Dehydrogenation of propane combined with selective hydrogen combustion over Pt-Sn bimetallic catalysts

Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal dehydrogenation was also carried out as part of the proposed process. Pt/Al 2O 3 modified with Sn and Zn was found to be suitable for both of thes...

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Published inApplied catalysis. A, General Vol. 356; no. 1; pp. 80 - 87
Main Authors Kaneko, Shinji, Arakawa, Tsuyoshi, Ohshima, Masa-aki, Kurokawa, Hideki, Miura, Hiroshi
Format Journal Article
LanguageEnglish
Published Kidlington Elsevier B.V 01.03.2009
Elsevier
Subjects
Catalysis
Chemistry
Dehydrogenation of propane
Exact sciences and technology
General and physical chemistry
Pt-Sn bimetallic catalysts
Selective hydrogen combustion
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
Zn-Al-O support
Zn-Al-O support
Dehydrogenation of propane
Pt-Sn bimetallic catalysts
Selective hydrogen combustion
Mixed catalyst
Binary compound
Composition
Catalytic reaction
Support
Hydrogen
Transition metal
Combustion
Selectivity
Conversion
Equilibrium
Supported catalyst
Optimization
Heterogeneous catalysis
Propene
Dehydrogenation
Platinum
Alumina
Propane
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Abstract Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal dehydrogenation was also carried out as part of the proposed process. Pt/Al 2O 3 modified with Sn and Zn was found to be suitable for both of these two reactions. In the normal dehydrogenation, conversions equal to the calculated equilibrium conversion were achieved with almost complete selectivity for propylene. Optimization of catalyst composition was done by addition of various amounts of Sn to Pt/Al 2O 3 and Pt/Zn-Al-O. For dehydrogenation combined with hydrogen combustion, selective hydrogen combustion was achieved over Pt-Sn bimetallic catalysts. Moreover, a stable conversion higher than that of equilibrium for normal dehydrogenation was obtained using Pt-Sn/Zn-Al-O under certain reaction conditions. Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal dehydrogenation was also carried out as part of the proposed process. Pt/Al 2O 3 modified with Sn and Zn was found to be suitable for both of these two reactions. In the normal dehydrogenation, conversions equal to the calculated equilibrium conversion were achieved with almost complete selectivity for propylene. Optimization of catalyst composition was done by addition of various amounts of Sn to Pt/Al 2O 3 and Pt/Zn-Al-O. For dehydrogenation combined with hydrogen combustion, selective hydrogen combustion was achieved over Pt-Sn bimetallic catalysts. Moreover, a stable conversion higher than that of equilibrium for normal dehydrogenation was obtained using Pt-Sn/Zn-Al-O under certain reaction conditions.
AbstractList Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal dehydrogenation was also carried out as part of the proposed process. Pt/Al2O3 modified with Sn and Zn was found to be suitable for both of these two reactions. In the normal dehydrogenation, conversions equal to the calculated equilibrium conversion were achieved with almost complete selectivity for propylene. Optimization of catalyst composition was done by addition of various amounts of Sn to Pt/Al2O3 and Pt/Zn-Al-O. For dehydrogenation combined with hydrogen combustion, selective hydrogen combustion was achieved over Pt-Sn bimetallic catalysts. Moreover, a stable conversion higher than that of equilibrium for normal dehydrogenation was obtained using Pt-Sn/Zn-Al-O under certain reaction conditions.
Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal dehydrogenation was also carried out as part of the proposed process. Pt/Al 2O 3 modified with Sn and Zn was found to be suitable for both of these two reactions. In the normal dehydrogenation, conversions equal to the calculated equilibrium conversion were achieved with almost complete selectivity for propylene. Optimization of catalyst composition was done by addition of various amounts of Sn to Pt/Al 2O 3 and Pt/Zn-Al-O. For dehydrogenation combined with hydrogen combustion, selective hydrogen combustion was achieved over Pt-Sn bimetallic catalysts. Moreover, a stable conversion higher than that of equilibrium for normal dehydrogenation was obtained using Pt-Sn/Zn-Al-O under certain reaction conditions. Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal dehydrogenation was also carried out as part of the proposed process. Pt/Al 2O 3 modified with Sn and Zn was found to be suitable for both of these two reactions. In the normal dehydrogenation, conversions equal to the calculated equilibrium conversion were achieved with almost complete selectivity for propylene. Optimization of catalyst composition was done by addition of various amounts of Sn to Pt/Al 2O 3 and Pt/Zn-Al-O. For dehydrogenation combined with hydrogen combustion, selective hydrogen combustion was achieved over Pt-Sn bimetallic catalysts. Moreover, a stable conversion higher than that of equilibrium for normal dehydrogenation was obtained using Pt-Sn/Zn-Al-O under certain reaction conditions.
Author Ohshima, Masa-aki
Arakawa, Tsuyoshi
Miura, Hiroshi
Kaneko, Shinji
Kurokawa, Hideki
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Issue 1
Keywords Zn-Al-O support
Dehydrogenation of propane
Pt-Sn bimetallic catalysts
Selective hydrogen combustion
Mixed catalyst
Binary compound
Composition
Catalytic reaction
Support
Hydrogen
Transition metal
Combustion
Selectivity
Conversion
Equilibrium
Supported catalyst
Optimization
Heterogeneous catalysis
Propene
Dehydrogenation
Platinum
Alumina
Propane
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Snippet Dehydrogenation of propane combined with selective hydrogen combustion was studied over supported Pt-Sn bimetallic catalysts. A catalytic test for normal...
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SubjectTerms Catalysis
Chemistry
Dehydrogenation of propane
Exact sciences and technology
General and physical chemistry
Pt-Sn bimetallic catalysts
Selective hydrogen combustion
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
Zn-Al-O support
Title Dehydrogenation of propane combined with selective hydrogen combustion over Pt-Sn bimetallic catalysts
URI https://dx.doi.org/10.1016/j.apcata.2008.12.022
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