Polycrystalline BiCuSeO oxide as a potential thermoelectric material
This work revealed that BiCuSeO oxyselenide is a potential oxide-based thermoelectric material, whose dimensionless figure of merit ( ZT ) reaches ∼0.70 at 773 K. High phase-purity BiCuSeO polycrystalline materials with fine grains were synthesized by a facile method combining a solid-state reaction...
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| Published in | Energy & environmental science Vol. 5; no. 5; pp. 7188 - 7195 |
|---|---|
| Main Authors | , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
01.05.2012
|
| Subjects | |
| Online Access | Get full text |
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| Abstract | This work revealed that BiCuSeO oxyselenide is a potential oxide-based thermoelectric material, whose dimensionless figure of merit (
ZT
) reaches ∼0.70 at 773 K. High phase-purity BiCuSeO polycrystalline materials with fine grains were synthesized by a facile method combining a solid-state reaction and spark plasma sintering. Purifying the constitutive phase and reducing the grain sizes by introducing a high-energy ball milling process before spark plasma sintering were found to be effective in property enhancement. The resultant single-phased BiCuSeO sample derived from ball-milled powders shows good electrical conductivity above 4.0 × 10
3
S m
−1
and a large Seebeck coefficient above 200 μV K
−1
. This compound has a low thermal conductivity (∼0.5 W m
−1
K
−1
), which is associated with its low phonon transport speed and Young's modulus. Results indicated that BiCuSeO-based materials are promising for energy conversion applications in the moderate temperature range.
Good electrical conductivity, large Seebeck coefficients and low thermal conductivity were obtained for pristine BiCuSeO oxides with a layered structure of alternately stacked conductive (Cu
2
Se
2
)
2−
and insulating (Bi
2
O
2
)
2+
layers, resulting in a high
ZT
value of 0.70 at 773 K. |
|---|---|
| AbstractList | This work revealed that BiCuSeO oxyselenide is a potential oxide-based thermoelectric material, whose dimensionless figure of merit (ZT) reaches similar to 0.70 at 773 K. High phase-purity BiCuSeO polycrystalline materials with fine grains were synthesized by a facile method combining a solid-state reaction and spark plasma sintering. Purifying the constitutive phase and reducing the grain sizes by introducing a high-energy ball milling process before spark plasma sintering were found to be effective in property enhancement. The resultant single-phased BiCuSeO sample derived from ball-milled powders shows good electrical conductivity above 4.0 10 super(3) S m super(-1) and a large Seebeck coefficient above 200 mu V K super(-1). This compound has a low thermal conductivity ( similar to 0.5 W m super(-1) K super(-1)), which is associated with its low phonon transport speed and Young's modulus. Results indicated that BiCuSeO-based materials are promising for energy conversion applications in the moderate temperature range. This work revealed that BiCuSeO oxyselenide is a potential oxide-based thermoelectric material, whose dimensionless figure of merit ( ZT ) reaches ∼0.70 at 773 K. High phase-purity BiCuSeO polycrystalline materials with fine grains were synthesized by a facile method combining a solid-state reaction and spark plasma sintering. Purifying the constitutive phase and reducing the grain sizes by introducing a high-energy ball milling process before spark plasma sintering were found to be effective in property enhancement. The resultant single-phased BiCuSeO sample derived from ball-milled powders shows good electrical conductivity above 4.0 × 10 3 S m −1 and a large Seebeck coefficient above 200 μV K −1 . This compound has a low thermal conductivity (∼0.5 W m −1 K −1 ), which is associated with its low phonon transport speed and Young's modulus. Results indicated that BiCuSeO-based materials are promising for energy conversion applications in the moderate temperature range. Good electrical conductivity, large Seebeck coefficients and low thermal conductivity were obtained for pristine BiCuSeO oxides with a layered structure of alternately stacked conductive (Cu 2 Se 2 ) 2− and insulating (Bi 2 O 2 ) 2+ layers, resulting in a high ZT value of 0.70 at 773 K. |
| Author | Zhang, Bo-Ping Zhao, Li-Dong Li, Jing-Feng Lin, Yuan-Hua Xiang, Kai Nan, Ce-Wen Liu, Yong Li, Fu Zhu, Hong-Min |
| AuthorAffiliation | Department of Chemistry School of Materials Science and Engineering Tsinghua University University of Science and Technology Beijing School of Metallurgical and Ecological Engineering Northwestern University Department of Materials Science and Engineering State Key Laboratory of New Ceramics and Fine Processing |
| AuthorAffiliation_xml | – name: State Key Laboratory of New Ceramics and Fine Processing – name: School of Metallurgical and Ecological Engineering – name: Department of Chemistry – name: School of Materials Science and Engineering – name: University of Science and Technology Beijing – name: Northwestern University – name: Tsinghua University – name: Department of Materials Science and Engineering |
| Author_xml | – sequence: 1 givenname: Fu surname: Li fullname: Li, Fu – sequence: 2 givenname: Jing-Feng surname: Li fullname: Li, Jing-Feng – sequence: 3 givenname: Li-Dong surname: Zhao fullname: Zhao, Li-Dong – sequence: 4 givenname: Kai surname: Xiang fullname: Xiang, Kai – sequence: 5 givenname: Yong surname: Liu fullname: Liu, Yong – sequence: 6 givenname: Bo-Ping surname: Zhang fullname: Zhang, Bo-Ping – sequence: 7 givenname: Yuan-Hua surname: Lin fullname: Lin, Yuan-Hua – sequence: 8 givenname: Ce-Wen surname: Nan fullname: Nan, Ce-Wen – sequence: 9 givenname: Hong-Min surname: Zhu fullname: Zhu, Hong-Min |
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| Snippet | This work revealed that BiCuSeO oxyselenide is a potential oxide-based thermoelectric material, whose dimensionless figure of merit (
ZT
) reaches ∼0.70 at 773... This work revealed that BiCuSeO oxyselenide is a potential oxide-based thermoelectric material, whose dimensionless figure of merit (ZT) reaches similar to... |
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| SubjectTerms | Ball milling Coefficients Figure of merit Phonons Resistivity Spark plasma sintering Thermal conductivity Thermoelectric materials |
| Title | Polycrystalline BiCuSeO oxide as a potential thermoelectric material |
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