Mechanochemistry: an efficient and versatile toolbox for synthesis, transformation, and functionalization of porous metal-organic frameworks
Mechanochemistry is nowadays recognized as a green approach to chemical synthesis, but the full scope of the accompanying solid-state reactivity is just beginning to be unravelled. This is especially true for the preparation of porous metal-organic frameworks, whose synthesis by the use of mechanica...
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| Published in | CrystEngComm Vol. 22; no. 27; pp. 4511 - 4525 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
Cambridge
Royal Society of Chemistry
01.01.2020
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Mechanochemistry is nowadays recognized as a green approach to chemical synthesis, but the full scope of the accompanying solid-state reactivity is just beginning to be unravelled. This is especially true for the preparation of porous metal-organic frameworks, whose synthesis by the use of mechanical force lagged behind that of other relevant classes of materials. Nevertheless, mechanochemical procedures have rapidly evolved from a mere synthetic curiosity towards efficient methods for obtaining high-quality MOFs on different scales. This Highlight is dedicated to the functional approach of using mechanochemistry for the preparation of catalytically active MOF composites and mixed-metal and mixed-ligand MOFs with synergistic properties as well as fine-tuning of the MOF performance
via
defect engineering and amorphization.
Multiple ways in which the synergy of mechanochemistry and MOFs advances the field of materials chemistry are presented here. |
|---|---|
| AbstractList | Mechanochemistry is nowadays recognized as a green approach to chemical synthesis, but the full scope of the accompanying solid-state reactivity is just beginning to be unravelled. This is especially true for the preparation of porous metal–organic frameworks, whose synthesis by the use of mechanical force lagged behind that of other relevant classes of materials. Nevertheless, mechanochemical procedures have rapidly evolved from a mere synthetic curiosity towards efficient methods for obtaining high-quality MOFs on different scales. This Highlight is dedicated to the functional approach of using mechanochemistry for the preparation of catalytically active MOF composites and mixed-metal and mixed-ligand MOFs with synergistic properties as well as fine-tuning of the MOF performance
via
defect engineering and amorphization. Mechanochemistry is nowadays recognized as a green approach to chemical synthesis, but the full scope of the accompanying solid-state reactivity is just beginning to be unravelled. This is especially true for the preparation of porous metal-organic frameworks, whose synthesis by the use of mechanical force lagged behind that of other relevant classes of materials. Nevertheless, mechanochemical procedures have rapidly evolved from a mere synthetic curiosity towards efficient methods for obtaining high-quality MOFs on different scales. This Highlight is dedicated to the functional approach of using mechanochemistry for the preparation of catalytically active MOF composites and mixed-metal and mixed-ligand MOFs with synergistic properties as well as fine-tuning of the MOF performance via defect engineering and amorphization. Multiple ways in which the synergy of mechanochemistry and MOFs advances the field of materials chemistry are presented here. Mechanochemistry is nowadays recognized as a green approach to chemical synthesis, but the full scope of the accompanying solid-state reactivity is just beginning to be unravelled. This is especially true for the preparation of porous metal–organic frameworks, whose synthesis by the use of mechanical force lagged behind that of other relevant classes of materials. Nevertheless, mechanochemical procedures have rapidly evolved from a mere synthetic curiosity towards efficient methods for obtaining high-quality MOFs on different scales. This Highlight is dedicated to the functional approach of using mechanochemistry for the preparation of catalytically active MOF composites and mixed-metal and mixed-ligand MOFs with synergistic properties as well as fine-tuning of the MOF performance via defect engineering and amorphization. |
| Author | U arevi, Krunoslav Stolar, Tomislav |
| AuthorAffiliation | Ru er Boškovi Institute |
| AuthorAffiliation_xml | – name: Ru er Boškovi Institute |
| Author_xml | – sequence: 1 givenname: Tomislav surname: Stolar fullname: Stolar, Tomislav – sequence: 2 givenname: Krunoslav surname: U arevi fullname: U arevi, Krunoslav |
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| ContentType | Journal Article |
| Copyright | Copyright Royal Society of Chemistry 2020 |
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| Notes | Krunoslav U arevi graduated in 2009 at the University of Zagreb in the field of structural and inorganic chemistry. After a Marie-Curie Newfelpro Fellowship with Prof. Tomislav Friš i at McGill University in Montreal, he started working as a Head of Laboratory for Green Synthesis at Ru er Boškovi Institute in Zagreb in 2016. His main scientific focus is on developing mechanochemical and solvent-free procedures for the synthesis and transformation of various classes of functional materials, from supramolecular receptors and organic compounds to porous metal-organic frameworks (MOFs). A particular part of his research involves designing new milling reactors and developing new methodologies for monitoring of milling and aging reactions. Tomislav Stolar is a PhD candidate at Ru er Boškovi Institute in Zagreb, Croatia under the supervision of Dr. Krunoslav U arevi . He started his scientific career as an undergraduate volunteer at the same institution in 2013. His research interest spans solid-state chemistry, crystal engineering, prebiotic chemistry, mechanochemistry and MOFs. in situ ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 14 |
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| Title | Mechanochemistry: an efficient and versatile toolbox for synthesis, transformation, and functionalization of porous metal-organic frameworks |
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