Low-carbon, hydrogen-rich syngas from sorption-enhanced gasification: A review

•Sustainable energy conversion via sorption-enhanced gasification is thoroughly reviewed.•Fundamental reactions and limitations of CaO sorbents are critically examined.•Pilot-scale tests are analyzed to highlight advancements and gaps in SEG research.•Practical challenges and process intensification...

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Published inCarbon Capture Science & Technology Vol. 14; p. 100372
Main Authors Dziva, Godknows, Weitzel, Jonas, Cui, Pengjun, Yew, Maxine, Ding, Guangchao, Zeng, Liang, Li, Songgeng
Format Journal Article
LanguageEnglish
Published Elsevier Ltd 01.03.2025
Elsevier
Subjects
Calcium looping
Carbon capture
Dual fluidized bed
Gasification
Hydrogen
Dual fluidized bed
DFB
SER
WGS
SEWGS
Hydrogen
LEGS
BECCUS
CHP
DFM
SNG
CaL
TRL
RING
HHV
RWGS
DFBG
Gasification
LHV
IGCC
Carbon capture
DME
PSA
CCUS
MO
CaLG
CL
AER
ICCU
MSW
CER
IGCCU
SEG
Calcium looping
CaCL
SMR
TCES
CFB
DRM
BFB
HRSG
Online AccessGet full text

