High-capacity graphene oxide/graphite/carbon nanotube composites for use in Li-ion battery anodes

A composite of graphene oxide sheets, carbon nanotubes (CNTs), and commercial graphite particles was prepared. The composite’s use as a high-capacity and binder-free anode material for Li-ion batteries was examined. Results showed that this novel composite had a very high reversible Li-storage capac...

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Published inCarbon (New York) Vol. 74; pp. 153 - 162
Main Authors Zhang, Jingxian, Xie, Zhengwei, Li, Wen, Dong, Shaoqiang, Qu, Meizhen
Format Journal Article
LanguageEnglish
Published Kidlington Elsevier Ltd 01.08.2014
Elsevier
Subjects
Anodes
Applied sciences
Carbon
Carbon nanotubes
Cross-disciplinary physics: materials science; rheology
Direct energy conversion and energy accumulation
Electrical engineering. Electrical power engineering
Electrical power engineering
Electrochemical conversion: primary and secondary batteries, fuel cells
Exact sciences and technology
Fullerenes and related materials; diamonds, graphite
Graphene
Graphite
Lithium-ion batteries
Materials science
Nanocrystalline materials
Nanoscale materials and structures: fabrication and characterization
Nanotubes
Oxides
Particulate composites
Physics
Specific materials
Lithium battery
Composite materials
Graphite
Carbon nanotubes
Ions
Carbon fiber reinforced plastics
Graphene oxide
Anodes
Nanostructured materials
Particles
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Abstract A composite of graphene oxide sheets, carbon nanotubes (CNTs), and commercial graphite particles was prepared. The composite’s use as a high-capacity and binder-free anode material for Li-ion batteries was examined. Results showed that this novel composite had a very high reversible Li-storage capacity of 1172.5mAhg−1 at 0.5C (1C=372mAg−1), which is thrice that of commercial graphite anode. The composite also exceeded the theoretical sum of capacities of the three ingredients. More importantly, its reversible capacity below 0.25V can reach up to 600mAhg−1. In summary, the graphene oxide/graphite/CNT composite had higher reversible capacity, better cycling performance, and similar rate capability compared with the graphene oxide/graphite composite.
AbstractList A composite of graphene oxide sheets, carbon nanotubes (CNTs), and commercial graphite particles was prepared. The composite’s use as a high-capacity and binder-free anode material for Li-ion batteries was examined. Results showed that this novel composite had a very high reversible Li-storage capacity of 1172.5mAhg−1 at 0.5C (1C=372mAg−1), which is thrice that of commercial graphite anode. The composite also exceeded the theoretical sum of capacities of the three ingredients. More importantly, its reversible capacity below 0.25V can reach up to 600mAhg−1. In summary, the graphene oxide/graphite/CNT composite had higher reversible capacity, better cycling performance, and similar rate capability compared with the graphene oxide/graphite composite.
A composite of graphene oxide sheets, carbon nanotubes (CNTs), and commercial graphite particles was prepared. The composite's use as a high-capacity and binder-free anode material for Li-ion batteries was examined. Results showed that this novel composite had a very high reversible Li-storage capacity of 1172.5 mA h g super(-1) at 0.5C (1C = 372 mA g super(-1)), which is thrice that of commercial graphite anode. The composite also exceeded the theoretical sum of capacities of the three ingredients. More importantly, its reversible capacity below 0.25 V can reach up to 600 mA h g super(-1). In summary, the graphene oxide/graphite/CNT composite had higher reversible capacity, better cycling performance, and similar rate capability compared with the graphene oxide/graphite composite.
Author Zhang, Jingxian
Xie, Zhengwei
Li, Wen
Dong, Shaoqiang
Qu, Meizhen
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  orcidid: 0000-0002-0542-0317
  surname: Xie
  fullname: Xie, Zhengwei
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  organization: Chengdu Institute of Organic Chemistry, Chinese Academy of Sciences, Chengdu 610041, PR China
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  givenname: Shaoqiang
  surname: Dong
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Composite materials
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Ions
Carbon fiber reinforced plastics
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Anodes
Nanostructured materials
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SSID ssj0004814
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Snippet A composite of graphene oxide sheets, carbon nanotubes (CNTs), and commercial graphite particles was prepared. The composite’s use as a high-capacity and...
A composite of graphene oxide sheets, carbon nanotubes (CNTs), and commercial graphite particles was prepared. The composite's use as a high-capacity and...
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StartPage 153
SubjectTerms Anodes
Applied sciences
Carbon
Carbon nanotubes
Cross-disciplinary physics: materials science; rheology
Direct energy conversion and energy accumulation
Electrical engineering. Electrical power engineering
Electrical power engineering
Electrochemical conversion: primary and secondary batteries, fuel cells
Exact sciences and technology
Fullerenes and related materials; diamonds, graphite
Graphene
Graphite
Lithium-ion batteries
Materials science
Nanocrystalline materials
Nanoscale materials and structures: fabrication and characterization
Nanotubes
Oxides
Particulate composites
Physics
Specific materials
Title High-capacity graphene oxide/graphite/carbon nanotube composites for use in Li-ion battery anodes
URI https://dx.doi.org/10.1016/j.carbon.2014.03.017
https://search.proquest.com/docview/1560125633
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