Modeling the roles of carbon nanotubes and interphase dimensions in the conductivity of nanocomposites

The influences of interphase regions on the percolation threshold and electrical conductivity of nanocomposites polymer/carbon nanotubes (CNT) nanocomposites (PCNT) have been ignored in previous articles, although the interphase layer around CNT can encourage the conductivity. In this paper, the dim...

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Published inResults in physics Vol. 15; p. 102562
Main Authors Zare, Yasser, Yop Rhee, Kyong, Park, Soo-Jin
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.12.2019
Elsevier
Subjects
Electrical conductivity
Interphase
Percolation threshold
Polymer/CNT nanocomposites
Percolation threshold
Electrical conductivity
Interphase
Polymer/CNT nanocomposites
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Abstract The influences of interphase regions on the percolation threshold and electrical conductivity of nanocomposites polymer/carbon nanotubes (CNT) nanocomposites (PCNT) have been ignored in previous articles, although the interphase layer around CNT can encourage the conductivity. In this paper, the dimensions of CNT and surrounding interphase suggest the percolation threshold of CNT in PCNT. The comparisons between predictions and experimental measurements in several samples confirm the suggested equation. Moreover, the effective volume fraction of CNT and the fraction of networked CNT in the presence of interphase zones are expressed. Finally, a model is developed to investigate the roles of CNT and interphase dimensions as well as percolation threshold and CNT conductivity in the conductivity of PCNT. Thin CNT and thick interphase increase the effective volume fraction of nanoparticles in PCNT, whereas the CNT length is ineffective. A thick interphase and a high concentration of thin and long CNT grow the percentage of networked CNT and the conductivity of PCNT. The conductivity directly correlates to the CNT conductivity, while the smallest percolation threshold causes the highest conductivity. Additionally, a high waviness worsens the percolation threshold, the network size and the CNT conductivity resulting in a poor conductivity in nanocomposites.
AbstractList The influences of interphase regions on the percolation threshold and electrical conductivity of nanocomposites polymer/carbon nanotubes (CNT) nanocomposites (PCNT) have been ignored in previous articles, although the interphase layer around CNT can encourage the conductivity. In this paper, the dimensions of CNT and surrounding interphase suggest the percolation threshold of CNT in PCNT. The comparisons between predictions and experimental measurements in several samples confirm the suggested equation. Moreover, the effective volume fraction of CNT and the fraction of networked CNT in the presence of interphase zones are expressed. Finally, a model is developed to investigate the roles of CNT and interphase dimensions as well as percolation threshold and CNT conductivity in the conductivity of PCNT. Thin CNT and thick interphase increase the effective volume fraction of nanoparticles in PCNT, whereas the CNT length is ineffective. A thick interphase and a high concentration of thin and long CNT grow the percentage of networked CNT and the conductivity of PCNT. The conductivity directly correlates to the CNT conductivity, while the smallest percolation threshold causes the highest conductivity. Additionally, a high waviness worsens the percolation threshold, the network size and the CNT conductivity resulting in a poor conductivity in nanocomposites. Keywords: Polymer/CNT nanocomposites, Interphase, Electrical conductivity, Percolation threshold
The influences of interphase regions on the percolation threshold and electrical conductivity of nanocomposites polymer/carbon nanotubes (CNT) nanocomposites (PCNT) have been ignored in previous articles, although the interphase layer around CNT can encourage the conductivity. In this paper, the dimensions of CNT and surrounding interphase suggest the percolation threshold of CNT in PCNT. The comparisons between predictions and experimental measurements in several samples confirm the suggested equation. Moreover, the effective volume fraction of CNT and the fraction of networked CNT in the presence of interphase zones are expressed. Finally, a model is developed to investigate the roles of CNT and interphase dimensions as well as percolation threshold and CNT conductivity in the conductivity of PCNT. Thin CNT and thick interphase increase the effective volume fraction of nanoparticles in PCNT, whereas the CNT length is ineffective. A thick interphase and a high concentration of thin and long CNT grow the percentage of networked CNT and the conductivity of PCNT. The conductivity directly correlates to the CNT conductivity, while the smallest percolation threshold causes the highest conductivity. Additionally, a high waviness worsens the percolation threshold, the network size and the CNT conductivity resulting in a poor conductivity in nanocomposites.
ArticleNumber 102562
Author Zare, Yasser
Yop Rhee, Kyong
Park, Soo-Jin
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Interphase
Polymer/CNT nanocomposites
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Snippet The influences of interphase regions on the percolation threshold and electrical conductivity of nanocomposites polymer/carbon nanotubes (CNT) nanocomposites...
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StartPage 102562
SubjectTerms Electrical conductivity
Interphase
Percolation threshold
Polymer/CNT nanocomposites
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Title Modeling the roles of carbon nanotubes and interphase dimensions in the conductivity of nanocomposites
URI https://dx.doi.org/10.1016/j.rinp.2019.102562
https://doaj.org/article/9ad6bc2271754e5f8d9127494bfb3a24
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