Stepped Channels Integrated Lithium–Sulfur Separator via Photoinduced Multidimensional Fabrication of Metal–Organic Frameworks
Multidimensional fabrication of metal–organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li‐S separators. Such separators have advantages in pore‐engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the L...
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| Published in | Angewandte Chemie International Edition Vol. 60; no. 18; pp. 10147 - 10154 |
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| Main Authors | , , , , , , , , , |
| Format | Journal Article |
| Language | English |
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26.04.2021
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| Edition | International ed. in English |
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| Abstract | Multidimensional fabrication of metal–organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li‐S separators. Such separators have advantages in pore‐engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li+/electrolyte transfer in Li‐S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li+ transfer across the separators. A photoinduced heat‐assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double‐or triple‐layer membranes). For the first time, a triple‐layer separator with stepped‐channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g−1) and cycling performance (0.03 % fading per cycle from 100th to 700th cycle), which is superior to single/double‐layer and commercial separators. The findings may expedite the development of MOF‐based membranes and extend the scope of MOFs in energy‐storage technologies.
A two‐step photoinduced heat‐assisted processing (PHAP) method is proposed to fabricate a kind of metal–organic framework (MOF)‐based triple‐layer membrane with stepped channels. The membrane can be applied as a high performance separator in a lithium–sulfur battery. |
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| AbstractList | Multidimensional fabrication of metal–organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li‐S separators. Such separators have advantages in pore‐engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li+/electrolyte transfer in Li‐S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li+ transfer across the separators. A photoinduced heat‐assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double‐or triple‐layer membranes). For the first time, a triple‐layer separator with stepped‐channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g−1) and cycling performance (0.03 % fading per cycle from 100th to 700th cycle), which is superior to single/double‐layer and commercial separators. The findings may expedite the development of MOF‐based membranes and extend the scope of MOFs in energy‐storage technologies.
A two‐step photoinduced heat‐assisted processing (PHAP) method is proposed to fabricate a kind of metal–organic framework (MOF)‐based triple‐layer membrane with stepped channels. The membrane can be applied as a high performance separator in a lithium–sulfur battery. Multidimensional fabrication of metal–organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li‐S separators. Such separators have advantages in pore‐engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li+/electrolyte transfer in Li‐S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li+ transfer across the separators. A photoinduced heat‐assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double‐or triple‐layer membranes). For the first time, a triple‐layer separator with stepped‐channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g−1) and cycling performance (0.03 % fading per cycle from 100th to 700th cycle), which is superior to single/double‐layer and commercial separators. The findings may expedite the development of MOF‐based membranes and extend the scope of MOFs in energy‐storage technologies. Multidimensional fabrication of metal-organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li-S separators. Such separators have advantages in pore-engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li+ /electrolyte transfer in Li-S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li+ transfer across the separators. A photoinduced heat-assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double-or triple-layer membranes). For the first time, a triple-layer separator with stepped-channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g-1 ) and cycling performance (0.03 % fading per cycle from 100th to 700th cycle), which is superior to single/double-layer and commercial separators. The findings may expedite the development of MOF-based membranes and extend the scope of MOFs in energy-storage technologies.Multidimensional fabrication of metal-organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li-S separators. Such separators have advantages in pore-engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li+ /electrolyte transfer in Li-S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li+ transfer across the separators. A photoinduced heat-assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double-or triple-layer membranes). For the first time, a triple-layer separator with stepped-channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g-1 ) and cycling performance (0.03 % fading per cycle from 100th to 700th cycle), which is superior to single/double-layer and commercial separators. The findings may expedite the development of MOF-based membranes and extend the scope of MOFs in energy-storage technologies. Multidimensional fabrication of metal–organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li‐S separators. Such separators have advantages in pore‐engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li + /electrolyte transfer in Li‐S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li + transfer across the separators. A photoinduced heat‐assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double‐or triple‐layer membranes). For the first time, a triple‐layer separator with stepped‐channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g −1 ) and cycling performance (0.03 % fading per cycle from 100 th to 700 th cycle), which is superior to single/double‐layer and commercial separators. The findings may expedite the development of MOF‐based membranes and extend the scope of MOFs in energy‐storage technologies. Multidimensional fabrication of metal-organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li-S separators. Such separators have advantages in pore-engineering that might fulfill requirements such as intercepting the diffusing polysulfides and improving the Li /electrolyte transfer in Li-S batteries. However, most reported works focus on the roles of MOFs as ionic sieves for polysulfides while offering limited investigation on the tuning of Li transfer across the separators. A photoinduced heat-assisted processing strategy is proposed to fabricate MOFs into multidimensional devices (e.g., hollow/Janus fibers, double-or triple-layer membranes). For the first time, a triple-layer separator with stepped-channels has been designed and demonstrated as a powerful separator with outstanding specific capacity (1365.0 mAh g ) and cycling performance (0.03 % fading per cycle from 100 to 700 cycle), which is superior to single/double-layer and commercial separators. The findings may expedite the development of MOF-based membranes and extend the scope of MOFs in energy-storage technologies. |
| Author | Chen, Yifa Jiang, Cheng Ma, Huiyuan Wang, Si‐Bo Lan, Ya‐Qian Zhang, Yu Gao, Guang‐Kuo Yang, Ru‐Xin Wang, Yi‐Rong Wei, Mei‐Jie |
| Author_xml | – sequence: 1 givenname: Guang‐Kuo surname: Gao fullname: Gao, Guang‐Kuo organization: Harbin University of Science and Technology – sequence: 2 givenname: Yi‐Rong surname: Wang fullname: Wang, Yi‐Rong organization: Nanjing Normal University – sequence: 3 givenname: Si‐Bo surname: Wang fullname: Wang, Si‐Bo organization: Nanjing Normal University – sequence: 4 givenname: Ru‐Xin surname: Yang fullname: Yang, Ru‐Xin organization: Nanjing Normal University – sequence: 5 givenname: Yifa surname: Chen fullname: Chen, Yifa email: chyf927821@163.com organization: Nanjing Normal University – sequence: 6 givenname: Yu surname: Zhang fullname: Zhang, Yu organization: Nanjing Normal University – sequence: 7 givenname: Cheng surname: Jiang fullname: Jiang, Cheng organization: Nanjing Normal University – sequence: 8 givenname: Mei‐Jie surname: Wei fullname: Wei, Mei‐Jie organization: Nanjing Normal University – sequence: 9 givenname: Huiyuan surname: Ma fullname: Ma, Huiyuan organization: Harbin University of Science and Technology – sequence: 10 givenname: Ya‐Qian orcidid: 0000-0002-2140-7980 surname: Lan fullname: Lan, Ya‐Qian email: yqlan@m.scnu.edu.cn, yqlan@njnu.edu.cn organization: Nanjing Normal University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/33511739$$D View this record in MEDLINE/PubMed |
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| Keywords | Li-S battery stepped channel separators mixed matrix membranes metal-organic frameworks |
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| Snippet | Multidimensional fabrication of metal–organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li‐S separators. Such... Multidimensional fabrication of metal-organic frameworks (MOFs) into multilevel channel integrated devices are in high demanded for Li-S separators. Such... |
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| SubjectTerms | Channels Energy storage Fabrication Li-S battery Lithium Membranes Metal-organic frameworks mixed matrix membranes Polysulfides Separators Specific capacity stepped channel separators Sulfur |
| Title | Stepped Channels Integrated Lithium–Sulfur Separator via Photoinduced Multidimensional Fabrication of Metal–Organic Frameworks |
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