_2016_03_044 |
| Cites_doi | 10.1016/0926-860X(92)80195-I 10.1039/C0EE00436G 10.1016/0021-9517(88)90011-5 10.1016/0926-860X(92)80197-K 10.1126/science.1113354 10.1023/A:1019095832277 10.1016/j.cattod.2009.03.004 10.1038/447914a 10.1021/ef700411x 10.2174/138620712798868365 10.1002/cjce.5450610106 10.1039/ft9908602725 10.1016/0021-9517(78)90035-0 10.1039/b414039g 10.1016/j.jcat.2010.02.020 10.1016/S0926-860X(98)00299-3 10.1039/dc9817200121 |
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| Keywords | Activated Carbon Ethanol Titanium Dioxide Support Copper Zinc Oxide Catalyst |
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| Title | Effect of support for alcohol-hydrocarbon synthesis from syngas in Cu-based catalyst |
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