An Adjustable‐Porosity Plastic Crystal Electrolyte Enables High‐Performance All‐Solid‐State Lithium‐Oxygen Batteries

• Published in: Angewandte Chemie International Edition Vol. 59; no. 24; pp. 9382 - 9387
• Main Authors: Wang, Jin, Huang, Gang, Chen, Kai, Zhang, Xin‐Bo
• Format: Journal Article
• Language: English
• Published: Germany Wiley Subscription Services, Inc 08.06.2020
• Edition: International ed. in English
• Subjects: all-solid-state; Cathodes; Electrolytes; High resistance; Lithium; lithium-oxygen batteries; Molten salt electrolytes; Oxygen; Phase separation; plastic crystal electrolytes; Porosity; Softness; Solid electrolytes; Specific capacity; succinonitrile; lithium-oxygen batteries; succinonitrile; all-solid-state; plastic crystal electrolytes; solid electrolytes

The limited triple‐phase boundaries (TPBs) in solid‐state cathodes (SSCs) and high resistance imposed by solid electrolytes (SEs) make the achievement of high‐performance all‐solid‐state lithium‐oxygen (ASS Li‐O2) batteries a challenge. Herein, an adjustable‐porosity plastic crystal electrolyte (PCE...