A Dendrite‐Free Lithium/Carbon Nanotube Hybrid for Lithium‐Metal Batteries

Lithium (Li) metal is promising in the next‐generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite‐free Li/carbon nanotube (CNT) hybrid is proposed, whic...

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Published inAdvanced materials (Weinheim) Vol. 33; no. 4; pp. e2006702 - n/a
Main Authors Wang, Zhi Yong, Lu, Zhong Xu, Guo, Wei, Luo, Qin, Yin, Yan Hong, Liu, Xian Bin, Li, Ye Sheng, Xia, Bao Yu, Wu, Zi Ping
Format Journal Article
LanguageEnglish
Published Germany Wiley Subscription Services, Inc 01.01.2021
Subjects
Carbon nanotubes
Current density
Cycles
dendrite‐free batteries
Dendritic structure
Energy storage
Lithium batteries
Li‐metal batteries
Materials science
molten lithium
Storage batteries
Storage systems
undercooling
Li-metal batteries
dendrite-free batteries
molten lithium
carbon nanotubes
undercooling
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Abstract Lithium (Li) metal is promising in the next‐generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite‐free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li‐metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super‐stable functions even at an ultrahigh current density of 40 mA cm−2 for 2000 cycles with a stripping/plating capacity of 2 mAh cm−2 in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li‐S battery. This work provides valuable concepts in fabricating Li anodes toward Li‐metal batteries and beyond for their high‐level services. A dendrite‐free Li/carbon nanotube (CNT) hybrid is fabricated by direct coating of molten Li on CNTs for Li‐metal batteries. Favorable thermodynamic and kinetic conditions are a powerful force to drive the rapid lift upward and infusion of molten Li into CNTs network. The obtained hybrid exhibits superstable function even at an ultrahigh current density.
AbstractList Lithium (Li) metal is promising in the next-generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite-free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li-metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super-stable functions even at an ultrahigh current density of 40 mA cm-2 for 2000 cycles with a stripping/plating capacity of 2 mAh cm-2 in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li-S battery. This work provides valuable concepts in fabricating Li anodes toward Li-metal batteries and beyond for their high-level services.Lithium (Li) metal is promising in the next-generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite-free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li-metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super-stable functions even at an ultrahigh current density of 40 mA cm-2 for 2000 cycles with a stripping/plating capacity of 2 mAh cm-2 in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li-S battery. This work provides valuable concepts in fabricating Li anodes toward Li-metal batteries and beyond for their high-level services.
Lithium (Li) metal is promising in the next‐generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite‐free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li‐metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super‐stable functions even at an ultrahigh current density of 40 mA cm−2 for 2000 cycles with a stripping/plating capacity of 2 mAh cm−2 in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li‐S battery. This work provides valuable concepts in fabricating Li anodes toward Li‐metal batteries and beyond for their high‐level services.
Lithium (Li) metal is promising in the next-generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite-free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li-metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super-stable functions even at an ultrahigh current density of 40 mA cm for 2000 cycles with a stripping/plating capacity of 2 mAh cm in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li-S battery. This work provides valuable concepts in fabricating Li anodes toward Li-metal batteries and beyond for their high-level services.
Lithium (Li) metal is promising in the next‐generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite‐free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li‐metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super‐stable functions even at an ultrahigh current density of 40 mA cm−2 for 2000 cycles with a stripping/plating capacity of 2 mAh cm−2 in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li‐S battery. This work provides valuable concepts in fabricating Li anodes toward Li‐metal batteries and beyond for their high‐level services. A dendrite‐free Li/carbon nanotube (CNT) hybrid is fabricated by direct coating of molten Li on CNTs for Li‐metal batteries. Favorable thermodynamic and kinetic conditions are a powerful force to drive the rapid lift upward and infusion of molten Li into CNTs network. The obtained hybrid exhibits superstable function even at an ultrahigh current density.
Lithium (Li) metal is promising in the next‐generation energy storage systems. However, its practical application is still hindered by the poor cycling performance and serious safety issues for the consequence of dendritic Li. Herein, a dendrite‐free Li/carbon nanotube (CNT) hybrid is proposed, which is fabricated by direct coating molten Li on CNTs, for Li‐metal batteries. The favorable thermodynamic and kinetic conditions are the powerful force to drive the rapid lift upwards and infusion of molten Li into CNTs network, which is the key to form a uniform metallic layer in Li/CNTs hybrid. The obtained hybrid indicates super‐stable functions even at an ultrahigh current density of 40 mA cm −2 for 2000 cycles with a stripping/plating capacity of 2 mAh cm −2 in symmetric cells. Subsequently, this hybrid also demonstrates a significantly decreased resistance, excellent cycling stability at high current density and flexibility in the full Li‐S battery. This work provides valuable concepts in fabricating Li anodes toward Li‐metal batteries and beyond for their high‐level services.
Author Guo, Wei
Luo, Qin
Li, Ye Sheng
Yin, Yan Hong
Lu, Zhong Xu
Wu, Zi Ping
Wang, Zhi Yong
Liu, Xian Bin
Xia, Bao Yu
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  fullname: Lu, Zhong Xu
  organization: Jiangxi University of Science and Technology (JXUST)
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  fullname: Yin, Yan Hong
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  organization: Jiangxi University of Science and Technology (JXUST)
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  surname: Wu
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  email: wuziping724@jxust.edu.cn
  organization: Jiangxi University of Science and Technology (JXUST)
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Keywords Li-metal batteries
dendrite-free batteries
molten lithium
carbon nanotubes
undercooling
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Snippet Lithium (Li) metal is promising in the next‐generation energy storage systems. However, its practical application is still hindered by the poor cycling...
Lithium (Li) metal is promising in the next-generation energy storage systems. However, its practical application is still hindered by the poor cycling...
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SubjectTerms Carbon nanotubes
Current density
Cycles
dendrite‐free batteries
Dendritic structure
Energy storage
Lithium batteries
Li‐metal batteries
Materials science
molten lithium
Storage batteries
Storage systems
undercooling
Title A Dendrite‐Free Lithium/Carbon Nanotube Hybrid for Lithium‐Metal Batteries
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fadma.202006702
https://www.ncbi.nlm.nih.gov/pubmed/33314412
https://www.proquest.com/docview/2480196671
https://www.proquest.com/docview/2470024265
Volume 33
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