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Abstract •Sustainable energy conversion via sorption-enhanced gasification is thoroughly reviewed.•Fundamental reactions and limitations of CaO sorbents are critically examined.•Pilot-scale tests are analyzed to highlight advancements and gaps in SEG research.•Practical challenges and process intensification strategies are discussed. This review aims to provide a comprehensive overview of sorption-enhanced gasification (SEG) with CaO, highlighting its potential as an efficient and sustainable energy conversion technology. SEG integrates dual bed steam gasification with in situ CO2 removal using CaO, efficiently converting solid carbonaceous fuels such as biomass and low-rank coal into hydrogen-rich (up to 80 vol% H2), low-carbon and tar, medium calorific value and nitrogen-free syngas that can be adapted for various downstream applications. The review details the working principle, operating conditions and reaction mechanisms of SEG, emphasizing how these factors influence product distribution. Calcium sorbents are central to the SEG process, so their reactions, catalytic activity and limitations are discussed in this review. Pilot-scale tests are examined to underscore process engineering advancements as well as to highlight scale-up challenges that currently limit the technology to TRL 5–6. Unsustainable long-term sorbent performance and energy penalties from sorbent regeneration and CO2 capture still need to be addressed through scalable and cost-effective material development and process engineering. This review discusses various process intensification concepts as potential solutions to the inherent shortcomings of SEG. Process systems analyses examined indicate the potential of SEG in hydrogen, synthetic fuel and electricity production, positioning it as a promising technology for decentralized sustainable energy conversion. Furthermore, the review explores the sustainable repurposing and disposal of spent solids to foster circular economies. Overall, this comprehensive review provides crucial insights to further leverage and advance the SEG process, offering a platform for future research and development. [Display omitted]
AbstractList This review aims to provide a comprehensive overview of sorption-enhanced gasification (SEG) with CaO, highlighting its potential as an efficient and sustainable energy conversion technology. SEG integrates dual bed steam gasification with in situ CO2 removal using CaO, efficiently converting solid carbonaceous fuels such as biomass and low-rank coal into hydrogen-rich (up to 80 vol% H2), low-carbon and tar, medium calorific value and nitrogen-free syngas that can be adapted for various downstream applications. The review details the working principle, operating conditions and reaction mechanisms of SEG, emphasizing how these factors influence product distribution. Calcium sorbents are central to the SEG process, so their reactions, catalytic activity and limitations are discussed in this review. Pilot-scale tests are examined to underscore process engineering advancements as well as to highlight scale-up challenges that currently limit the technology to TRL 5–6. Unsustainable long-term sorbent performance and energy penalties from sorbent regeneration and CO2 capture still need to be addressed through scalable and cost-effective material development and process engineering. This review discusses various process intensification concepts as potential solutions to the inherent shortcomings of SEG. Process systems analyses examined indicate the potential of SEG in hydrogen, synthetic fuel and electricity production, positioning it as a promising technology for decentralized sustainable energy conversion. Furthermore, the review explores the sustainable repurposing and disposal of spent solids to foster circular economies. Overall, this comprehensive review provides crucial insights to further leverage and advance the SEG process, offering a platform for future research and development.
•Sustainable energy conversion via sorption-enhanced gasification is thoroughly reviewed.•Fundamental reactions and limitations of CaO sorbents are critically examined.•Pilot-scale tests are analyzed to highlight advancements and gaps in SEG research.•Practical challenges and process intensification strategies are discussed. This review aims to provide a comprehensive overview of sorption-enhanced gasification (SEG) with CaO, highlighting its potential as an efficient and sustainable energy conversion technology. SEG integrates dual bed steam gasification with in situ CO2 removal using CaO, efficiently converting solid carbonaceous fuels such as biomass and low-rank coal into hydrogen-rich (up to 80 vol% H2), low-carbon and tar, medium calorific value and nitrogen-free syngas that can be adapted for various downstream applications. The review details the working principle, operating conditions and reaction mechanisms of SEG, emphasizing how these factors influence product distribution. Calcium sorbents are central to the SEG process, so their reactions, catalytic activity and limitations are discussed in this review. Pilot-scale tests are examined to underscore process engineering advancements as well as to highlight scale-up challenges that currently limit the technology to TRL 5–6. Unsustainable long-term sorbent performance and energy penalties from sorbent regeneration and CO2 capture still need to be addressed through scalable and cost-effective material development and process engineering. This review discusses various process intensification concepts as potential solutions to the inherent shortcomings of SEG. Process systems analyses examined indicate the potential of SEG in hydrogen, synthetic fuel and electricity production, positioning it as a promising technology for decentralized sustainable energy conversion. Furthermore, the review explores the sustainable repurposing and disposal of spent solids to foster circular economies. Overall, this comprehensive review provides crucial insights to further leverage and advance the SEG process, offering a platform for future research and development. [Display omitted]
ArticleNumber 100372
Author Li, Songgeng
Yew, Maxine
Zeng, Liang
Dziva, Godknows
Cui, Pengjun
Weitzel, Jonas
Ding, Guangchao
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  surname: Dziva
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  organization: State Key Laboratory of Mesoscience and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China
– sequence: 2
  givenname: Jonas
  surname: Weitzel
  fullname: Weitzel, Jonas
  organization: Department of Chemical and Process Engineering, University of Canterbury, Christchurch, New Zealand
– sequence: 3
  givenname: Pengjun
  surname: Cui
  fullname: Cui, Pengjun
  organization: Key Laboratory for Green Chemical Technology of the Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
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  givenname: Maxine
  surname: Yew
  fullname: Yew, Maxine
  organization: Tianjin Institute of Industrial Biotechnology, Chinese Academy of Sciences, Tianjin 300308, China
– sequence: 5
  givenname: Guangchao
  surname: Ding
  fullname: Ding, Guangchao
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  fullname: Zeng, Liang
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  organization: Key Laboratory for Green Chemical Technology of the Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China
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  givenname: Songgeng
  surname: Li
  fullname: Li, Songgeng
  email: sgli@ipe.ac.cn
  organization: State Key Laboratory of Mesoscience and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China
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Keywords Dual fluidized bed
DFB
SER
WGS
SEWGS
Hydrogen
LEGS
BECCUS
CHP
DFM
SNG
CaL
TRL
RING
HHV
RWGS
DFBG
Gasification
LHV
IGCC
Carbon capture
DME
PSA
CCUS
MO
CaLG
CL
AER
ICCU
MSW
CER
IGCCU
SEG
Calcium looping
CaCL
SMR
TCES
CFB
DRM
BFB
HRSG
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Snippet •Sustainable energy conversion via sorption-enhanced gasification is thoroughly reviewed.•Fundamental reactions and limitations of CaO sorbents are critically...
This review aims to provide a comprehensive overview of sorption-enhanced gasification (SEG) with CaO, highlighting its potential as an efficient and...
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StartPage 100372
SubjectTerms Calcium looping
Carbon capture
Dual fluidized bed
Gasification
Hydrogen
Title Low-carbon, hydrogen-rich syngas from sorption-enhanced gasification: A review
URI https://dx.doi.org/10.1016/j.ccst.2025.100372
https://doaj.org/article/3d53b01b36a348bb9c26ba4da9141490
Volume 14
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