A benchmark for gel structures: bond percolation enables the fabrication of extremely homogeneous gels

Gels are soft-elastic materials consisting of a three-dimensional crosslinked polymer network and liquid filling the space between this network. Numerous gels with unique physical properties have been synthesized and are widely used in our daily lives. However, all of these gels contain a substantia...

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Bibliographic Details
Published inPolymer journal Vol. 53; no. 7; pp. 765 - 777
Main Author Li, Xiang
Format Journal Article
LanguageEnglish
Published London Nature Publishing Group UK 01.07.2021
Nature Publishing Group
Subjects
639/301/923/1027
639/638/455/959
Benchmarks
Biomaterials
Bioorganic Chemistry
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Defects
Focus Review
Percolation
Physical properties
Polymer gels
Polymer Sciences
Polymers
Scattering
Surfaces and Interfaces
Thin Films
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Abstract Gels are soft-elastic materials consisting of a three-dimensional crosslinked polymer network and liquid filling the space between this network. Numerous gels with unique physical properties have been synthesized and are widely used in our daily lives. However, all of these gels contain a substantial level of structural defects, as detected by scattering measurements. Despite the tremendous efforts made in recent decades to remove imperfections from gels, discernible signs of spatial defects have been persistently observed in gels. Researchers believe that gels are inherently heterogeneous. In this focus review, I briefly introduce a recent finding from our research group’s efforts to fabricate polymer gels free of spatial heterogeneities. The commonly observed scattering profiles for the spatial defects disappeared in the homogeneous gels. The newly observed scattering profiles are a benchmark for gel structures. Despite the tremendous efforts made in recent decades to remove imperfections from gels, discernible signs of spatial defects have been persistently observed in gels. Researchers believe that gels are inherently heterogeneous. In this focus review, I briefly introduce a recent finding from our research group’s efforts to fabricate polymer gels free of spatial heterogeneities via “bond percolation”. The commonly observed scattering profiles for the spatial defects disappeared in the homogeneous gels. The newly observed scattering profiles are a benchmark for gel structures.
AbstractList Gels are soft-elastic materials consisting of a three-dimensional crosslinked polymer network and liquid filling the space between this network. Numerous gels with unique physical properties have been synthesized and are widely used in our daily lives. However, all of these gels contain a substantial level of structural defects, as detected by scattering measurements. Despite the tremendous efforts made in recent decades to remove imperfections from gels, discernible signs of spatial defects have been persistently observed in gels. Researchers believe that gels are inherently heterogeneous. In this focus review, I briefly introduce a recent finding from our research group’s efforts to fabricate polymer gels free of spatial heterogeneities. The commonly observed scattering profiles for the spatial defects disappeared in the homogeneous gels. The newly observed scattering profiles are a benchmark for gel structures.Despite the tremendous efforts made in recent decades to remove imperfections from gels, discernible signs of spatial defects have been persistently observed in gels. Researchers believe that gels are inherently heterogeneous. In this focus review, I briefly introduce a recent finding from our research group’s efforts to fabricate polymer gels free of spatial heterogeneities via “bond percolation”. The commonly observed scattering profiles for the spatial defects disappeared in the homogeneous gels. The newly observed scattering profiles are a benchmark for gel structures.
Gels are soft-elastic materials consisting of a three-dimensional crosslinked polymer network and liquid filling the space between this network. Numerous gels with unique physical properties have been synthesized and are widely used in our daily lives. However, all of these gels contain a substantial level of structural defects, as detected by scattering measurements. Despite the tremendous efforts made in recent decades to remove imperfections from gels, discernible signs of spatial defects have been persistently observed in gels. Researchers believe that gels are inherently heterogeneous. In this focus review, I briefly introduce a recent finding from our research group’s efforts to fabricate polymer gels free of spatial heterogeneities. The commonly observed scattering profiles for the spatial defects disappeared in the homogeneous gels. The newly observed scattering profiles are a benchmark for gel structures. Despite the tremendous efforts made in recent decades to remove imperfections from gels, discernible signs of spatial defects have been persistently observed in gels. Researchers believe that gels are inherently heterogeneous. In this focus review, I briefly introduce a recent finding from our research group’s efforts to fabricate polymer gels free of spatial heterogeneities via “bond percolation”. The commonly observed scattering profiles for the spatial defects disappeared in the homogeneous gels. The newly observed scattering profiles are a benchmark for gel structures.
Author Li, Xiang
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  organization: Institute for Solid State Physics, The University of Tokyo
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Snippet Gels are soft-elastic materials consisting of a three-dimensional crosslinked polymer network and liquid filling the space between this network. Numerous gels...
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springer
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SubjectTerms 639/301/923/1027
639/638/455/959
Benchmarks
Biomaterials
Bioorganic Chemistry
Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Defects
Focus Review
Percolation
Physical properties
Polymer gels
Polymer Sciences
Polymers
Scattering
Surfaces and Interfaces
Thin Films
Title A benchmark for gel structures: bond percolation enables the fabrication of extremely homogeneous gels
URI https://link.springer.com/article/10.1038/s41428-021-00479-x
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