Adsorption of BiOBr microspheres to rhodamine B and its influence on photocatalytic reaction
Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyr...
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| Published in | Chemosphere (Oxford) Vol. 304; p. 135320 |
|---|---|
| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.10.2022
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyrrolidone (PVP) as additive in this work, and then the adsorption of the BiOBr microspheres to RhB and its influence on the photocatalytic degradation of RhB were investigated in detail. Experimental results show that the BiOBr microspheres have a very strong adsorption capacity to RhB. The adsorption behavior follows the Langmuir model and the quasi second order kinetic equation. Tests of the photocatalytic degradation of RhB under visible irradiation verify that the adsorption of the BiOBr microspheres to RhB greatly boosts the degradation of RhB due to the “enriching effect”, and a complete degradation of 20 mg L−1 RhB only requires 37 min.
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•The adsorption behavior of photocatalyst was detailedly studied using the synthesized BiOBr microspheres.•The adsorption model and parameters were determined through experiments.•The remarkably improved adsorption capacity of BiOBr microspheres was explained through experiments and DFT calculation.•The strong adsorption of the BiOBr microspheres to RhB was proved to facilitate its photodegradation.•This work provides new insights into adsorption phenomenon during photocatalytic degradation of organic dyes. |
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| AbstractList | Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyrrolidone (PVP) as additive in this work, and then the adsorption of the BiOBr microspheres to RhB and its influence on the photocatalytic degradation of RhB were investigated in detail. Experimental results show that the BiOBr microspheres have a very strong adsorption capacity to RhB. The adsorption behavior follows the Langmuir model and the quasi second order kinetic equation. Tests of the photocatalytic degradation of RhB under visible irradiation verify that the adsorption of the BiOBr microspheres to RhB greatly boosts the degradation of RhB due to the “enriching effect”, and a complete degradation of 20 mg L−1 RhB only requires 37 min.
[Display omitted]
•The adsorption behavior of photocatalyst was detailedly studied using the synthesized BiOBr microspheres.•The adsorption model and parameters were determined through experiments.•The remarkably improved adsorption capacity of BiOBr microspheres was explained through experiments and DFT calculation.•The strong adsorption of the BiOBr microspheres to RhB was proved to facilitate its photodegradation.•This work provides new insights into adsorption phenomenon during photocatalytic degradation of organic dyes. Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyrrolidone (PVP) as additive in this work, and then the adsorption of the BiOBr microspheres to RhB and its influence on the photocatalytic degradation of RhB were investigated in detail. Experimental results show that the BiOBr microspheres have a very strong adsorption capacity to RhB. The adsorption behavior follows the Langmuir model and the quasi second order kinetic equation. Tests of the photocatalytic degradation of RhB under visible irradiation verify that the adsorption of the BiOBr microspheres to RhB greatly boosts the degradation of RhB due to the "enriching effect", and a complete degradation of 20 mg L RhB only requires 37 min. Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyrrolidone (PVP) as additive in this work, and then the adsorption of the BiOBr microspheres to RhB and its influence on the photocatalytic degradation of RhB were investigated in detail. Experimental results show that the BiOBr microspheres have a very strong adsorption capacity to RhB. The adsorption behavior follows the Langmuir model and the quasi second order kinetic equation. Tests of the photocatalytic degradation of RhB under visible irradiation verify that the adsorption of the BiOBr microspheres to RhB greatly boosts the degradation of RhB due to the "enriching effect", and a complete degradation of 20 mg L-1 RhB only requires 37 min.Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyrrolidone (PVP) as additive in this work, and then the adsorption of the BiOBr microspheres to RhB and its influence on the photocatalytic degradation of RhB were investigated in detail. Experimental results show that the BiOBr microspheres have a very strong adsorption capacity to RhB. The adsorption behavior follows the Langmuir model and the quasi second order kinetic equation. Tests of the photocatalytic degradation of RhB under visible irradiation verify that the adsorption of the BiOBr microspheres to RhB greatly boosts the degradation of RhB due to the "enriching effect", and a complete degradation of 20 mg L-1 RhB only requires 37 min. Adsorption and its influence are often neglected during photocatalytic degradation of organic pollutants. To call attention to these issues, a novel bismuth oxybromide (BiOBr) microsphere with hierarchical flower-like structure was fabricated through a facile hydrothermal process using polyvinyl pyrrolidone (PVP) as additive in this work, and then the adsorption of the BiOBr microspheres to RhB and its influence on the photocatalytic degradation of RhB were investigated in detail. Experimental results show that the BiOBr microspheres have a very strong adsorption capacity to RhB. The adsorption behavior follows the Langmuir model and the quasi second order kinetic equation. Tests of the photocatalytic degradation of RhB under visible irradiation verify that the adsorption of the BiOBr microspheres to RhB greatly boosts the degradation of RhB due to the “enriching effect”, and a complete degradation of 20 mg L⁻¹ RhB only requires 37 min. |
| ArticleNumber | 135320 |
| Author | Ma, Jian Cao, Yixi Li, Huaming Liang, Congjie Wu, Yingfeng Wang, Chongtai Yang, Chanyu Hua, Yingjie Xu, Hui Zhang, Taisong |
| Author_xml | – sequence: 1 givenname: Congjie surname: Liang fullname: Liang, Congjie organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 2 givenname: Jian surname: Ma fullname: Ma, Jian organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 3 givenname: Yixi surname: Cao fullname: Cao, Yixi organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 4 givenname: Taisong surname: Zhang fullname: Zhang, Taisong organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 5 givenname: Chanyu surname: Yang fullname: Yang, Chanyu organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 6 givenname: Yingfeng surname: Wu fullname: Wu, Yingfeng organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 7 givenname: Huaming surname: Li fullname: Li, Huaming organization: Institute for Energy Research, School of the Environment and Safety Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 8 givenname: Hui surname: Xu fullname: Xu, Hui organization: Institute for Energy Research, School of the Environment and Safety Engineering, Jiangsu University, Zhenjiang, 212013, PR China – sequence: 9 givenname: Yingjie surname: Hua fullname: Hua, Yingjie email: 521000hua282@sina.com organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China – sequence: 10 givenname: Chongtai orcidid: 0000-0001-7769-8580 surname: Wang fullname: Wang, Chongtai email: oehy2014@163.com organization: School of Chemistry and Chemical Engineering of Hainan Normal University, Key Laboratory of Electrochemical Energy Storage and Energy Conversion of Hainan Province, Key Laboratory of Electrochemical Energy Storage and Light Energy Conversion Materials of Haikou City, Haikou, 571158, PR China |
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| SubjectTerms | Adsorption BiOBr microspheres bismuth equations Hierarchical structure irradiation microparticles Photocatalysis polyvinylpyrrolidone Rhodamine B rhodamines sorption isotherms |
| Title | Adsorption of BiOBr microspheres to rhodamine B and its influence on photocatalytic reaction |
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