Geopolymer for use in heavy metals adsorption, and advanced oxidative processes: A critical review
Geopolymer is a ceramic material, most often amorphous; finds applications in fire- and heat-resistant coatings and adhesives, medicines, refractory ceramics and binders, and manufacturing of radioactive waste container. Over the last decade, new cement based on geopolymers has been developed. Most...
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| Published in | Journal of cleaner production Vol. 213; pp. 42 - 58 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
10.03.2019
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0959-6526 1879-1786 |
| DOI | 10.1016/j.jclepro.2018.12.145 |
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| Abstract | Geopolymer is a ceramic material, most often amorphous; finds applications in fire- and heat-resistant coatings and adhesives, medicines, refractory ceramics and binders, and manufacturing of radioactive waste container. Over the last decade, new cement based on geopolymers has been developed. Most relevant to this review is the fact that its porous nature and chemical similarity to zeolites is being employed for applications pertaining to wastewater treatment. Most of the work has been on the adsorptive treatment of water. However, using chemical reasoning and literature available we show that geopolymers have relevance for further activity on additional areas of relevance to waste water treatment such as photocatalysis, disinfection, and H2-energy production from waste water etc. These applications would depend strongly on the properties of geopolymers, which in turn would rely on the precursors employed and the synthetic methods used. The relevance of geopolymers for cleaner production is also highlighted. The use of fly ashes and metakaolin composites for the fabrication and surface tailoring of geopolymers (perhaps using relevant surfactants) is suggested as a plausible step in the right direction. Given the critical analysis of the state of the art, and the plausible directions identified, this article will benefit environmental scientists, engineers and chemists interested in deploying geopolymers for environmental remediation purposes. However moving forward, barriers are to be anticipated for the large scale implementation of geopolymers. Several barriers (e.g. legal, economical, technocrats and synthetic challenges) that are likely to hinder future research and translation are highlighted.
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•(i) Raw materials, and (ii) synthetic/process parameters influence geopolymer properties.•Properties relevant for H2-production and photodegradation are elaborated.•Filler-materials from wastes relevant for catalytic-enhancement are identified.•Heavy-metal removal using geopolymers: methods and mechanisms are elucidated.•Technology barriers of relevance to all stake holders are projected. |
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| AbstractList | Geopolymer is a ceramic material, most often amorphous; finds applications in fire- and heat-resistant coatings and adhesives, medicines, refractory ceramics and binders, and manufacturing of radioactive waste container. Over the last decade, new cement based on geopolymers has been developed. Most relevant to this review is the fact that its porous nature and chemical similarity to zeolites is being employed for applications pertaining to wastewater treatment. Most of the work has been on the adsorptive treatment of water. However, using chemical reasoning and literature available we show that geopolymers have relevance for further activity on additional areas of relevance to waste water treatment such as photocatalysis, disinfection, and H2-energy production from waste water etc. These applications would depend strongly on the properties of geopolymers, which in turn would rely on the precursors employed and the synthetic methods used. The relevance of geopolymers for cleaner production is also highlighted. The use of fly ashes and metakaolin composites for the fabrication and surface tailoring of geopolymers (perhaps using relevant surfactants) is suggested as a plausible step in the right direction. Given the critical analysis of the state of the art, and the plausible directions identified, this article will benefit environmental scientists, engineers and chemists interested in deploying geopolymers for environmental remediation purposes. However moving forward, barriers are to be anticipated for the large scale implementation of geopolymers. Several barriers (e.g. legal, economical, technocrats and synthetic challenges) that are likely to hinder future research and translation are highlighted.
▪
•(i) Raw materials, and (ii) synthetic/process parameters influence geopolymer properties.•Properties relevant for H2-production and photodegradation are elaborated.•Filler-materials from wastes relevant for catalytic-enhancement are identified.•Heavy-metal removal using geopolymers: methods and mechanisms are elucidated.•Technology barriers of relevance to all stake holders are projected. Geopolymer is a ceramic material, most often amorphous; finds applications in fire- and heat-resistant coatings and adhesives, medicines, refractory ceramics and binders, and manufacturing of radioactive waste container. Over the last decade, new cement based on geopolymers has been developed. Most relevant to this review is the fact that its porous nature and chemical similarity to zeolites is being employed for applications pertaining to wastewater treatment. Most of the work has been on the adsorptive treatment of water. However, using chemical reasoning and literature available we show that geopolymers have relevance for further activity on additional areas of relevance to waste water treatment such as photocatalysis, disinfection, and H₂-energy production from waste water etc. These applications would depend strongly on the properties of geopolymers, which in turn would rely on the precursors employed and the synthetic methods used. The relevance of geopolymers for cleaner production is also highlighted. The use of fly ashes and metakaolin composites for the fabrication and surface tailoring of geopolymers (perhaps using relevant surfactants) is suggested as a plausible step in the right direction. Given the critical analysis of the state of the art, and the plausible directions identified, this article will benefit environmental scientists, engineers and chemists interested in deploying geopolymers for environmental remediation purposes. However moving forward, barriers are to be anticipated for the large scale implementation of geopolymers. Several barriers (e.g. legal, economical, technocrats and synthetic challenges) that are likely to hinder future research and translation are highlighted. |
| Author | Bingxue, Zhang Guarecuco, Rohiverth Minghui, Yang Thomas, Tiju Rasaki, Sefiu Abolaji |
| Author_xml | – sequence: 1 givenname: Sefiu Abolaji surname: Rasaki fullname: Rasaki, Sefiu Abolaji organization: Solid State Functional Materials Research Laboratory, Ningbo Institute of Materials Technology and Engineering (NIMTE), Chinese Academy of Sciences (CAS), 315201, Ningbo, China – sequence: 2 givenname: Zhang surname: Bingxue fullname: Bingxue, Zhang organization: Solid State Functional Materials Research Laboratory, Ningbo Institute of Materials Technology and Engineering (NIMTE), Chinese Academy of Sciences (CAS), 315201, Ningbo, China – sequence: 3 givenname: Rohiverth surname: Guarecuco fullname: Guarecuco, Rohiverth organization: Department of Chemistry & Chemical Biology Cornell University, Ithaca, NY 14853, United States – sequence: 4 givenname: Tiju surname: Thomas fullname: Thomas, Tiju email: tijuthomas@iitm.ac.in organization: Department of Metallurgical and Materials Engineering, Indian Institute of Technology Madras Adyar, Chennai 600036, Tamil Nadu, India – sequence: 5 givenname: Yang surname: Minghui fullname: Minghui, Yang email: myang@nimte.ac.cn organization: Solid State Functional Materials Research Laboratory, Ningbo Institute of Materials Technology and Engineering (NIMTE), Chinese Academy of Sciences (CAS), 315201, Ningbo, China |
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| SubjectTerms | adhesives Adsorbent adsorption Antibacterial activity cement ceramics coatings disinfection Fly ash heavy metals manufacturing Metakaolin-geopolymer photocatalysis Photocatalytic support polymers radioactive waste remediation surfactants wastewater wastewater treatment zeolites |
| Title | Geopolymer for use in heavy metals adsorption, and advanced oxidative processes: A critical review |
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