Constructing N, P-dually doped biochar materials from biomass wastes for high-performance bifunctional oxygen electrocatalysts
The large scale lignocellulosic biomass wastes could also be regarded as abundantly-available renewable resources, and how to convert them into value-added products via sustainable approaches is still a big challenge. In this work, we demonstrated a facile pyrolysis method to construct N, P-dually d...
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| Published in | Chemosphere (Oxford) Vol. 278; p. 130508 |
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| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier Ltd
01.09.2021
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| Subjects | |
| Online Access | Get full text |
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| Abstract | The large scale lignocellulosic biomass wastes could also be regarded as abundantly-available renewable resources, and how to convert them into value-added products via sustainable approaches is still a big challenge. In this work, we demonstrated a facile pyrolysis method to construct N, P-dually doped biochar materials from the lignocellulosic biomass wastes. The as-synthesized N, P-dually doped biochar samples could act as electrocatalysts for oxygen reduction and evolution reactions (ORR/OER), showing excellent catalytic performance and long-term durability, as well as robust tolerance to CO and methanol. The unique hierarchical porous structure, favorable electronic structure modified by the N and P doping, as well as a variety of defect sites induced by the N and P doping into the carbon framework were identified as the main contributions to the prominent catalytic activity of the as-synthesized N, P-dually doped biochar materials. We expect this work would spur more efforts into developing advanced materials from the large scale lignocellulosic biomass wastes.
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•N, P doped biochar was synthesized via a facile thermochemical method from biomass wastes.•The N, P doped biochar exhibited robust bifunctional electrocatalytic activity.•The unique porous structure and electronic structure were attributed to its excellent activity. |
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| AbstractList | The large scale lignocellulosic biomass wastes could also be regarded as abundantly-available renewable resources, and how to convert them into value-added products via sustainable approaches is still a big challenge. In this work, we demonstrated a facile pyrolysis method to construct N, P-dually doped biochar materials from the lignocellulosic biomass wastes. The as-synthesized N, P-dually doped biochar samples could act as electrocatalysts for oxygen reduction and evolution reactions (ORR/OER), showing excellent catalytic performance and long-term durability, as well as robust tolerance to CO and methanol. The unique hierarchical porous structure, favorable electronic structure modified by the N and P doping, as well as a variety of defect sites induced by the N and P doping into the carbon framework were identified as the main contributions to the prominent catalytic activity of the as-synthesized N, P-dually doped biochar materials. We expect this work would spur more efforts into developing advanced materials from the large scale lignocellulosic biomass wastes. The large scale lignocellulosic biomass wastes could also be regarded as abundantly-available renewable resources, and how to convert them into value-added products via sustainable approaches is still a big challenge. In this work, we demonstrated a facile pyrolysis method to construct N, P-dually doped biochar materials from the lignocellulosic biomass wastes. The as-synthesized N, P-dually doped biochar samples could act as electrocatalysts for oxygen reduction and evolution reactions (ORR/OER), showing excellent catalytic performance and long-term durability, as well as robust tolerance to CO and methanol. The unique hierarchical porous structure, favorable electronic structure modified by the N and P doping, as well as a variety of defect sites induced by the N and P doping into the carbon framework were identified as the main contributions to the prominent catalytic activity of the as-synthesized N, P-dually doped biochar materials. We expect this work would spur more efforts into developing advanced materials from the large scale lignocellulosic biomass wastes. [Display omitted] •N, P doped biochar was synthesized via a facile thermochemical method from biomass wastes.•The N, P doped biochar exhibited robust bifunctional electrocatalytic activity.•The unique porous structure and electronic structure were attributed to its excellent activity. The large scale lignocellulosic biomass wastes could also be regarded as abundantly-available renewable resources, and how to convert them into value-added products via sustainable approaches is still a big challenge. In this work, we demonstrated a facile pyrolysis method to construct N, P-dually doped biochar materials from the lignocellulosic biomass wastes. The as-synthesized N, P-dually doped biochar samples could act as electrocatalysts for oxygen reduction and evolution reactions (ORR/OER), showing excellent catalytic performance and long-term durability, as well as robust tolerance to CO and methanol. The unique hierarchical porous structure, favorable electronic structure modified by the N and P doping, as well as a variety of defect sites induced by the N and P doping into the carbon framework were identified as the main contributions to the prominent catalytic activity of the as-synthesized N, P-dually doped biochar materials. We expect this work would spur more efforts into developing advanced materials from the large scale lignocellulosic biomass wastes.The large scale lignocellulosic biomass wastes could also be regarded as abundantly-available renewable resources, and how to convert them into value-added products via sustainable approaches is still a big challenge. In this work, we demonstrated a facile pyrolysis method to construct N, P-dually doped biochar materials from the lignocellulosic biomass wastes. The as-synthesized N, P-dually doped biochar samples could act as electrocatalysts for oxygen reduction and evolution reactions (ORR/OER), showing excellent catalytic performance and long-term durability, as well as robust tolerance to CO and methanol. The unique hierarchical porous structure, favorable electronic structure modified by the N and P doping, as well as a variety of defect sites induced by the N and P doping into the carbon framework were identified as the main contributions to the prominent catalytic activity of the as-synthesized N, P-dually doped biochar materials. We expect this work would spur more efforts into developing advanced materials from the large scale lignocellulosic biomass wastes. |
| ArticleNumber | 130508 |
| Author | Liu, Wu-Jun Li, Hong-Chao Yu, Han-Qing Lam, Paul K.S. Ma, Lin-Lin Hu, Xiao Zeng, Raymond Jianxiong |
| Author_xml | – sequence: 1 givenname: Lin-Lin surname: Ma fullname: Ma, Lin-Lin organization: Department of Environmental Science & Engineering, University of Science & Technology of China, Hefei, 230026, China – sequence: 2 givenname: Xiao surname: Hu fullname: Hu, Xiao organization: Department of Environmental Science & Engineering, University of Science & Technology of China, Hefei, 230026, China – sequence: 3 givenname: Wu-Jun surname: Liu fullname: Liu, Wu-Jun email: liuwujun@mail.ustc.edu.cn organization: Department of Environmental Science & Engineering, University of Science & Technology of China, Hefei, 230026, China – sequence: 4 givenname: Hong-Chao surname: Li fullname: Li, Hong-Chao organization: Department of Environmental Science & Engineering, University of Science & Technology of China, Hefei, 230026, China – sequence: 5 givenname: Paul K.S. orcidid: 0000-0002-2134-3710 surname: Lam fullname: Lam, Paul K.S. organization: USTC-CityU Joint Advanced Research Center, Suzhou, China – sequence: 6 givenname: Raymond Jianxiong surname: Zeng fullname: Zeng, Raymond Jianxiong organization: Centre of Wastewater Resource Recovery, College of Resources and Environment, Fujian Agriculture and Forestry University, Fuzhou, China – sequence: 7 givenname: Han-Qing surname: Yu fullname: Yu, Han-Qing email: hqyu@ustc.edu.cn organization: Department of Environmental Science & Engineering, University of Science & Technology of China, Hefei, 230026, China |
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| Keywords | Pyrolysis Oxygen evolution reaction Biochar Biomass wastes Oxygen reduction reaction |
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| SubjectTerms | Biochar biomass Biomass wastes carbon catalytic activity durability lignocellulose methanol oxygen Oxygen evolution reaction Oxygen reduction reaction Pyrolysis value added |
| Title | Constructing N, P-dually doped biochar materials from biomass wastes for high-performance bifunctional oxygen electrocatalysts |
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